Polycyclic aromatic compounds-modified graphitic carbon nitride for efficient visible-light-driven hydrogen evolution
Polycyclic aromatic compounds with strong conjugated effect, possess the advantage of improving electronic polarizability, thus accelerating the electron transportation. Here, a facile copolymerization between urea and polycyclic aromatic compounds (benzoic acid, naphthoic acid and anthroic acid) ha...
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| Published in | Carbon (New York) Vol. 134; pp. 134 - 144 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Elsevier Ltd
01.08.2018
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Polycyclic aromatic compounds with strong conjugated effect, possess the advantage of improving electronic polarizability, thus accelerating the electron transportation. Here, a facile copolymerization between urea and polycyclic aromatic compounds (benzoic acid, naphthoic acid and anthroic acid) has been applied to constructing aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts. Incorporation of aromatic rings in the GCN network is an effective protocol to extend its π-conjugated system for visible light harvesting and improves the charge transfer efficiency for prolonging lifetime of photogenerated charge carriers in photocatalytic reactions. The corresponding characterization methods demonstrate that the aromatic rings-modified GCN can effectively narrow the bandgap to favor broad band visible light absorption and suppress recombination of electrons and holes. Remarkably, the moderate conjugated effect of aromatic rings (naphthalene) is crucial to promote charge separation. The developed naphthalene-grafted GCN achieves the highest water splitting performance with hydrogen evolution rate up to 102.1 μmol h−1, nearly 3.5 times of that of the GCN, and apparent quantum efficiency reaches 5.6% at 450 nm. This finding reveals that the conjugated effect of aromatic rings is significant to control photocatalytic property and brings new ideas for designing aromatic system-modified GCN as highly active photocatalysts towards solar-to-chemical energy conversion.
This study reports the preparation, characterization and photocatalytic activity of aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts, which display enhanced visible light absorption and improved separation of charge carriers due to the extended π-conjugated system, and thus the high hydrogen evolution rate. [Display omitted] |
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| AbstractList | Polycyclic aromatic compounds with strong conjugated effect, possess the advantage of improving electronic polarizability, thus accelerating the electron transportation. Here, a facile copolymerization between urea and polycyclic aromatic compounds (benzoic acid, naphthoic acid and anthroic acid) has been applied to constructing aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts. Incorporation of aromatic rings in the GCN network is an effective protocol to extend its π-conjugated system for visible light harvesting and improves the charge transfer efficiency for prolonging lifetime of photogenerated charge carriers in photocatalytic reactions. The corresponding characterization methods demonstrate that the aromatic rings-modified GCN can effectively narrow the bandgap to favor broad band visible light absorption and suppress recombination of electrons and holes. Remarkably, the moderate conjugated effect of aromatic rings (naphthalene) is crucial to promote charge separation. The developed naphthalene-grafted GCN achieves the highest water splitting performance with hydrogen evolution rate up to 102.1 μmol h−1, nearly 3.5 times of that of the GCN, and apparent quantum efficiency reaches 5.6% at 450 nm. This finding reveals that the conjugated effect of aromatic rings is significant to control photocatalytic property and brings new ideas for designing aromatic system-modified GCN as highly active photocatalysts towards solar-to-chemical energy conversion.
This study reports the preparation, characterization and photocatalytic activity of aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts, which display enhanced visible light absorption and improved separation of charge carriers due to the extended π-conjugated system, and thus the high hydrogen evolution rate. [Display omitted] Polycyclic aromatic compounds with strong conjugated effect, possess the advantage of improving electronic polarizability, thus accelerating the electron transportation. Here, a facile copolymerization between urea and polycyclic aromatic compounds (benzoic acid, naphthoic acid and anthroic acid) has been applied to constructing aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts. Incorporation of aromatic rings in the GCN network is an effective protocol to extend its π-conjugated system for visible light harvesting and improves the charge transfer efficiency for prolonging lifetime of photogenerated charge carriers in photocatalytic reactions. The corresponding characterization methods demonstrate that the aromatic rings-modified GCN can effectively narrow the bandgap to favor broad band visible light absorption and suppress recombination of electrons and holes. Remarkably, the moderate conjugated effect of aromatic rings (naphthalene) is crucial to promote charge separation. The developed naphthalene-grafted GCN achieves the highest water splitting performance with hydrogen evolution rate up to 102.1 μmol h−1, nearly 3.5 times of that of the GCN, and apparent quantum efficiency reaches 5.6% at 450 nm. This finding reveals that the conjugated effect of aromatic rings is significant to control photocatalytic property and brings new ideas for designing aromatic system-modified GCN as highly active photocatalysts towards solar-to-chemical energy conversion. Polycyclic aromatic compounds with strong conjugated effect, possess the advantage of improving electronic polarizability, thus accelerating the electron transportation. Here, a facile copolymerization between urea and polycyclic aromatic compounds (benzoic acid, naphthoic acid and anthroic acid) has been applied to constructing aromatic rings-grafted graphitic carbon nitride (GCN) photocatalysts. Incorporation of aromatic rings in the GCN network is an effective protocol to extend its π-conjugated system for visible light harvesting and improves the charge transfer efficiency for prolonging lifetime of photogenerated charge carriers in photocatalytic reactions. The corresponding characterization methods demonstrate that the aromatic rings-modified GCN can effectively narrow the bandgap to favor broad band visible light absorption and suppress recombination of electrons and holes. Remarkably, the moderate conjugated effect of aromatic rings (naphthalene) is crucial to promote charge separation. The developed naphthalene-grafted GCN achieves the highest water splitting performance with hydrogen evolution rate up to 102.1 μmol h⁻¹, nearly 3.5 times of that of the GCN, and apparent quantum efficiency reaches 5.6% at 450 nm. This finding reveals that the conjugated effect of aromatic rings is significant to control photocatalytic property and brings new ideas for designing aromatic system-modified GCN as highly active photocatalysts towards solar-to-chemical energy conversion. |
| Author | Li, Kui Sun, Miao Zhang, Wei-De |
| Author_xml | – sequence: 1 givenname: Kui surname: Li fullname: Li, Kui – sequence: 2 givenname: Miao surname: Sun fullname: Sun, Miao – sequence: 3 givenname: Wei-De orcidid: 0000-0003-2483-626X surname: Zhang fullname: Zhang, Wei-De email: zhangwd@scut.edu.cn |
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| Keywords | Conjugated effect Polycyclic aromatic compounds Photocatalysis Hydrogen evolution Graphitic carbon nitride |
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| SubjectTerms | Aromatic compounds Benzoic acid Carbon Carbon nitride Charge efficiency Charge transfer Chemical compounds Chemical energy Conjugated effect Copolymerization Copolymers Current carriers Electromagnetic absorption Electron recombination electron transfer electrons Energy conversion graphene Graphitic carbon nitride Hydrogen Hydrogen evolution hydrogen production Naphthalene Organic chemistry Photocatalysis Photocatalysts Polycyclic aromatic compounds Polycyclic aromatic hydrocarbons polycyclic compounds Quantum efficiency urea Water splitting |
| Title | Polycyclic aromatic compounds-modified graphitic carbon nitride for efficient visible-light-driven hydrogen evolution |
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