Recent Advances in Graphitic Carbon Nitride Based Electro-Catalysts for CO2 Reduction Reactions

The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C3N4) has excellent chemical stability and unique structural properties that allow it to be widely used...

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Published inMolecules (Basel, Switzerland) Vol. 28; no. 8; p. 3292
Main Authors Mao, Xinyi, Guo, Ruitang, Chen, Quhan, Zhu, Huiwen, Li, Hongzhe, Yan, Zijun, Guo, Zeyu, Wu, Tao
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 07.04.2023
MDPI
Subjects
Carbon dioxide
Carbon monoxide
Catalysis
Climate change
CO2 reduction
Electrocatalysis
Electrodes
Electrolytes
graphitic phase carbon nitride (g-C3N4)
Hydrogen
Morphology
Nitrogen
novel catalyst carrier
Photocatalysis
Pore size
Review
single atom catalyst
Online AccessGet full text
ISSN1420-3049
1420-3049
DOI10.3390/molecules28083292

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Abstract The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C3N4) has excellent chemical stability and unique structural properties that allow it to be widely used in energy and materials fields. However, due to its relatively low electrical conductivity, to date, little effort has been made to summarize the application of g-C3N4 in the electrocatalytic reduction of CO2. This review focuses on the synthesis and functionalization of g-C3N4 and the recent advances of its application as a catalyst and a catalyst support in the electrocatalytic reduction of CO2. The modification of g-C3N4-based catalysts for enhanced CO2 reduction is critically reviewed. In addition, opportunities for future research on g-C3N4-based catalysts for electrocatalytic CO2 reduction are discussed.
AbstractList The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C3N4) has excellent chemical stability and unique structural properties that allow it to be widely used in energy and materials fields. However, due to its relatively low electrical conductivity, to date, little effort has been made to summarize the application of g-C3N4 in the electrocatalytic reduction of CO2. This review focuses on the synthesis and functionalization of g-C3N4 and the recent advances of its application as a catalyst and a catalyst support in the electrocatalytic reduction of CO2. The modification of g-C3N4-based catalysts for enhanced CO2 reduction is critically reviewed. In addition, opportunities for future research on g-C3N4-based catalysts for electrocatalytic CO2 reduction are discussed.The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C3N4) has excellent chemical stability and unique structural properties that allow it to be widely used in energy and materials fields. However, due to its relatively low electrical conductivity, to date, little effort has been made to summarize the application of g-C3N4 in the electrocatalytic reduction of CO2. This review focuses on the synthesis and functionalization of g-C3N4 and the recent advances of its application as a catalyst and a catalyst support in the electrocatalytic reduction of CO2. The modification of g-C3N4-based catalysts for enhanced CO2 reduction is critically reviewed. In addition, opportunities for future research on g-C3N4-based catalysts for electrocatalytic CO2 reduction are discussed.
The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C3N4) has excellent chemical stability and unique structural properties that allow it to be widely used in energy and materials fields. However, due to its relatively low electrical conductivity, to date, little effort has been made to summarize the application of g-C3N4 in the electrocatalytic reduction of CO2. This review focuses on the synthesis and functionalization of g-C3N4 and the recent advances of its application as a catalyst and a catalyst support in the electrocatalytic reduction of CO2. The modification of g-C3N4-based catalysts for enhanced CO2 reduction is critically reviewed. In addition, opportunities for future research on g-C3N4-based catalysts for electrocatalytic CO2 reduction are discussed.
The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions. Carbon nitride in the graphitic phase (g-C 3 N 4 ) has excellent chemical stability and unique structural properties that allow it to be widely used in energy and materials fields. However, due to its relatively low electrical conductivity, to date, little effort has been made to summarize the application of g-C 3 N 4 in the electrocatalytic reduction of CO 2 . This review focuses on the synthesis and functionalization of g-C 3 N 4 and the recent advances of its application as a catalyst and a catalyst support in the electrocatalytic reduction of CO 2 . The modification of g-C 3 N 4 -based catalysts for enhanced CO 2 reduction is critically reviewed. In addition, opportunities for future research on g-C 3 N 4 -based catalysts for electrocatalytic CO 2 reduction are discussed.
Author Mao, Xinyi
Li, Hongzhe
Yan, Zijun
Wu, Tao
Zhu, Huiwen
Chen, Quhan
Guo, Zeyu
Guo, Ruitang
AuthorAffiliation 3 Municipal Key Laboratory of Clean Energy Technologies of Ningbo, University of Nottingham Ningbo China, Ningbo 315100, China
2 Department of Chemical and Environmental Engineering, University of Nottingham Ningbo China, Ningbo 315100, China
1 College of Energy and Mechanical Engineering, Shanghai University of Electric Power, Shanghai 200090, China
4 Key Laboratory of Carbonaceous Wastes Processing and Process Intensification of Zhejiang Province, University of Nottingham Ningbo China, Ningbo 315100, China
AuthorAffiliation_xml – name: 2 Department of Chemical and Environmental Engineering, University of Nottingham Ningbo China, Ningbo 315100, China
– name: 4 Key Laboratory of Carbonaceous Wastes Processing and Process Intensification of Zhejiang Province, University of Nottingham Ningbo China, Ningbo 315100, China
– name: 1 College of Energy and Mechanical Engineering, Shanghai University of Electric Power, Shanghai 200090, China
– name: 3 Municipal Key Laboratory of Clean Energy Technologies of Ningbo, University of Nottingham Ningbo China, Ningbo 315100, China
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Snippet The electrocatalytic carbon dioxide reduction reaction is an effective means of combating the greenhouse effect caused by massive carbon dioxide emissions....
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StartPage 3292
SubjectTerms Carbon dioxide
Carbon monoxide
Catalysis
Climate change
CO2 reduction
Electrocatalysis
Electrodes
Electrolytes
graphitic phase carbon nitride (g-C3N4)
Hydrogen
Morphology
Nitrogen
novel catalyst carrier
Photocatalysis
Pore size
Review
single atom catalyst
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Title Recent Advances in Graphitic Carbon Nitride Based Electro-Catalysts for CO2 Reduction Reactions
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Volume 28
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