Styrene Epoxidation over Carbon Nanotube-Supported Gold Catalysts

Carbon nanotube supported gold catalysts prepared by deposition-precipitation with urea (DP urea) were characterized by various techniques. Its catalytic activity was examined for the oxidation of styrene using t-butylhydroperoxide as oxidant. This system showed good epoxide selectivity. The other f...

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Published in	Catalysis letters Vol. 134; no. 1-2; pp. 51 - 55
Main Authors	Liu, Junhua, Wang, Fang, Xu, Tan, Gu, Zhenggui
Format	Journal Article
Language	English
Published	Boston Boston : Springer US 2010 Springer US Springer Springer Nature B.V
Subjects	Carbon nanotubes Catalysis Catalysts Catalytic activity Chemistry Chemistry and Materials Science Epoxidation Ethylene oxide Exact sciences and technology General and physical chemistry Gold Industrial Chemistry/Chemical Engineering Nanotubes Olefins Organometallic Chemistry Oxidation Physical Chemistry Rain and rainfall Reaction time Selectivity Styrenes Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Urea Carbon nanotubes (CNTs) Epoxidation Gold Styrene Catalytic reaction Hydrocarbon Organic hydroperoxide Reuse Carbon nanotubes Transition metal Selectivity Oxidant Supported catalyst Heterogeneous catalysis Urea Precipitation Epoxide Reaction time Benzenic compound Ureas Oxidation Deposition
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Abstract	Carbon nanotube supported gold catalysts prepared by deposition-precipitation with urea (DP urea) were characterized by various techniques. Its catalytic activity was examined for the oxidation of styrene using t-butylhydroperoxide as oxidant. This system showed good epoxide selectivity. The other factors, such as solvent, reaction time, concentrations of oxidant and catalyst, have also been investigated and reaction conditions are optimized. It is a novel highly active/selective and reusable heterogeneous catalyst for styrene epoxidation.
AbstractList	Carbon nanotube supported gold catalysts prepared by deposition-precipitation with urea (DP urea) were characterized by various techniques. Its catalytic activity was examined for the oxidation of styrene using t-butylhydroperoxide as oxidant. This system showed good epoxide selectivity. The other factors, such as solvent, reaction time, concentrations of oxidant and catalyst, have also been investigated and reaction conditions are optimized. It is a novel highly active/selective and reusable heterogeneous catalyst for styrene epoxidation. Carbon nanotube supported gold catalysts prepared by deposition-precipitation with urea (DP urea) were characterized by various techniques. Its catalytic activity was examined for the oxidation of styrene using t-butylhydroperoxide as oxidant. This system showed good epoxide selectivity. The other factors, such as solvent, reaction time, concentrations of oxidant and catalyst, have also been investigated and reaction conditions are optimized. It is a novel highly active/selective and reusable heterogeneous catalyst for styrene epoxidation. Keywords Carbon nanotubes (CNTs) * Epoxidation * Gold * Styrene Carbon nanotube supported gold catalysts prepared by deposition–precipitation with urea (DP urea) were characterized by various techniques. Its catalytic activity was examined for the oxidation of styrene using t -butylhydroperoxide as oxidant. This system showed good epoxide selectivity. The other factors, such as solvent, reaction time, concentrations of oxidant and catalyst, have also been investigated and reaction conditions are optimized. It is a novel highly active/selective and reusable heterogeneous catalyst for styrene epoxidation.
Audience	Academic
Author	Wang, Fang Liu, Junhua Gu, Zhenggui Xu, Tan
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Keywords	Carbon nanotubes (CNTs) Epoxidation Gold Styrene Catalytic reaction Hydrocarbon Organic hydroperoxide Reuse Carbon nanotubes Transition metal Selectivity Oxidant Supported catalyst Heterogeneous catalysis Urea Precipitation Epoxide Reaction time Benzenic compound Ureas Oxidation Deposition
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Snippet	Carbon nanotube supported gold catalysts prepared by deposition-precipitation with urea (DP urea) were characterized by various techniques. Its catalytic... Carbon nanotube supported gold catalysts prepared by deposition–precipitation with urea (DP urea) were characterized by various techniques. Its catalytic...
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SubjectTerms	Carbon nanotubes Catalysis Catalysts Catalytic activity Chemistry Chemistry and Materials Science Epoxidation Ethylene oxide Exact sciences and technology General and physical chemistry Gold Industrial Chemistry/Chemical Engineering Nanotubes Olefins Organometallic Chemistry Oxidation Physical Chemistry Rain and rainfall Reaction time Selectivity Styrenes Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Urea
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Title	Styrene Epoxidation over Carbon Nanotube-Supported Gold Catalysts
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