Domain Wall Patterning and Giant Response Functions in Ferrimagnetic Spinels

The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechani...

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Published inAdvanced science Vol. 8; no. 23; pp. e2101402 - n/a
Main Authors Kish, Lazar L., Thaler, Alex, Lee, Minseong, Zakrzewski, Alexander V., Reig‐i‐Plessis, Dalmau, Wolin, Brian A., Wang, Xu, Littrell, Kenneth C., Budakian, Raffi, Zhou, Haidong, Gai, Zheng, Frontzek, Matthias D., Zapf, Vivien S., Aczel, Adam A., DeBeer‐Schmitt, Lisa, MacDougall, Gregory J.
Format Journal Article
LanguageEnglish
Published Germany John Wiley & Sons, Inc 01.12.2021
Wiley
John Wiley and Sons Inc
Subjects
Collaboration
Crystal structure
domain walls
Ferroelectrics
High Magnetic Field Science
magnetodielectrics
magnetoelastics
magnetostructural transitions
MATERIALS SCIENCE
Microscopy
small‐angle neutron scattering
magnetostructural transitions
small-angle neutron scattering
domain walls
magnetoelastics
magnetodielectrics
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Abstract The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn3O4 and MnV2O4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data. Magnetostructural transitions in the ferrimagnetic spinels Mn3O4 and MnV2O4 are linked to increased spin–lattice coupling, from which novel magnetic domain structures emerge on the mesoscale. Small‐angle neutron scattering measures the response of these domain patterns to applied magnetic field and stress. Correlations between scattering and bulk probes demonstrate tuning of macroscopic response functions via alterations to the domain structure.
AbstractList The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn3 O4 and MnV2 O4 and stripe-like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small-angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn3O4 and MnV2O4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn 3 O 4 and MnV 2 O 4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data. Magnetostructural transitions in the ferrimagnetic spinels Mn 3 O 4 and MnV 2 O 4 are linked to increased spin–lattice coupling, from which novel magnetic domain structures emerge on the mesoscale. Small‐angle neutron scattering measures the response of these domain patterns to applied magnetic field and stress. Correlations between scattering and bulk probes demonstrate tuning of macroscopic response functions via alterations to the domain structure.
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn3O4 and MnV2O4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data. Magnetostructural transitions in the ferrimagnetic spinels Mn3O4 and MnV2O4 are linked to increased spin–lattice coupling, from which novel magnetic domain structures emerge on the mesoscale. Small‐angle neutron scattering measures the response of these domain patterns to applied magnetic field and stress. Correlations between scattering and bulk probes demonstrate tuning of macroscopic response functions via alterations to the domain structure.
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn O and MnV O and stripe-like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small-angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
Abstract The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn3O4 and MnV2O4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn 3 O 4 and MnV 2 O 4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
Author Lee, Minseong
Wang, Xu
Thaler, Alex
Zakrzewski, Alexander V.
Littrell, Kenneth C.
Aczel, Adam A.
Wolin, Brian A.
Frontzek, Matthias D.
MacDougall, Gregory J.
Zapf, Vivien S.
Zhou, Haidong
Gai, Zheng
Kish, Lazar L.
DeBeer‐Schmitt, Lisa
Budakian, Raffi
Reig‐i‐Plessis, Dalmau
AuthorAffiliation 2 National High Magnetic Field Laboratory Los Alamos National Laboratory Los Alamos NM 87544 USA
1 Department of Physics and Materials Research Laboratory University of Illinois at Urbana‐Champaign Urbana IL 61801 USA
4 Department of Physics and Astronomy University of Tennessee Knoxville Tennessee 37996 USA
5 Department of Physics and Astronomy University of Waterloo Waterloo Ontario N2L 3G1 Canada
6 Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak Ridge TN 37831 USA
7 Neutron Scattering Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA
3 Department of Physics and Astronomy and Quantum Matter Institute University of British Columbia Vancouver British Columbia V6T 1Z1 Canada
AuthorAffiliation_xml – name: 4 Department of Physics and Astronomy University of Tennessee Knoxville Tennessee 37996 USA
– name: 7 Neutron Scattering Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA
– name: 1 Department of Physics and Materials Research Laboratory University of Illinois at Urbana‐Champaign Urbana IL 61801 USA
– name: 2 National High Magnetic Field Laboratory Los Alamos National Laboratory Los Alamos NM 87544 USA
– name: 3 Department of Physics and Astronomy and Quantum Matter Institute University of British Columbia Vancouver British Columbia V6T 1Z1 Canada
– name: 6 Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak Ridge TN 37831 USA
– name: 5 Department of Physics and Astronomy University of Waterloo Waterloo Ontario N2L 3G1 Canada
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  email: gmacdoug@illinois.edu
  organization: University of Illinois at Urbana‐Champaign
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https://www.osti.gov/biblio/1828393$$D View this record in Osti.gov
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Issue 23
Keywords magnetostructural transitions
small-angle neutron scattering
domain walls
magnetoelastics
magnetodielectrics
Language English
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35199496 - Adv Sci (Weinh). 2022 Feb;9(6):e2200207
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Snippet The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its...
Abstract The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices,...
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SubjectTerms Collaboration
Crystal structure
domain walls
Ferroelectrics
High Magnetic Field Science
magnetodielectrics
magnetoelastics
magnetostructural transitions
MATERIALS SCIENCE
Microscopy
small‐angle neutron scattering
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Title Domain Wall Patterning and Giant Response Functions in Ferrimagnetic Spinels
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadvs.202101402
https://www.ncbi.nlm.nih.gov/pubmed/34719881
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