The journey of tin chalcogenides towards high-performance thermoelectrics and topological materials
Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit ( zT ). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues...
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| Published in | Chemical communications (Cambridge, England) Vol. 54; no. 5; pp. 6573 - 659 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
2018
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 1359-7345 1364-548X 1364-548X |
| DOI | 10.1039/c8cc02230e |
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| Abstract | Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (
zT
). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin-orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials.
Sn-Chalcogenides are recognized as high performance thermoelectrics and topological insulators due to their unique crystal and electronic structures and lattice dynamics. |
|---|---|
| AbstractList | Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (
zT
). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin-orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials.
Sn-Chalcogenides are recognized as high performance thermoelectrics and topological insulators due to their unique crystal and electronic structures and lattice dynamics. Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit ( zT ). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin–orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials. Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (zT). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin–orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials. Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (zT). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin-orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials.Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (zT). However, recent research has shown a limitation in the use of lead (Pb)-based materials due to their toxicity and efforts have been made to produce non-toxic analogues of lead chalcogenides. Tin chalcogenides have been predicted to be promising for this purpose due to their unique electronic structure and phonon dispersion properties. Here, we discuss the journey of tin chalcogenides in the field of thermoelectrics and topological materials with the main emphasis on the bonding, crystal structures, electronic band structures, phonon dispersion and thermoelectric properties. The thermal transport properties of tin chalcogenides are explained based on lattice dynamics, where resonant bonding and local structural distortion play an important role in creating lattice anharmonicity, thereby lowering the lattice thermal conductivity. Since thermoelectric and topological materials, especially topological insulators and topological crystalline insulators, share similar material features, such as a narrow band gap, heavy constituent elements and significant spin-orbit coupling, we have discussed the thermoelectric properties of several topological tin chalcogenides from a chemistry perspective. This feature article serves as a useful reference for researchers who strive to improve the properties of tin chalcogenides and advance the field of thermoelectric and topological materials. |
| Author | Banik, Ananya Roychowdhury, Subhajit Biswas, Kanishka |
| AuthorAffiliation | New Chemistry Unit Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR) |
| AuthorAffiliation_xml | – name: New Chemistry Unit – name: Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR) |
| Author_xml | – sequence: 1 givenname: Ananya surname: Banik fullname: Banik, Ananya – sequence: 2 givenname: Subhajit surname: Roychowdhury fullname: Roychowdhury, Subhajit – sequence: 3 givenname: Kanishka surname: Biswas fullname: Biswas, Kanishka |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29749410$$D View this record in MEDLINE/PubMed |
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| Notes | Kanishka Biswas obtained his MS and PhD degree from the Solid State Structural Chemistry Unit at the Indian Institute of Science (2009) under the supervision of Prof. C. N. R. Rao and he did postdoctoral research with Prof. Mercouri G. Kanatzidis at the Department of Chemistry, Northwestern University (2009-2012). He is an Assistant Professor in the New Chemistry Unit, at the Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR), Bangalore. He is pursuing research in the solid state inorganic chemistry of metal chalcogenides, thermoelectrics, topological materials, 2D materials and perovskite halides. He has published 96 research papers, 1 book and 4 book chapters. He is a Young Affiliate of The World Academy of Sciences (TWAS) and an Associate of the Indian Academy of Science (IASc), Bangalore, India. He was also the recipient of a Young Scientist Medal in 2016 from the Indian National Science Academy (INSA), Delhi, India and Young Scientist Platinum Jubilee Award in 2015 from The National Academy of Sciences (NASI), Allahabad, India. He received a Materials Research Society of India Medal in 2017. He was the recipient of an IUMRS-MRS Singapore Young Researcher Merit Award in 2016 and he also received a Young Scientist Wiley Award from IUMRS in 2017 in Kyoto, Japan. Ananya Banik obtained her BSc degree from Presidency University, Kolkata in 2012 and her MS degree in Chemical Science in 2015 from the Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR). Currently, she is pursuing her PhD under Dr Kanishka Biswas at the New Chemistry Unit, at the Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR), Bangalore, India. Her research focuses on the thermoelectric properties of tin chalcogenides. Subhajit Roychowdhury received his BSc (2012) degree from the University of Burdwan and MSc (2014) degree in Chemistry from the Indian Institute of Technology (IIT), Kharagpur, West Bengal, India. He is currently pursuing his PhD under Dr Kanishka Biswas at the New Chemistry Unit, Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR), Bangalore, India. His research focuses on topological insulators and the thermoelectric properties of heavy metal chalcogenides. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 |
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| Snippet | Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (
zT
). However, recent research... Lead chalcogenides and their alloys belong at the heart of thermoelectrics due to their large thermoelectric figure of merit (zT). However, recent research has... |
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| SubjectTerms | alloys Anharmonicity Chalcogenides chemical reactions Crystal structure Dispersion Electronic structure Figure of merit Lead Organic chemistry Properties (attributes) Thermal conductivity Thermoelectric materials tin Topological insulators topology Toxicity |
| Title | The journey of tin chalcogenides towards high-performance thermoelectrics and topological materials |
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