The investigation of giant magnetic moment in ultrathin Fe3O4 films

The magnetic and transport properties of Fe3O4 films with a series of thicknesses are investigated. For the films with thickness below 15 nm, the saturation magnetization (Ms) increases and the coercivity decreases with the decrease in films’ thickness. The Ms of 3 nm Fe3O4 film is dramatically incr...

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Published inAPL materials Vol. 4; no. 3; pp. 036104 - 036104-6
Main Authors Guan, Xiaofen, Zhou, Guowei, Xue, Wuhong, Quan, Zhiyong, Xu, Xiaohong
Format Journal Article
LanguageEnglish
Published AIP Publishing LLC 01.03.2016
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Abstract The magnetic and transport properties of Fe3O4 films with a series of thicknesses are investigated. For the films with thickness below 15 nm, the saturation magnetization (Ms) increases and the coercivity decreases with the decrease in films’ thickness. The Ms of 3 nm Fe3O4 film is dramatically increased to 1017 emu/cm3. As for films’ thickness more than 15 nm, Ms is tending to be close to the Fe3O4 bulk value. Furthermore, the Verwey transition temperature (Tv) is visible for all the films, but suppressed for 3 nm film. We also find that the ρ of 3 nm film is the highest of all the films. The suppressed Tv and high ρ may be related to the islands morphology in 3 nm film. To study the structure, magnetic, and transport properties of the Fe3O4 films, we propose that the giant magnetic moment most likely comes from the spin of Fe ions in the tetrahedron site switching parallel to the Fe ions in the octahedron site at the surface, interface, and grain boundaries. The above results are of great significance and also provide a promising future for either device applications or fundamental research.
AbstractList The magnetic and transport properties of Fe3O4 films with a series of thicknesses are investigated. For the films with thickness below 15 nm, the saturation magnetization (Ms) increases and the coercivity decreases with the decrease in films’ thickness. The Ms of 3 nm Fe3O4 film is dramatically increased to 1017 emu/cm3. As for films’ thickness more than 15 nm, Ms is tending to be close to the Fe3O4 bulk value. Furthermore, the Verwey transition temperature (Tv) is visible for all the films, but suppressed for 3 nm film. We also find that the ρ of 3 nm film is the highest of all the films. The suppressed Tv and high ρ may be related to the islands morphology in 3 nm film. To study the structure, magnetic, and transport properties of the Fe3O4 films, we propose that the giant magnetic moment most likely comes from the spin of Fe ions in the tetrahedron site switching parallel to the Fe ions in the octahedron site at the surface, interface, and grain boundaries. The above results are of great significance and also provide a promising future for either device applications or fundamental research.
Author Quan, Zhiyong
Zhou, Guowei
Xue, Wuhong
Guan, Xiaofen
Xu, Xiaohong
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Snippet The magnetic and transport properties of Fe3O4 films with a series of thicknesses are investigated. For the films with thickness below 15 nm, the saturation...
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Title The investigation of giant magnetic moment in ultrathin Fe3O4 films
URI http://dx.doi.org/10.1063/1.4944590
https://doaj.org/article/acadee9ef592451085fc43277fe9e731
Volume 4
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