Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte
The performance of Li‐ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non‐pola...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 8; pp. 4090 - 4097 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
19.02.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The performance of Li‐ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non‐polar solvent, which leads to a peculiar solvation structure where ion pairs and aggregates prevail under a low salt concentration of 1.0 M. Importantly, WSE forms unique anion‐derived interphases on graphite electrodes that exhibit fast‐charging and long‐term cycling characteristics. First‐principles calculations unravel a general principle that the competitive coordination between anions and solvents to Li ions is the origin of different interfacial chemistries. By bridging the gap between solution thermodynamics and interfacial chemistry in batteries, this work opens a brand‐new way towards precise electrolyte engineering for energy storage devices with desired properties.
A weakly solvating electrolyte affords a new path towards anion‐derived interfacial chemistry in lithium‐ion batteries. By formulating electrolyte with a non‐polar solvent, ion pairs and aggregates prevail under normal concentrations and give rise to anion‐derived interphases on graphite electrodes with superior electrochemical performances. |
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| AbstractList | The performance of Li-ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non-polar solvent, which leads to a peculiar solvation structure where ion pairs and aggregates prevail under a low salt concentration of 1.0 M. Importantly, WSE forms unique anion-derived interphases on graphite electrodes that exhibit fast-charging and long-term cycling characteristics. First-principles calculations unravel a general principle that the competitive coordination between anions and solvents to Li ions is the origin of different interfacial chemistries. By bridging the gap between solution thermodynamics and interfacial chemistry in batteries, this work opens a brand-new way towards precise electrolyte engineering for energy storage devices with desired properties.The performance of Li-ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non-polar solvent, which leads to a peculiar solvation structure where ion pairs and aggregates prevail under a low salt concentration of 1.0 M. Importantly, WSE forms unique anion-derived interphases on graphite electrodes that exhibit fast-charging and long-term cycling characteristics. First-principles calculations unravel a general principle that the competitive coordination between anions and solvents to Li ions is the origin of different interfacial chemistries. By bridging the gap between solution thermodynamics and interfacial chemistry in batteries, this work opens a brand-new way towards precise electrolyte engineering for energy storage devices with desired properties. The performance of Li-ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non-polar solvent, which leads to a peculiar solvation structure where ion pairs and aggregates prevail under a low salt concentration of 1.0 M. Importantly, WSE forms unique anion-derived interphases on graphite electrodes that exhibit fast-charging and long-term cycling characteristics. First-principles calculations unravel a general principle that the competitive coordination between anions and solvents to Li ions is the origin of different interfacial chemistries. By bridging the gap between solution thermodynamics and interfacial chemistry in batteries, this work opens a brand-new way towards precise electrolyte engineering for energy storage devices with desired properties. The performance of Li‐ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte typically contains polar solvents to dissociate Li salts. Herein we report a weakly solvating electrolyte (WSE) that consists of a pure non‐polar solvent, which leads to a peculiar solvation structure where ion pairs and aggregates prevail under a low salt concentration of 1.0 M. Importantly, WSE forms unique anion‐derived interphases on graphite electrodes that exhibit fast‐charging and long‐term cycling characteristics. First‐principles calculations unravel a general principle that the competitive coordination between anions and solvents to Li ions is the origin of different interfacial chemistries. By bridging the gap between solution thermodynamics and interfacial chemistry in batteries, this work opens a brand‐new way towards precise electrolyte engineering for energy storage devices with desired properties. A weakly solvating electrolyte affords a new path towards anion‐derived interfacial chemistry in lithium‐ion batteries. By formulating electrolyte with a non‐polar solvent, ion pairs and aggregates prevail under normal concentrations and give rise to anion‐derived interphases on graphite electrodes with superior electrochemical performances. |
| Author | Cai, Wen‐Long Huang, Jia‐Qi Yao, Yu‐Xing Zhang, Qiang Zhang, Xue‐Qiang Chen, Xiang Yan, Chong |
| Author_xml | – sequence: 1 givenname: Yu‐Xing surname: Yao fullname: Yao, Yu‐Xing organization: Tsinghua University – sequence: 2 givenname: Xiang surname: Chen fullname: Chen, Xiang organization: Tsinghua University – sequence: 3 givenname: Chong surname: Yan fullname: Yan, Chong organization: Beijing Institute of Technology – sequence: 4 givenname: Xue‐Qiang surname: Zhang fullname: Zhang, Xue‐Qiang organization: Tsinghua University – sequence: 5 givenname: Wen‐Long surname: Cai fullname: Cai, Wen‐Long organization: Tsinghua University – sequence: 6 givenname: Jia‐Qi surname: Huang fullname: Huang, Jia‐Qi organization: Beijing Institute of Technology – sequence: 7 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32976693$$D View this record in MEDLINE/PubMed |
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| Snippet | The performance of Li‐ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte... The performance of Li-ion batteries (LIBs) is highly dependent on their interfacial chemistry, which is regulated by electrolytes. Conventional electrolyte... |
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| SubjectTerms | Anions batteries Chemistry Electrolytes Energy storage graphite interfacial chemistry Ion pairs Ions Lithium Lithium-ion batteries Salts Solvation Solvents |
| Title | Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte |
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