Thermodynamics and kinetics of hydriding and dehydriding reactions in Mg-based hydrogen storage materials
Mg-based materials are one of the most promising hydrogen storage candidates due to their high hydrogen storage capacity, environmental benignity, and high Clarke number characteristics. However, the limited thermodynamics and kinetic properties pose major challenges for their engineering applicatio...
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| Published in | Journal of magnesium and alloys Vol. 9; no. 6; pp. 1922 - 1941 |
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| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.11.2021
KeAi Communications Co., Ltd |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Mg-based materials are one of the most promising hydrogen storage candidates due to their high hydrogen storage capacity, environmental benignity, and high Clarke number characteristics. However, the limited thermodynamics and kinetic properties pose major challenges for their engineering applications. Herein, we review the recent progress in improving their thermodynamics and kinetics, with an emphasis on the models and the influence of various parameters in the calculated models. Subsequently, the impact of alloying, composite, and nano-crystallization on both thermodynamics and dynamics are discussed in detail. In particular, the correlation between various modification strategies and the hydrogen capacity, dehydrogenation enthalpy and temperature, hydriding/dehydriding rates are summarized. In addition, the mechanism of hydrogen storage processes of Mg-based materials is discussed from the aspect of classical kinetic theories and microscope hydrogen transferring behavior. This review concludes with an outlook on the remaining challenge issues and prospects. |
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| AbstractList | Mg-based materials are one of the most promising hydrogen storage candidates due to their high hydrogen storage capacity, environmental benignity, and high Clarke number characteristics. However, the limited thermodynamics and kinetic properties pose major challenges for their engineering applications. Herein, we review the recent progress in improving their thermodynamics and kinetics, with an emphasis on the models and the influence of various parameters in the calculated models. Subsequently, the impact of alloying, composite, and nano-crystallization on both thermodynamics and dynamics are discussed in detail. In particular, the correlation between various modification strategies and the hydrogen capacity, dehydrogenation enthalpy and temperature, hydriding/dehydriding rates are summarized. In addition, the mechanism of hydrogen storage processes of Mg-based materials is discussed from the aspect of classical kinetic theories and microscope hydrogen transferring behavior. This review concludes with an outlook on the remaining challenge issues and prospects. |
| Author | Tan, Jun Chen, Yuan Luo, Qun Pan, Fusheng Li, Qian Sun, Shuhui Jiang, Bin Yang, Xiaohua Dang, Jie Lu, Yangfan Yang, Yan Dong, Zhihua Li, Jianbo |
| Author_xml | – sequence: 1 givenname: Qian surname: Li fullname: Li, Qian email: cquliqian@cqu.edu.cn organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 2 givenname: Yangfan surname: Lu fullname: Lu, Yangfan organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 3 givenname: Qun surname: Luo fullname: Luo, Qun organization: State Key Laboratory of Advanced Special Steels, Shanghai Key Laboratory of Advanced Ferrometallurgy, School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China – sequence: 4 givenname: Xiaohua orcidid: 0000-0002-7126-667X surname: Yang fullname: Yang, Xiaohua organization: Institute of Quantum and Sustainable Technology (IQST), School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013, China – sequence: 5 givenname: Yan surname: Yang fullname: Yang, Yan organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 6 givenname: Jun orcidid: 0000-0003-0701-7449 surname: Tan fullname: Tan, Jun organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 7 givenname: Zhihua surname: Dong fullname: Dong, Zhihua organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 8 givenname: Jie surname: Dang fullname: Dang, Jie organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 9 givenname: Jianbo surname: Li fullname: Li, Jianbo organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 10 givenname: Yuan surname: Chen fullname: Chen, Yuan organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 11 givenname: Bin surname: Jiang fullname: Jiang, Bin organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 12 givenname: Shuhui surname: Sun fullname: Sun, Shuhui organization: Institut National de la Recherche Scientifique-Énergie Matériaux et Télécommunications, Varennes, J3×1S2, Québec, Canada – sequence: 13 givenname: Fusheng surname: Pan fullname: Pan, Fusheng email: fspan@cqu.edu.cn organization: National Engineering Research Center for Magnesium Alloys, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China |
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| Keywords | Thermodynamics Magnesium-based hydrogen storage materials Analysis methods Hydriding/dehydriding reactions Kinetic models |
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