The interplay of thermally activated delayed fluorescence (TADF) and room temperature organic phosphorescence in sterically-constrained donor-acceptor charge-transfer molecules
A series of phenothiazine-dibenzothiophene-S, S-dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the donor-acceptor bond significantly alters contributions from TADF and phosphorescence. Bulky substituents on the 1-(and 9) position(s) of the phenothiazine...
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Published in | Chemical communications (Cambridge, England) Vol. 52; no. 12; pp. 2612 - 2615 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
CAMBRIDGE
Royal Soc Chemistry
11.02.2016
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Abstract | A series of phenothiazine-dibenzothiophene-S, S-dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the donor-acceptor bond significantly alters contributions from TADF and phosphorescence. Bulky substituents on the 1-(and 9) position(s) of the phenothiazine result in no TADF in the solid state; instead strong phosphorescence is observed at ambient temperature. |
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AbstractList | A series of phenothiazine-dibenzothiophene-S,S-dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the donor-acceptor bond significantly alters contributions from TADF and phosphorescence. Bulky substituents on the 1-(and 9) position(s) of the phenothiazine result in no TADF in the solid state; instead strong phosphorescence is observed at ambient temperature. A series of phenothiazine–dibenzothiophene- S , S -dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the donor–acceptor bond significantly alters contributions from TADF and phosphorescence. Bulky substituents on the 1-(and 9) position(s) of the phenothiazine result in no TADF in the solid state; instead strong phosphorescence is observed at ambient temperature. |
Author | Data, Przemyslaw Ward, Jonathan S. Monkman, Andrew P. Dias, Fernando B. Nobuyasu, Roberto S. Batsanov, Andrei S. Bryce, Martin R. |
Author_xml | – sequence: 1 givenname: Jonathan S. orcidid: 0000-0002-4985-8572 surname: Ward fullname: Ward, Jonathan S. organization: Univ Durham, Dept Chem, South Rd, Durham DH1 3LE, England – sequence: 2 givenname: Roberto S. surname: Nobuyasu fullname: Nobuyasu, Roberto S. organization: Univ Durham, Dept Phys, Durham DH1 3LE, England – sequence: 3 givenname: Andrei S. surname: Batsanov fullname: Batsanov, Andrei S. organization: Univ Durham, Dept Chem, South Rd, Durham DH1 3LE, England – sequence: 4 givenname: Przemyslaw orcidid: 0000-0002-1831-971X surname: Data fullname: Data, Przemyslaw organization: Univ Durham, Dept Phys, Durham DH1 3LE, England – sequence: 5 givenname: Andrew P. orcidid: 0000-0002-0784-8640 surname: Monkman fullname: Monkman, Andrew P. organization: Univ Durham, Dept Phys, Durham DH1 3LE, England – sequence: 6 givenname: Fernando B. orcidid: 0000-0001-9841-863X surname: Dias fullname: Dias, Fernando B. organization: Univ Durham, Dept Phys, Durham DH1 3LE, England – sequence: 7 givenname: Martin R. orcidid: 0000-0003-2097-7823 surname: Bryce fullname: Bryce, Martin R. email: m.r.bryce@durham.ac.uk organization: Univ Durham, Dept Chem, South Rd, Durham DH1 3LE, England |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26750426$$D View this record in MEDLINE/PubMed |
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Snippet | A series of phenothiazine-dibenzothiophene-S, S-dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the... A series of phenothiazine-dibenzothiophene-S,S-dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the donor-acceptor... A series of phenothiazine–dibenzothiophene- S , S -dioxide charge-transfer molecules have been synthesized. Increasing steric restriction around the... |
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SubjectTerms | Activated Ambient temperature Bonding Chemistry Chemistry, Multidisciplinary Constrictions Fluorescence Phenothiazines Phosphorescence Physical Sciences Science & Technology Solid state |
Title | The interplay of thermally activated delayed fluorescence (TADF) and room temperature organic phosphorescence in sterically-constrained donor-acceptor charge-transfer molecules |
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