Reconstruction of time changes in radiocesium concentrations in the river of the Fukushima Dai-ichi NPP contaminated area based on its depth distribution in dam reservoir's bottom sediments
Radionuclide depth distribution in bottom sediments in deep-water zones of dam reservoirs, where no sediment mixing occurs, can be used to reconstruct time changes in particulate activity concentrations of radionuclides strongly bound to bottom sediments. This approach was used to analyze the 137Cs...
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Published in | Environmental research Vol. 206; p. 112307 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Abstract | Radionuclide depth distribution in bottom sediments in deep-water zones of dam reservoirs, where no sediment mixing occurs, can be used to reconstruct time changes in particulate activity concentrations of radionuclides strongly bound to bottom sediments. This approach was used to analyze the 137Cs concentration profile in a bottom sediment core collected from Ogaki dam reservoir on the Ukedo River in the Fukushima Dai-ichi nuclear power plant contaminated zone in October 2019. The derived 137Cs particulate concentrations provided a basis for estimating the dissolved concentration and its temporal trend in the Ukedo River, using the mean value of the apparent 137Cs distribution coefficient. The reconstructed particulate and dissolved 137Cs concentrations and their temporal trends are consistent with monitoring data. The annual mean particulate and dissolved 137Cs wash-off ratios were also calculated for the period of eight years after the accident. Interestingly, the particulate 137Cs wash-off ratios for the Ukedo River at Ogaki dam were found to be similar to those for the Pripyat River at Chernobyl in the same time period after the accident, while the dissolved 137Cs wash-off ratios in the Ukedo River were an order of magnitude lower than the corresponding values in the Pripyat River. Both the particulate and dissolved 137Cs wash-off ratios in the Ukedo River declined faster during the first eight years after the FDNPP accident than predicted by the diffusional model, most likely, due to greater natural attenuation and, to some extent, remediation measures implemented on the catchments in Fukushima.
•137Cs depth profile in bottom sediments can be taken as representing radionuclide dynamics in river.•Reconstructed 137Cs concentrations in Ukedo River are consistent with monitoring data.•137Cs wash-off ratios in Fukushima tend to decrease faster than in Chernobyl. |
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AbstractList | Radionuclide depth distribution in bottom sediments in deep-water zones of dam reservoirs, where no sediment mixing occurs, can be used to reconstruct time changes in particulate activity concentrations of radionuclides strongly bound to bottom sediments. This approach was used to analyze the 137Cs concentration profile in a bottom sediment core collected from Ogaki dam reservoir on the Ukedo River in the Fukushima Dai-ichi nuclear power plant contaminated zone in October 2019. The derived 137Cs particulate concentrations provided a basis for estimating the dissolved concentration and its temporal trend in the Ukedo River, using the mean value of the apparent 137Cs distribution coefficient. The reconstructed particulate and dissolved 137Cs concentrations and their temporal trends are consistent with monitoring data. The annual mean particulate and dissolved 137Cs wash-off ratios were also calculated for the period of eight years after the accident. Interestingly, the particulate 137Cs wash-off ratios for the Ukedo River at Ogaki dam were found to be similar to those for the Pripyat River at Chernobyl in the same time period after the accident, while the dissolved 137Cs wash-off ratios in the Ukedo River were an order of magnitude lower than the corresponding values in the Pripyat River. Both the particulate and dissolved 137Cs wash-off ratios in the Ukedo River declined faster during the first eight years after the FDNPP accident than predicted by the diffusional model, most likely, due to greater natural attenuation and, to some extent, remediation measures implemented on the catchments in Fukushima.
•137Cs depth profile in bottom sediments can be taken as representing radionuclide dynamics in river.•Reconstructed 137Cs concentrations in Ukedo River are consistent with monitoring data.•137Cs wash-off ratios in Fukushima tend to decrease faster than in Chernobyl. Radionuclide depth distribution in bottom sediments in deep-water zones of dam reservoirs, where no sediment mixing occurs, can be used to reconstruct time changes in particulate activity concentrations of radionuclides strongly bound to bottom sediments. This approach was used to analyze the Cs concentration profile in a bottom sediment core collected from Ogaki dam reservoir on the Ukedo River in the Fukushima Dai-ichi nuclear power plant contaminated zone in October 2019. The derived Cs particulate concentrations provided a basis for estimating the dissolved concentration and its temporal trend in the Ukedo River, using the mean value of the apparent Cs distribution coefficient. The reconstructed particulate and dissolved Cs concentrations and their temporal trends are consistent with monitoring data. The annual mean particulate and dissolved Cs wash-off ratios were also calculated for the period of eight years after the accident. Interestingly, the particulate Cs wash-off ratios for the Ukedo River at Ogaki dam were found to be similar to those for the Pripyat River at Chernobyl in the same time period after the accident, while the dissolved Cs wash-off ratios in the Ukedo River were an order of magnitude lower than the corresponding values in the Pripyat River. Both the particulate and dissolved Cs wash-off ratios in the Ukedo River declined faster during the first eight years after the FDNPP accident than predicted by the diffusional model, most likely, due to greater natural attenuation and, to some extent, remediation measures implemented on the catchments in Fukushima. |
ArticleNumber | 112307 |
Author | Wakiyama, Yoshifumi Konoplev, Alexei Komissarov, Mikhail Wada, Toshihiro Nanba, Kenji Ivanov, Maxim |
Author_xml | – sequence: 1 givenname: Alexei orcidid: 0000-0002-9930-8739 surname: Konoplev fullname: Konoplev, Alexei email: r701@ipc.fukushima-u.ac.jp organization: Institute of Environmental Radioactivity, Fukushima University, Kanayagawa 1, Fukushima, 960-1296, Japan – sequence: 2 givenname: Yoshifumi orcidid: 0000-0001-6085-7063 surname: Wakiyama fullname: Wakiyama, Yoshifumi organization: Institute of Environmental Radioactivity, Fukushima University, Kanayagawa 1, Fukushima, 960-1296, Japan – sequence: 3 givenname: Toshihiro surname: Wada fullname: Wada, Toshihiro organization: Institute of Environmental Radioactivity, Fukushima University, Kanayagawa 1, Fukushima, 960-1296, Japan – sequence: 4 givenname: Maxim surname: Ivanov fullname: Ivanov, Maxim organization: Faculty of Geography, Moscow State University, Moscow, 119991, Russia – sequence: 5 givenname: Mikhail orcidid: 0000-0001-6135-7212 surname: Komissarov fullname: Komissarov, Mikhail organization: Ufa Institute of Biology UFRS RAS, Ufa, 450054, Russia – sequence: 6 givenname: Kenji surname: Nanba fullname: Nanba, Kenji organization: Institute of Environmental Radioactivity, Fukushima University, Kanayagawa 1, Fukushima, 960-1296, Japan |
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Keywords | Dam reservoir Particulate MEXT Dissolved IAEA HPGe Fukushima River FDNPP Radiocesium NPP |
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SubjectTerms | Cesium Radioisotopes Dam reservoir Dissolved Fukushima Fukushima Nuclear Accident Japan Nuclear Power Plants Particulate Radiation Monitoring Radiocesium River Rivers Water Pollutants, Radioactive - analysis |
Title | Reconstruction of time changes in radiocesium concentrations in the river of the Fukushima Dai-ichi NPP contaminated area based on its depth distribution in dam reservoir's bottom sediments |
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