Formation of tooeleite and the role of direct removal of As(III) from high-arsenic acid wastewater
[Display omitted] A novel method for direct removal of As(III) by forming tooeleite is developed.Arsenic removal efficiency can reach 99% for high As(III) concentration of 7.5g/L.Ferrihydrite contributes to the formation of tooeleite and the removal of As(III). In this study, an earth-mimetic met...
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| Published in | Journal of hazardous materials Vol. 320; pp. 620 - 627 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
15.12.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
A novel method for direct removal of As(III) by forming tooeleite is developed.Arsenic removal efficiency can reach 99% for high As(III) concentration of 7.5g/L.Ferrihydrite contributes to the formation of tooeleite and the removal of As(III).
In this study, an earth-mimetic method was proposed for the direct removal of As(III) by the formation of tooeleite, a ferric arsenite sulfate mineral. A series of batch experiments was used to study the relationship between the formation of tooeleite and the removal of As(III). The results indicate that As(III) removal efficiency reached up to 99% under the treatment condition of pH 1.8⿿4.5, initial As(III) concentration higher than 0.75g/L, and Fe/As ranged from 0.8 to 2 at room temperature. Various characterizations confirm that the precipitate obtained by this treatment was tooeleite with relatively high stability. In addition, it is assumed that ferrihydrite exists as a precursor, which is vital to the formation of tooeleite and the removal of As(III). This study suggests that tooeleite formation may be an alternative method in the direct removal of As(III) from high-arsenic acid wastewater. |
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| AbstractList | In this study, an earth-mimetic method was proposed for the direct removal of As(III) by the formation of tooeleite, a ferric arsenite sulfate mineral. A series of batch experiments was used to study the relationship between the formation of tooeleite and the removal of As(III). The results indicate that As(III) removal efficiency reached up to 99% under the treatment condition of pH 1.8-4.5, initial As(III) concentration higher than 0.75g/L, and Fe/As ranged from 0.8 to 2 at room temperature. Various characterizations confirm that the precipitate obtained by this treatment was tooeleite with relatively high stability. In addition, it is assumed that ferrihydrite exists as a precursor, which is vital to the formation of tooeleite and the removal of As(III). This study suggests that tooeleite formation may be an alternative method in the direct removal of As(III) from high-arsenic acid wastewater. [Display omitted] A novel method for direct removal of As(III) by forming tooeleite is developed.Arsenic removal efficiency can reach 99% for high As(III) concentration of 7.5g/L.Ferrihydrite contributes to the formation of tooeleite and the removal of As(III). In this study, an earth-mimetic method was proposed for the direct removal of As(III) by the formation of tooeleite, a ferric arsenite sulfate mineral. A series of batch experiments was used to study the relationship between the formation of tooeleite and the removal of As(III). The results indicate that As(III) removal efficiency reached up to 99% under the treatment condition of pH 1.8⿿4.5, initial As(III) concentration higher than 0.75g/L, and Fe/As ranged from 0.8 to 2 at room temperature. Various characterizations confirm that the precipitate obtained by this treatment was tooeleite with relatively high stability. In addition, it is assumed that ferrihydrite exists as a precursor, which is vital to the formation of tooeleite and the removal of As(III). This study suggests that tooeleite formation may be an alternative method in the direct removal of As(III) from high-arsenic acid wastewater. |
| Author | Yang, Jinqin Liu, Hui Yue, Mengqing Li, Qingzhu Wang, Qingwei Chai, Liyuan |
| Author_xml | – sequence: 1 givenname: Liyuan surname: Chai fullname: Chai, Liyuan organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China – sequence: 2 givenname: Mengqing surname: Yue fullname: Yue, Mengqing organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China – sequence: 3 givenname: Jinqin surname: Yang fullname: Yang, Jinqin organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China – sequence: 4 givenname: Qingwei surname: Wang fullname: Wang, Qingwei email: qw_wang@csu.edu.cn organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China – sequence: 5 givenname: Qingzhu surname: Li fullname: Li, Qingzhu email: qingzhuli@csu.edu.cn organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China – sequence: 6 givenname: Hui surname: Liu fullname: Liu, Hui organization: School of Metallurgy and Environment, Central South University, Changsha 410083, China |
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A novel method for direct removal of As(III) by forming tooeleite is developed.Arsenic removal efficiency can reach 99% for high As(III)... In this study, an earth-mimetic method was proposed for the direct removal of As(III) by the formation of tooeleite, a ferric arsenite sulfate mineral. A... |
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| SubjectTerms | Acid wastewater Arsenite Efficiency Ferrihydrite Formations Hazardous wastes Precipitates Precipitation Precursors Stability Tooeleite Wastewater treatment |
| Title | Formation of tooeleite and the role of direct removal of As(III) from high-arsenic acid wastewater |
| URI | https://dx.doi.org/10.1016/j.jhazmat.2016.07.069 https://www.ncbi.nlm.nih.gov/pubmed/27528124 https://search.proquest.com/docview/1827915799 https://search.proquest.com/docview/1835383662 https://search.proquest.com/docview/1845825953 |
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