Atomic site electrocatalysts for water splitting, oxygen reduction and selective oxidation
Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives...
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| Published in | Chemical Society reviews Vol. 49; no. 7; pp. 2215 - 2264 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
07.04.2020
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e
−
- ORR toward H
2
O/OH
−
and 2e
−
- ORR toward H
2
O
2
/HO
2
−
; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs.
This review summarized the fabrication routes and characterization methods of atomic site electrocatalysts (ASCs) followed by their applications for water splitting, oxygen reduction and selective oxidation. |
|---|---|
| AbstractList | Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e- - ORR toward H2O/OH- and 2e- - ORR toward H2O2/HO2-; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e − – ORR toward H 2 O/OH − and 2e − – ORR toward H 2 O 2 /HO 2 − ; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e− – ORR toward H2O/OH− and 2e− – ORR toward H2O2/HO2−; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e − - ORR toward H 2 O/OH − and 2e − - ORR toward H 2 O 2 /HO 2 − ; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. This review summarized the fabrication routes and characterization methods of atomic site electrocatalysts (ASCs) followed by their applications for water splitting, oxygen reduction and selective oxidation. Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e- - ORR toward H2O/OH- and 2e- - ORR toward H2O2/HO2-; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs.Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e- - ORR toward H2O/OH- and 2e- - ORR toward H2O2/HO2-; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. Electrocatalysis plays a central role in clean energy conversion, enabling a number of processes for future sustainable technologies. Atomic site electrocatalysts (ASCs), including single-atomic site catalysts (SASCs) and diatomic site catalysis (DASCs), are being pursued as economical alternatives to noble-metal-based catalysts for these reactions by virtue of their exceptionally high atom utilization efficiencies, well-defined active sites and high selectivities. In this review, we start from a systematic review on the fabrication routes of ASCs followed by an overview of some new and effective characterization methods to precisely probe the atomic structure. Then we give a comprehensive summary on the current advances in some typical clean energy reactions: water splitting, including hydrogen evolution reaction (HER) and oxygen evolution reaction (OER); oxygen reduction reaction (ORR), including selective 4e⁻ – ORR toward H₂O/OH⁻ and 2e⁻ – ORR toward H₂O₂/HO₂⁻; selective electrooxidation of formic acid, methanol and ethanol (FAOR, MOR and EOR). At the end of this paper, we present a brief conclusion, and discuss the challenges and opportunities on the further development of more selective, active, stable and less expensive ASCs. |
| Author | Chen, Chen Li, Yadong Zhang, Chao Peng, Qing Zhuang, Zewen Zhao, Di Cao, Xing |
| AuthorAffiliation | Department of Chemistry Tsinghua University |
| AuthorAffiliation_xml | – name: Department of Chemistry – name: Tsinghua University |
| Author_xml | – sequence: 1 givenname: Di surname: Zhao fullname: Zhao, Di – sequence: 2 givenname: Zewen surname: Zhuang fullname: Zhuang, Zewen – sequence: 3 givenname: Xing surname: Cao fullname: Cao, Xing – sequence: 4 givenname: Chao surname: Zhang fullname: Zhang, Chao – sequence: 5 givenname: Qing surname: Peng fullname: Peng, Qing – sequence: 6 givenname: Chen surname: Chen fullname: Chen, Chen – sequence: 7 givenname: Yadong surname: Li fullname: Li, Yadong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32133461$$D View this record in MEDLINE/PubMed |
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| Notes | Di Zhao is currently a postdoctoral fellow under the supervision of Prof. Yadong Li at the Department of Chemistry, Tsinghua University. She received her BS degree from the College of Chemistry and Pharmaceutical Sciences, Qingdao Agricultural University in 2011 and her PhD degree from the School of Chemistry and Chemical Engineering in 2017, Beijing Institute of Technology. Her research interests include the design, synthesis and characterization of nanostructured materials and their applications in energy storage and conversion. Yadong Li received his BS degree from the Department of Chemistry, Anhui Normal University in 1986 and his PhD degree from the Department of Chemistry, University of Science and Technology of China in 1998, with Prof. Yitai Qian. He joined the faculty of the Department of Chemistry, Tsinghua University in 1999 as a full professor. His research interests are focused on the synthesis, assembly, structure, and application exploration of nanomaterials. Chen Chen received his BS degree from the Department of Chemistry, Beijing Institute of Technology in 2006, and his PhD degree from the Department of Chemistry, Tsinghua University in 2011 under the direction of Prof. Yadong Li. After postdoctoral work at Lawrence Berkeley National Laboratory with Prof. Peidong Yang, he joined the Department of Chemistry at Tsinghua University as an associate professor in 2015. His research interests are focused on nanomaterials and catalysis. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 ObjectType-Review-3 content type line 23 |
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| Title | Atomic site electrocatalysts for water splitting, oxygen reduction and selective oxidation |
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