Novel L-DOPA-Derived Poly(ester amide)s: Monomers, Polymers, and the First L-DOPA-Functionalized Biobased Adhesive Tape
The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optim...
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| Published in | Macromolecular rapid communications. Vol. 35; no. 1; pp. 71 - 76 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Blackwell Publishing Ltd
01.01.2014
Wiley Wiley Subscription Services, Inc |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials.
A family of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L‐DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results. |
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| AbstractList | The synthesis, characterization, and testing of a range of novel bio‐inspired
L
‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased
L
‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials.
image The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L-DOPA-containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)-based materials. A family of novel bio-inspired L-DOPA-derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L-DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results. The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials. A family of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L‐DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results. The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L-DOPA-containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)-based materials.The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L-DOPA-containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)-based materials. The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L-DOPA-containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)-based materials. [PUBLICATION ABSTRACT] The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L-DOPA-containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)-based materials. |
| Author | Vendamme, Richard Eevers, Walter Manolakis, Ioannis Noordover, Bart A. J. |
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| Keywords | Nitro compound bio-inspired polymers Adhesivity Solution polycondensation Polyesteramide Head to tail polymer Adhesive tape Esteramide copolymer Experimental study Functional polymer adhesive properties polycondensation poly(ester amide)s Biomimetic compound Preparation L-DOPA Surface properties Unsaturated copolymer Phenols Levodopa |
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| Snippet | The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable,... The synthesis, characterization, and testing of a range of novel bio‐inspired L ‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable,... The synthesis, characterization, and testing of a range of novel bio-inspired L-DOPA-derived poly(ester amide)s is presented, using a widely applicable,... |
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| SubjectTerms | adhesive properties Adhesives Amides - chemistry Applied sciences bio-inspired polymers Exact sciences and technology L-DOPA Levodopa - chemistry Magnetic Resonance Spectroscopy Organic polymers Physicochemistry of polymers poly(ester amide)s polycondensation Polyesters - chemistry Polymers Polymers with particular properties Preparation, kinetics, thermodynamics, mechanism and catalysts Tissue Adhesives |
| Title | Novel L-DOPA-Derived Poly(ester amide)s: Monomers, Polymers, and the First L-DOPA-Functionalized Biobased Adhesive Tape |
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