Virtual Frisch grid perovskite CsPbBr3 semiconductor with 2.2-centimeter thickness for high energy resolution gamma-ray spectrometer

High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr 3 detector up to 2.2 cm thick...

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Published in	Nature communications Vol. 16; no. 1; pp. 158 - 10
Main Authors	Qin, Haoming, Xiao, Bao, He, Xuchang, Ouyang, Xiao, Gao, Tingting, Wang, Yuquan, Wang, Luyao, Sun, Qihao, Shen, Nannan, Ouyang, Xiaoping, He, Yihui
Format	Journal Article
Language	English
Published	London Nature Publishing Group UK 02.01.2025 Nature Publishing Group Nature Portfolio
Subjects	639/301/119 639/766/1130 Carrier recombination Configurations Crystal defects Crystals Current carriers Detectors Efficiency Energy distribution Energy resolution Fabrication Gamma ray detectors Gamma ray spectrometers Gamma rays Gamma spectroscopy Humanities and Social Sciences multidisciplinary Perovskites Recombination Science Science (multidisciplinary) Semiconductors Sensors Single crystals Space charge Spectral sensitivity Spectroscopy Thickness Time measurement
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Abstract	High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr 3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr 3 single crystals up to ~1 cm 3 , we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors. Qin et al. report single crystalline columnar CsPbBr3 with thickness up to 2.2 cm in a hole-only virtual Frisch grid configuration for gamma-ray detector with energy resolution of 1.9% at 662 keV. Time-of-light measurement reveals hole multiplication due to the defect-assisted Auger recombination.
AbstractList	High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr 3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr 3 single crystals up to ~1 cm 3 , we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors. Qin et al. report single crystalline columnar CsPbBr3 with thickness up to 2.2 cm in a hole-only virtual Frisch grid configuration for gamma-ray detector with energy resolution of 1.9% at 662 keV. Time-of-light measurement reveals hole multiplication due to the defect-assisted Auger recombination. High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr3 single crystals up to ~1 cm3, we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors.High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr3 single crystals up to ~1 cm3, we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors. High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr3 single crystals up to ~1 cm3, we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors.Qin et al. report single crystalline columnar CsPbBr3 with thickness up to 2.2 cm in a hole-only virtual Frisch grid configuration for gamma-ray detector with energy resolution of 1.9% at 662 keV. Time-of-light measurement reveals hole multiplication due to the defect-assisted Auger recombination. Abstract High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite semiconductors from reaching sufficient detection efficiency. We report a hole-only virtual-Frisch-grid CsPbBr3 detector up to 2.2 cm thick for efficient gamma-ray spectroscopy. By utilizing high-quality columnar CsPbBr3 single crystals up to ~1 cm3, we configure virtual-Frisch-grid detectors with optimized weighting potential distribution. These centimeter-thick detectors outperform ambipolar planar configuration, achieving a champion energy resolution of 1.9% at 662 keV. Time-of-flight analysis, stimulated by single gamma-ray photon, reveals hole carrier multiplication effect possibly caused by Auger recombination and space charge accumulation effect, collectively driving an anomalous stabilization process. Digital pulse measurements reduce the ballistic deficit, thereby improving the spectral response to 2.2% at 662 keV for 2.2 cm thick detector. The low-cost device fabrication and adequate detection efficiency of virtual-Frisch-grid detectors will surely foster the development of large-volume perovskite detectors.
ArticleNumber	158
Author	Gao, Tingting Shen, Nannan Qin, Haoming He, Yihui He, Xuchang Sun, Qihao Wang, Luyao Wang, Yuquan Ouyang, Xiao Ouyang, Xiaoping Xiao, Bao
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Snippet	High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing perovskite... Abstract High intrinsic detection efficiency is as decisive as high energy resolution. Scaling up detector volume has presented great challenges, preventing...
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SubjectTerms	639/301/119 639/766/1130 Carrier recombination Configurations Crystal defects Crystals Current carriers Detectors Efficiency Energy distribution Energy resolution Fabrication Gamma ray detectors Gamma ray spectrometers Gamma rays Gamma spectroscopy Humanities and Social Sciences multidisciplinary Perovskites Recombination Science Science (multidisciplinary) Semiconductors Sensors Single crystals Space charge Spectral sensitivity Spectroscopy Thickness Time measurement
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Title	Virtual Frisch grid perovskite CsPbBr3 semiconductor with 2.2-centimeter thickness for high energy resolution gamma-ray spectrometer
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