Three-Dimensional Hierarchical Porous Structure of PPy/Porous-Graphene to Encapsulate Polysulfides for Lithium/Sulfur Batteries
Herein, we demonstrate the fabrication of a three-dimensional (3D) polypyrrole-coated-porous graphene (PPy/PG) composite through in-situ polymerization of pyrrole monomer on PG surface. The PPy/PG displays a 3D hierarchical porous structure and the resulting PPy/PG hybrid serves as a conductive trap...
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Published in | Nanomaterials (Basel, Switzerland) Vol. 8; no. 8; p. 606 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
Published |
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09.08.2018
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Abstract | Herein, we demonstrate the fabrication of a three-dimensional (3D) polypyrrole-coated-porous graphene (PPy/PG) composite through in-situ polymerization of pyrrole monomer on PG surface. The PPy/PG displays a 3D hierarchical porous structure and the resulting PPy/PG hybrid serves as a conductive trap to lithium polysulfides enhancing the electrochemical performances. Owing to the superior conductivity and peculiar structure, a high initial discharge capacity of 1020 mAh g
and the reversible capacity of 802 mAh g
over 200 cycles are obtained for the S/PPy/PG cathode at 0.1 C, remaining the remarkable cyclic stability. In addition, the S/PPy/PG cathodes demonstrate an excellent rate performance exhibiting 477 mAh g
at 2 C. |
---|---|
AbstractList | Herein, we demonstrate the fabrication of a three-dimensional (3D) polypyrrole-coated-porous graphene (PPy/PG) composite through in-situ polymerization of pyrrole monomer on PG surface. The PPy/PG displays a 3D hierarchical porous structure and the resulting PPy/PG hybrid serves as a conductive trap to lithium polysulfides enhancing the electrochemical performances. Owing to the superior conductivity and peculiar structure, a high initial discharge capacity of 1020 mAh g
−1
and the reversible capacity of 802 mAh g
−1
over 200 cycles are obtained for the S/PPy/PG cathode at 0.1 C, remaining the remarkable cyclic stability. In addition, the S/PPy/PG cathodes demonstrate an excellent rate performance exhibiting 477 mAh g
−1
at 2 C. Herein, we demonstrate the fabrication of a three-dimensional (3D) polypyrrole-coated-porous graphene (PPy/PG) composite through in-situ polymerization of pyrrole monomer on PG surface. The PPy/PG displays a 3D hierarchical porous structure and the resulting PPy/PG hybrid serves as a conductive trap to lithium polysulfides enhancing the electrochemical performances. Owing to the superior conductivity and peculiar structure, a high initial discharge capacity of 1020 mAh g and the reversible capacity of 802 mAh g over 200 cycles are obtained for the S/PPy/PG cathode at 0.1 C, remaining the remarkable cyclic stability. In addition, the S/PPy/PG cathodes demonstrate an excellent rate performance exhibiting 477 mAh g at 2 C. Herein, we demonstrate the fabrication of a three-dimensional (3D) polypyrrole-coated-porous graphene (PPy/PG) composite through in-situ polymerization of pyrrole monomer on PG surface. The PPy/PG displays a 3D hierarchical porous structure and the resulting PPy/PG hybrid serves as a conductive trap to lithium polysulfides enhancing the electrochemical performances. Owing to the superior conductivity and peculiar structure, a high initial discharge capacity of 1020 mAh g−1 and the reversible capacity of 802 mAh g−1 over 200 cycles are obtained for the S/PPy/PG cathode at 0.1 C, remaining the remarkable cyclic stability. In addition, the S/PPy/PG cathodes demonstrate an excellent rate performance exhibiting 477 mAh g−1 at 2 C. |
Author | Tan, Taizhe Bakenov, Zhumabay Huang, Jin Zhang, Yongguang |
AuthorAffiliation | 1 School of Materials and Energy, Synergy Innovation Institute of GDUT (Heyuan), Guangdong University of Technology, Guangzhou 510006, China; ygzhang126@126.com 2 Institute of Batteries LLC, National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan; zbakenov@nu.edu.kz |
AuthorAffiliation_xml | – name: 1 School of Materials and Energy, Synergy Innovation Institute of GDUT (Heyuan), Guangdong University of Technology, Guangzhou 510006, China; ygzhang126@126.com – name: 2 Institute of Batteries LLC, National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan; zbakenov@nu.edu.kz |
Author_xml | – sequence: 1 givenname: Yongguang surname: Zhang fullname: Zhang, Yongguang email: ygzhang126@126.com organization: School of Materials and Energy, Synergy Innovation Institute of GDUT (Heyuan), Guangdong University of Technology, Guangzhou 510006, China. ygzhang126@126.com – sequence: 2 givenname: Zhumabay orcidid: 0000-0003-2781-4955 surname: Bakenov fullname: Bakenov, Zhumabay email: zbakenov@nu.edu.kz organization: Institute of Batteries LLC, National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. zbakenov@nu.edu.kz – sequence: 3 givenname: Taizhe surname: Tan fullname: Tan, Taizhe email: tztansii18@163.com organization: School of Materials and Energy, Synergy Innovation Institute of GDUT (Heyuan), Guangdong University of Technology, Guangzhou 510006, China. tztansii18@163.com – sequence: 4 givenname: Jin surname: Huang fullname: Huang, Jin email: huangjiner@126.com organization: School of Materials and Energy, Synergy Innovation Institute of GDUT (Heyuan), Guangdong University of Technology, Guangzhou 510006, China. huangjiner@126.com |
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CitedBy_id | crossref_primary_10_1016_j_jelechem_2019_04_027 crossref_primary_10_3390_nano10050840 crossref_primary_10_1039_D2SE00254J crossref_primary_10_1002_smll_201903780 crossref_primary_10_1021_acsaem_1c02054 crossref_primary_10_1016_j_ceramint_2020_04_145 crossref_primary_10_1002_adfm_202100457 crossref_primary_10_3390_nano10040745 crossref_primary_10_3390_nano11040827 crossref_primary_10_1039_C9CP01036J crossref_primary_10_1016_j_electacta_2023_143539 crossref_primary_10_1016_j_mtcomm_2022_103211 crossref_primary_10_1149_1945_7111_ab6bc0 crossref_primary_10_1021_acsaem_9b00352 crossref_primary_10_1039_C9RA04205A |
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Keywords | sulfur/polypyrrole/porous graphene composite hierarchical 3D porous structure lithium/sulfur battery |
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SubjectTerms | Batteries Carbon Cathodes Electrochemistry Electrodes Energy Fabrication Fourier transforms Graphene hierarchical 3D porous structure Lithium Lithium sulfur batteries lithium/sulfur battery Microscopy Nanocomposites Polymerization Polypyrroles Polysulfides Spectrum analysis Structural hierarchy Sulfur sulfur/polypyrrole/porous graphene composite |
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Title | Three-Dimensional Hierarchical Porous Structure of PPy/Porous-Graphene to Encapsulate Polysulfides for Lithium/Sulfur Batteries |
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