Tailored topotactic chemistry unlocks heterostructures of magnetic intercalation compounds

The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between...

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Published inNature communications Vol. 16; no. 1; pp. 1208 - 12
Main Authors Husremović, Samra, Gonzalez, Oscar, Goodge, Berit H., Xie, Lilia S., Kong, Zhizhi, Zhang, Wanlin, Ryu, Sae Hee, Ribet, Stephanie M., Fender, Shannon S., Bustillo, Karen C., Song, Chengyu, Ciston, Jim, Taniguchi, Takashi, Watanabe, Kenji, Ophus, Colin, Jozwiak, Chris, Bostwick, Aaron, Rotenberg, Eli, Bediako, D. Kwabena
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 31.01.2025
Nature Publishing Group
Nature Portfolio
Subjects
639/301/357/1018
639/638/298/920
639/925/357/997
Annealing
Chalcogenides
Chemical synthesis
Chemistry
Controllability
Crystallography
Design
Dissimilar materials
Electrons
Heterostructures
Humanities and Social Sciences
Intercalation
Intercalation compounds
Laboratories
Magnetic properties
Metal oxides
Metals
Microscopy
multidisciplinary
Multilayers
Oxide coatings
Physical properties
Science
Science (multidisciplinary)
Thin films
Transition metal compounds
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Abstract The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry. Synthesis of heterostructures of magnetic intercalation compounds in transition metal dichalcogenides (TMDs) via directed topotactic reactions enables the creation of multi-component magnetic architectures, overcoming limitations of crystallographic incommensurability
AbstractList The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry.Synthesis of heterostructures of magnetic intercalation compounds in transition metal dichalcogenides (TMDs) via directed topotactic reactions enables the creation of multi-component magnetic architectures, overcoming limitations of crystallographic incommensurability
The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry.
Abstract The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry.
The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry.The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry.
The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This strategy is of particular importance for the design of multilayer magnetic architectures in which direct interfacial spin-spin interactions between magnetic phases in dissimilar layers lead to emergent and controllable magnetic behavior. However, crystallographic incommensurability and atomic-scale interfacial disorder can severely limit the types of materials amenable to this strategy, as well as the performance of these systems. Here, we demonstrate a method for synthesizing heterostructures comprising magnetic intercalation compounds of transition metal dichalcogenides (TMDs), through directed topotactic reaction of the TMD with a metal oxide. The mechanism of the intercalation reaction enables thermally initiated intercalation of the TMD from lithographically patterned oxide films, giving access to a family of multi-component magnetic architectures through the combination of deterministic van der Waals assembly and directed intercalation chemistry. Synthesis of heterostructures of magnetic intercalation compounds in transition metal dichalcogenides (TMDs) via directed topotactic reactions enables the creation of multi-component magnetic architectures, overcoming limitations of crystallographic incommensurability
ArticleNumber 1208
Author Gonzalez, Oscar
Goodge, Berit H.
Bustillo, Karen C.
Taniguchi, Takashi
Fender, Shannon S.
Rotenberg, Eli
Ribet, Stephanie M.
Xie, Lilia S.
Bediako, D. Kwabena
Jozwiak, Chris
Husremović, Samra
Ciston, Jim
Song, Chengyu
Kong, Zhizhi
Zhang, Wanlin
Ophus, Colin
Watanabe, Kenji
Bostwick, Aaron
Ryu, Sae Hee
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Snippet The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties. This...
Abstract The construction of thin film heterostructures has been a widely successful archetype for fabricating materials with emergent physical properties....
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StartPage 1208
SubjectTerms 639/301/357/1018
639/638/298/920
639/925/357/997
Annealing
Chalcogenides
Chemical synthesis
Chemistry
Controllability
Crystallography
Design
Dissimilar materials
Electrons
Heterostructures
Humanities and Social Sciences
Intercalation
Intercalation compounds
Laboratories
Magnetic properties
Metal oxides
Metals
Microscopy
multidisciplinary
Multilayers
Oxide coatings
Physical properties
Science
Science (multidisciplinary)
Thin films
Transition metal compounds
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Title Tailored topotactic chemistry unlocks heterostructures of magnetic intercalation compounds
URI https://link.springer.com/article/10.1038/s41467-025-56467-9
https://www.ncbi.nlm.nih.gov/pubmed/39885123
https://www.proquest.com/docview/3161623234
https://www.proquest.com/docview/3161915829
https://www.osti.gov/servlets/purl/2528036
https://doaj.org/article/42aae75e229a409991a746a18fb06c55
Volume 16
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