Photoionization of clusters in intense few-cycle near infrared femtosecond pulses
In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as ∼10 fs which...
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| Published in | Physical chemistry chemical physics : PCCP Vol. 16; no. 19; pp. 8721 - 873 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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England
01.01.2014
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| Abstract | In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as ∼10 fs which approach the natural timescales of collective electronic motion in such nanoscale aggregates. In contrast to the dynamics occurring on few- and sub-picosecond timescales where ionic motion sets in and plays a key role marked by resonant plasmon oscillations, the few-cycle limit precludes cluster expansion due to the nuclear motion of ionic constituents. Thus, pulses lasting just a few optical cycles explore a new "impulsive" regime for the first time in cluster nanoplasmas wherein ions essentially remain "frozen". Along with the perspective on this new regime, we present first measurements of photoelectron distributions and temperatures.
In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. |
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| AbstractList | In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as ∼10 fs which approach the natural timescales of collective electronic motion in such nanoscale aggregates. In contrast to the dynamics occurring on few- and sub-picosecond timescales where ionic motion sets in and plays a key role marked by resonant plasmon oscillations, the few-cycle limit precludes cluster expansion due to the nuclear motion of ionic constituents. Thus, pulses lasting just a few optical cycles explore a new “impulsive” regime for the first time in cluster nanoplasmas wherein ions essentially remain “frozen”. Along with the perspective on this new regime, we present first measurements of photoelectron distributions and temperatures. In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as ~10 fs which approach the natural timescales of collective electronic motion in such nanoscale aggregates. In contrast to the dynamics occurring on few- and sub-picosecond timescales where ionic motion sets in and plays a key role marked by resonant plasmon oscillations, the few-cycle limit precludes cluster expansion due to the nuclear motion of ionic constituents. Thus, pulses lasting just a few optical cycles explore a new "impulsive" regime for the first time in cluster nanoplasmas wherein ions essentially remain "frozen". Along with the perspective on this new regime, we present first measurements of photoelectron distributions and temperatures. In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as similar to 10 fs which approach the natural timescales of collective electronic motion in such nanoscale aggregates. In contrast to the dynamics occurring on few- and sub-picosecond timescales where ionic motion sets in and plays a key role marked by resonant plasmon oscillations, the few-cycle limit precludes cluster expansion due to the nuclear motion of ionic constituents. Thus, pulses lasting just a few optical cycles explore a new "impulsive" regime for the first time in cluster nanoplasmas wherein ions essentially remain "frozen". Along with the perspective on this new regime, we present first measurements of photoelectron distributions and temperatures. In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. Recently, several studies have reported intriguing phenomena associated with the photoionization of clusters by pulses as short as ∼10 fs which approach the natural timescales of collective electronic motion in such nanoscale aggregates. In contrast to the dynamics occurring on few- and sub-picosecond timescales where ionic motion sets in and plays a key role marked by resonant plasmon oscillations, the few-cycle limit precludes cluster expansion due to the nuclear motion of ionic constituents. Thus, pulses lasting just a few optical cycles explore a new "impulsive" regime for the first time in cluster nanoplasmas wherein ions essentially remain "frozen". Along with the perspective on this new regime, we present first measurements of photoelectron distributions and temperatures. In this article we present a perspective on the current state of the art in the photoionization of atomic clusters in few-cycle near-infrared laser pulses. |
| Author | Krishnan, S. R Rajeev, R Sharma, V Gopal, R Moshammer, R Mudrich, M Krishnamurthy, M Jha, J |
| AuthorAffiliation | Physikalisches Institut, Universität Freiburg Tata Institute of Fundamental Research Max-Planck-Institut für Kernphysik Indian Institute of Technology - Hyderabad Tata Institute of Fundamental Research (Hyderabad) |
| AuthorAffiliation_xml | – name: Tata Institute of Fundamental Research (Hyderabad) – name: Max-Planck-Institut für Kernphysik – name: Tata Institute of Fundamental Research – name: Physikalisches Institut, Universität Freiburg – name: Indian Institute of Technology - Hyderabad |
| Author_xml | – sequence: 1 givenname: S. R surname: Krishnan fullname: Krishnan, S. R – sequence: 2 givenname: R surname: Gopal fullname: Gopal, R – sequence: 3 givenname: R surname: Rajeev fullname: Rajeev, R – sequence: 4 givenname: J surname: Jha fullname: Jha, J – sequence: 5 givenname: V surname: Sharma fullname: Sharma, V – sequence: 6 givenname: M surname: Mudrich fullname: Mudrich, M – sequence: 7 givenname: R surname: Moshammer fullname: Moshammer, R – sequence: 8 givenname: M surname: Krishnamurthy fullname: Krishnamurthy, M |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24695536$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Atomic clusters Clusters Constituents Electronics Nanostructure Oscillations Photoionization State of the art |
| Title | Photoionization of clusters in intense few-cycle near infrared femtosecond pulses |
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