Spin-reorientation-induced magnetodielectric coupling effects in two layered perovskite magnets

Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C 6 H 5 CH 2 CH 2 NH 3 ] 2 [MCl 4 ] (M = Mn 2+ and Cu 2+ ), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin...

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Published inChemical science (Cambridge) Vol. 9; no. 37; pp. 7413 - 7418
Main Authors Huang, Bo, Zhang, Jian-Yu, Huang, Rui-Kang, Chen, Ming-Kun, Xue, Wei, Zhang, Wei-Xiong, Zeng, Ming-Hua, Chen, Xiao-Ming
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 2018
Subjects
Antiferromagnetism
Chemistry
Copper
Coupling
Ferromagnetism
Hybrid systems
Hydrogen bonds
Magnetic properties
Magnets
Manganese
Perovskites
Single crystals
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Abstract Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C 6 H 5 CH 2 CH 2 NH 3 ] 2 [MCl 4 ] (M = Mn 2+ and Cu 2+ ), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn 2+ ) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the “soft” ferromagnet (M = Cu 2+ ) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic–inorganic hybrid systems to host magnetodielectric coupling effects.
AbstractList Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C6H5CH2CH2NH3]2[MCl4] (M = Mn2+ and Cu2+), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn2+) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the “soft” ferromagnet (M = Cu2+) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic–inorganic hybrid systems to host magnetodielectric coupling effects.
Spin-reorientation-induced magnetodielectric effects were discovered in two layered perovskite magnets, (C 6 H 5 CH 2 CH 2 NH 3 ) 2 [MCl 4 ] (M = Mn 2+ and Cu 2+ ), via highly reproducible isothermal magnetodielectric measurements on single-crystal samples. Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C 6 H 5 CH 2 CH 2 NH 3 ] 2 [MCl 4 ] (M = Mn 2+ and Cu 2+ ), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn 2+ ) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the “soft” ferromagnet (M = Cu 2+ ) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic–inorganic hybrid systems to host magnetodielectric coupling effects.
Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C6H5CH2CH2NH3]2[MCl4] (M = Mn2+ and Cu2+), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn2+) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the "soft" ferromagnet (M = Cu2+) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic-inorganic hybrid systems to host magnetodielectric coupling effects.Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C6H5CH2CH2NH3]2[MCl4] (M = Mn2+ and Cu2+), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn2+) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the "soft" ferromagnet (M = Cu2+) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic-inorganic hybrid systems to host magnetodielectric coupling effects.
Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C 6 H 5 CH 2 CH 2 NH 3 ] 2 [MCl 4 ] (M = Mn 2+ and Cu 2+ ), via isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn 2+ ) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the “soft” ferromagnet (M = Cu 2+ ) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic–inorganic hybrid systems to host magnetodielectric coupling effects.
Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C H CH CH NH ] [MCl ] (M = Mn and Cu ), isothermal magnetodielectric measurements on single-crystal samples. Specifically, peak-like dielectric anomalies and spin-flop transitions appeared simultaneously at around ±34 kOe for the canted antiferromagnet (M = Mn ) at below 44.3 K, while a low-field (1 kOe) controlled magnetodielectric effect was observed in the "soft" ferromagnet (M = Cu ) at below 9.5 K. These isothermal magnetodielectric effects are highly reproducible and synchronous with the field-induced magnetization at different temperatures, well confirming the essential role of spin reorientation on inducing magnetodielectric coupling effects. These findings strongly imply that the layered perovskite magnets are new promising organic-inorganic hybrid systems to host magnetodielectric coupling effects.
Author Chen, Xiao-Ming
Chen, Ming-Kun
Huang, Bo
Huang, Rui-Kang
Zhang, Wei-Xiong
Xue, Wei
Zeng, Ming-Hua
Zhang, Jian-Yu
AuthorAffiliation a MOE Key Laboratory of Bioinorganic and Synthetic Chemistry , School of Chemistry , Sun Yat-Sen University , Guangzhou , 510275 , P. R. China . Email: zhangwx6@mail.sysu.edu.cn
b School of Chemistry and Pharmaceutical Sciences , GuangXi Normal University , Guilin 541004 , P. R. China
AuthorAffiliation_xml – name: a MOE Key Laboratory of Bioinorganic and Synthetic Chemistry , School of Chemistry , Sun Yat-Sen University , Guangzhou , 510275 , P. R. China . Email: zhangwx6@mail.sysu.edu.cn
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  givenname: Xiao-Ming
  surname: Chen
  fullname: Chen, Xiao-Ming
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/30542545$$D View this record in MEDLINE/PubMed
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Snippet Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C 6 H 5 CH 2 CH 2 NH 3 ] 2 [MCl 4 ] (M = Mn...
Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C H CH CH NH ] [MCl ] (M = Mn and Cu ),...
Spin-reorientation-induced magnetodielectric coupling effects were discovered in two layered perovskite magnets, [C6H5CH2CH2NH3]2[MCl4] (M = Mn2+ and Cu2+),...
Spin-reorientation-induced magnetodielectric effects were discovered in two layered perovskite magnets, (C 6 H 5 CH 2 CH 2 NH 3 ) 2 [MCl 4 ] (M = Mn 2+ and Cu...
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StartPage 7413
SubjectTerms Antiferromagnetism
Chemistry
Copper
Coupling
Ferromagnetism
Hybrid systems
Hydrogen bonds
Magnetic properties
Magnets
Manganese
Perovskites
Single crystals
Title Spin-reorientation-induced magnetodielectric coupling effects in two layered perovskite magnets
URI https://www.ncbi.nlm.nih.gov/pubmed/30542545
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https://www.proquest.com/docview/2155917266
https://pubmed.ncbi.nlm.nih.gov/PMC6237123
Volume 9
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