Recent Advances in the Development of Water Oxidation Electrocatalysts at Mild pH

Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water‐oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral o...

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Published inSmall (Weinheim an der Bergstrasse, Germany) Vol. 15; no. 13; pp. e1805103 - n/a
Main Authors Li, Peipei, Zhao, Runbo, Chen, Hongyu, Wang, Huanbo, Wei, Peipei, Huang, Hong, Liu, Qian, Li, Tingshuai, Shi, Xifeng, Zhang, Youyu, Liu, Meiling, Sun, Xuping
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.03.2019
Subjects
Anodizing
Catalysis
earth‐abundant metals
Electrocatalysts
mild pH
Nanotechnology
Organic chemistry
Oxidation
oxygen evolution reaction (OER)
Oxygen evolution reactions
water oxidation
Water splitting
electrocatalysts
water oxidation
oxygen evolution reaction (OER)
mild pH
earth-abundant metals
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Abstract Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water‐oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral or near neutral conditions are more environmentally friendly with less corrosion issues. This review starts with a brief introduction of OER, the importance of OER in mild‐pH media, as well as the fundamentals and performance parameters of OER electrocatalysts. Then, recent progress of the rational design of electrocatalysts for OER in mild‐pH conditions is discussed. The chemical structures or components, synthetic approaches, and catalytic performances of the OER catalysts will be reviewed. Some interesting insights into the catalytic mechanism are also included and discussed. It concludes with a brief outlook on the possible remaining challenges and future trends of neutral or near‐neutral OER electrocatalysts. It hopefully provides the readers with a distinct perspective of the history, present, and future of OER electrocatalysts at mild conditions. Electrocatalytic water oxidation under environmentally‐friendly conditions has received considerable recent research attention. This paper reviews recent advances in the design and development of water oxidation electrocatalysts operating at mild pH, and current challenges and future research directions are also provided.
AbstractList Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water-oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral or near neutral conditions are more environmentally friendly with less corrosion issues. This review starts with a brief introduction of OER, the importance of OER in mild-pH media, as well as the fundamentals and performance parameters of OER electrocatalysts. Then, recent progress of the rational design of electrocatalysts for OER in mild-pH conditions is discussed. The chemical structures or components, synthetic approaches, and catalytic performances of the OER catalysts will be reviewed. Some interesting insights into the catalytic mechanism are also included and discussed. It concludes with a brief outlook on the possible remaining challenges and future trends of neutral or near-neutral OER electrocatalysts. It hopefully provides the readers with a distinct perspective of the history, present, and future of OER electrocatalysts at mild conditions.Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water-oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral or near neutral conditions are more environmentally friendly with less corrosion issues. This review starts with a brief introduction of OER, the importance of OER in mild-pH media, as well as the fundamentals and performance parameters of OER electrocatalysts. Then, recent progress of the rational design of electrocatalysts for OER in mild-pH conditions is discussed. The chemical structures or components, synthetic approaches, and catalytic performances of the OER catalysts will be reviewed. Some interesting insights into the catalytic mechanism are also included and discussed. It concludes with a brief outlook on the possible remaining challenges and future trends of neutral or near-neutral OER electrocatalysts. It hopefully provides the readers with a distinct perspective of the history, present, and future of OER electrocatalysts at mild conditions.
Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water-oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral or near neutral conditions are more environmentally friendly with less corrosion issues. This review starts with a brief introduction of OER, the importance of OER in mild-pH media, as well as the fundamentals and performance parameters of OER electrocatalysts. Then, recent progress of the rational design of electrocatalysts for OER in mild-pH conditions is discussed. The chemical structures or components, synthetic approaches, and catalytic performances of the OER catalysts will be reviewed. Some interesting insights into the catalytic mechanism are also included and discussed. It concludes with a brief outlook on the possible remaining challenges and future trends of neutral or near-neutral OER electrocatalysts. It hopefully provides the readers with a distinct perspective of the history, present, and future of OER electrocatalysts at mild conditions.
Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting. Compared with the water‐oxidation electrocatalysts that are commonly utilized in alkaline conditions, the ones operating efficiently under neutral or near neutral conditions are more environmentally friendly with less corrosion issues. This review starts with a brief introduction of OER, the importance of OER in mild‐pH media, as well as the fundamentals and performance parameters of OER electrocatalysts. Then, recent progress of the rational design of electrocatalysts for OER in mild‐pH conditions is discussed. The chemical structures or components, synthetic approaches, and catalytic performances of the OER catalysts will be reviewed. Some interesting insights into the catalytic mechanism are also included and discussed. It concludes with a brief outlook on the possible remaining challenges and future trends of neutral or near‐neutral OER electrocatalysts. It hopefully provides the readers with a distinct perspective of the history, present, and future of OER electrocatalysts at mild conditions. Electrocatalytic water oxidation under environmentally‐friendly conditions has received considerable recent research attention. This paper reviews recent advances in the design and development of water oxidation electrocatalysts operating at mild pH, and current challenges and future research directions are also provided.
Author Zhang, Youyu
Liu, Qian
Sun, Xuping
Wang, Huanbo
Shi, Xifeng
Zhao, Runbo
Wei, Peipei
Li, Tingshuai
Liu, Meiling
Chen, Hongyu
Li, Peipei
Huang, Hong
Author_xml – sequence: 1
  givenname: Peipei
  surname: Li
  fullname: Li, Peipei
  organization: Hunan Normal University
– sequence: 2
  givenname: Runbo
  surname: Zhao
  fullname: Zhao, Runbo
  organization: University of Electronic Science and Technology of China
– sequence: 3
  givenname: Hongyu
  surname: Chen
  fullname: Chen, Hongyu
  organization: University of Electronic Science and Technology of China
– sequence: 4
  givenname: Huanbo
  surname: Wang
  fullname: Wang, Huanbo
  organization: Southwest University of Science and Technology
– sequence: 5
  givenname: Peipei
  surname: Wei
  fullname: Wei, Peipei
  organization: University of Electronic Science and Technology of China
– sequence: 6
  givenname: Hong
  surname: Huang
  fullname: Huang, Hong
  organization: University of Electronic Science and Technology of China
– sequence: 7
  givenname: Qian
  surname: Liu
  fullname: Liu, Qian
  organization: University of Electronic Science and Technology of China
– sequence: 8
  givenname: Tingshuai
  surname: Li
  fullname: Li, Tingshuai
  organization: University of Electronic Science and Technology of China
– sequence: 9
  givenname: Xifeng
  surname: Shi
  fullname: Shi, Xifeng
  organization: Chemical Engineering and Materials Science
– sequence: 10
  givenname: Youyu
  surname: Zhang
  fullname: Zhang, Youyu
  organization: Hunan Normal University
– sequence: 11
  givenname: Meiling
  surname: Liu
  fullname: Liu, Meiling
  email: liuml@hunnu.edu.cn
  organization: Hunan Normal University
– sequence: 12
  givenname: Xuping
  orcidid: 0000-0002-5326-3838
  surname: Sun
  fullname: Sun, Xuping
  email: xpsun@uestc.edu.cn
  organization: University of Electronic Science and Technology of China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/30773809$$D View this record in MEDLINE/PubMed
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Snippet Developing anodic oxygen evolution reaction (OER) electrocatalysts with high catalytic activities is of great importance for effective water splitting....
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SubjectTerms Anodizing
Catalysis
earth‐abundant metals
Electrocatalysts
mild pH
Nanotechnology
Organic chemistry
Oxidation
oxygen evolution reaction (OER)
Oxygen evolution reactions
water oxidation
Water splitting
Title Recent Advances in the Development of Water Oxidation Electrocatalysts at Mild pH
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fsmll.201805103
https://www.ncbi.nlm.nih.gov/pubmed/30773809
https://www.proquest.com/docview/2197269342
https://www.proquest.com/docview/2183191018
Volume 15
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