Sub-lattice of Jahn-Teller centers in hexaferrite crystal

A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe 3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground stat...

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Published inScientific reports Vol. 10; no. 1; p. 7076
Main Authors Gudkov, V. V., Sarychev, M. N., Zherlitsyn, S., Zhevstovskikh, I. V., Averkiev, N. S., Vinnik, D. A., Gudkova, S. A., Niewa, R., Dressel, M., Alyabyeva, L. N., Gorshunov, B. P., Bersuker, I. B.
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 27.04.2020
Nature Publishing Group
Subjects
639/766/119/996
639/766/25/3927
639/766/400/561
Adiabatic
Approximation
Barium
Chemical elements
Chemistry
Humanities and Social Sciences
Ions
Iron
Magnetic fields
multidisciplinary
Phase transitions
Physics
Potential energy
Quantum theory
Science
Science (multidisciplinary)
Symmetry
Ultrasound
Online AccessGet full text
ISSN2045-2322
2045-2322
DOI10.1038/s41598-020-63915-7

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Abstract A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe 3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe 2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the E ⊗ e problem of the JT effect. The arranged JT complexes, Fe 2+ O 4 , their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
AbstractList A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe12O19. In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the E⊗e problem of the JT effect. The arranged JT complexes, Fe2+O4, their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe12O19. In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the [Formula: see text] problem of the JT effect. The arranged JT complexes, Fe2+O4, their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe12O19. In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the [Formula: see text] problem of the JT effect. The arranged JT complexes, Fe2+O4, their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe O . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the [Formula: see text] problem of the JT effect. The arranged JT complexes, Fe O , their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe 3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe 2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the E ⊗ e problem of the JT effect. The arranged JT complexes, Fe 2+ O 4 , their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe 3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe 2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$E\otimes e$$\end{document} E ⊗ e problem of the JT effect. The arranged JT complexes, Fe 2+ O 4 , their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions, sitting in five different crystallographic positions, are Fe 3+ in the high-spin configuration (S = 5/2) and have a non-degenerate ground state. We show that the electron-donor Ti substitution converts the ions to Fe 2+ predominantly in tetrahedral coordination, resulting in doubly-degenerate states subject to the $$E\otimes e$$ E ⊗ e problem of the JT effect. The arranged JT complexes, Fe 2+ O 4 , their adiabatic potential energy, non-linear and quantum dynamics, have been studied by means of ultrasound and terahertz-infrared spectroscopies. The JT complexes are sensitive to external stress and applied magnetic field. For that reason, the properties of the doped crystal can be controlled by the amount and state of the JT complexes.
ArticleNumber 7076
Author Gudkova, S. A.
Zhevstovskikh, I. V.
Bersuker, I. B.
Niewa, R.
Alyabyeva, L. N.
Gudkov, V. V.
Dressel, M.
Averkiev, N. S.
Zherlitsyn, S.
Gorshunov, B. P.
Sarychev, M. N.
Vinnik, D. A.
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Snippet A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe 12 O 19 . In the un-doped crystal all iron ions,...
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe O . In the un-doped crystal all iron ions, sitting...
A novel type of sub-lattice of the Jahn-Teller (JT) centers was arranged in Ti-doped barium hexaferrite BaFe12O19. In the un-doped crystal all iron ions,...
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SubjectTerms 639/766/119/996
639/766/25/3927
639/766/400/561
Adiabatic
Approximation
Barium
Chemical elements
Chemistry
Humanities and Social Sciences
Ions
Iron
Magnetic fields
multidisciplinary
Phase transitions
Physics
Potential energy
Quantum theory
Science
Science (multidisciplinary)
Symmetry
Ultrasound
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Title Sub-lattice of Jahn-Teller centers in hexaferrite crystal
URI https://link.springer.com/article/10.1038/s41598-020-63915-7
https://www.ncbi.nlm.nih.gov/pubmed/32341430
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Volume 10
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