Room temperature deposition of homogeneous, highly transparent and conductive Al-doped ZnO films by reactive high power impulse magnetron sputtering
Aluminum doped zinc oxide (AZO) films have been deposited using reactive high power impulse magnetron sputtering (HiPIMS) and reactive direct current (DC) magnetron sputtering from an alloyed target without thermal assistance. These films have been compared in terms of their optical, electrical and...
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Published in | Solar energy materials and solar cells Vol. 157; pp. 742 - 749 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
01.12.2016
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Abstract | Aluminum doped zinc oxide (AZO) films have been deposited using reactive high power impulse magnetron sputtering (HiPIMS) and reactive direct current (DC) magnetron sputtering from an alloyed target without thermal assistance. These films have been compared in terms of their optical, electrical and structural properties. While both DC and HiPIMS deposited films show comparable transmittance, their electrical properties are significantly improved by the HiPIMS process. The HiPIMS deposited films show a low resistivity down to the order of 10−4Ωcm with a good homogeneity across the substrate, making them potential candidates for electrodes in solar cells. The density of electrons reached up to 11×1020cm−3, making ionized impurities the main scattering defects. This improvement of the film properties can be related to the specific plasma/target interactions in a HiPIMS discharge. This allows the process to take place in the transition mode and to deposit highly conductive, transparent AZO films on large surfaces at low temperature. While the overall oxygen content is above that of stoichiometric ZnO, higher localization of oxygen is found at the interfaces between crystalline domains with substoichiometric composition.
•Transparent Al-doped ZnO films of high and homogeneous conductivity have been synthesized at room temperature.•The properties of the films were optimized by using a reactive High Power Impulse Magnetron Sputtering (HiPIMS).•The improved properties have been related to the high instantaneous sputtering rate in HiPIMS. |
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AbstractList | Aluminum doped zinc oxide (AZO) films have been deposited using reactive high power impulse magnetron sputtering (HiPIMS) and reactive direct current (DC) magnetron sputtering from an alloyed target without thermal assistance. These films have been compared in terms of their optical, electrical and structural properties. While both DC and HiPIMS deposited films show comparable transmittance, their electrical properties are significantly improved by the HiPIMS process. The HiPIMS deposited films show a low resistivity down to the order of 10(-4) Omega cm with a good homogeneity across the substrate, making them potential candidates for electrodes in solar cells. The density of electrons reached up to 11 x 10(20) cm(-3), making ionized impurities the main scattering defects. This improvement of the film properties can be related to the specific plasma/target interactions in a HiPIMS discharge. This allows the process to take place in the transition mode and to deposit highly conductive, transparent AZO films on large surfaces at low temperature. While the overall oxygen content is above that of stoichiometric ZnO, higher localization of oxygen is found at the interfaces between crystalline domains with substoichiometric composition. (C) 2016 Elsevier B.V. All rights reserved. Aluminum doped zinc oxide (AZO) films have been deposited using reactive high power impulse magnetron sputtering (HiPIMS) and reactive direct current (DC) magnetron sputtering from an alloyed target without thermal assistance. These films have been compared in terms of their optical, electrical and structural properties. While both DC and HiPIMS deposited films show comparable transmittance, their electrical properties are significantly improved by the HiPIMS process. The HiPIMS deposited films show a low resistivity down to the order of 10−4Ωcm with a good homogeneity across the substrate, making them potential candidates for electrodes in solar cells. The density of electrons reached up to 11×1020cm−3, making ionized impurities the main scattering defects. This improvement of the film properties can be related to the specific plasma/target interactions in a HiPIMS discharge. This allows the process to take place in the transition mode and to deposit highly conductive, transparent AZO films on large surfaces at low temperature. While the overall oxygen content is above that of stoichiometric ZnO, higher localization of oxygen is found at the interfaces between crystalline domains with substoichiometric composition. •Transparent Al-doped ZnO films of high and homogeneous conductivity have been synthesized at room temperature.•The properties of the films were optimized by using a reactive High Power Impulse Magnetron Sputtering (HiPIMS).•The improved properties have been related to the high instantaneous sputtering rate in HiPIMS. |
Author | Helmersson, Ulf Ghanbaja, Jaafar Horwat, David Mickan, Martin Rinnert, Hervé Muller, Dominique |
Author_xml | – sequence: 1 givenname: Martin surname: Mickan fullname: Mickan, Martin organization: Université de Lorraine, Institut Jean Lamour, UMR7198, Nancy F-54011, France – sequence: 2 givenname: Ulf surname: Helmersson fullname: Helmersson, Ulf organization: Plasma & Coatings Physics Division, IFM-Material Physics, Linköping University, SE-581 83 Linköping, Sweden – sequence: 3 givenname: Hervé surname: Rinnert fullname: Rinnert, Hervé organization: Université de Lorraine, Institut Jean Lamour, UMR7198, Nancy F-54011, France – sequence: 4 givenname: Jaafar surname: Ghanbaja fullname: Ghanbaja, Jaafar organization: Université de Lorraine, Institut Jean Lamour, UMR7198, Nancy F-54011, France – sequence: 5 givenname: Dominique surname: Muller fullname: Muller, Dominique organization: Laboratoire ICube, Université de Strasbourg, CNRS UMR 7357, 67037 Strasbourg Cedex 2, France – sequence: 6 givenname: David surname: Horwat fullname: Horwat, David email: david.horwat@univ-lorraine.fr organization: Université de Lorraine, Institut Jean Lamour, UMR7198, Nancy F-54011, France |
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Snippet | Aluminum doped zinc oxide (AZO) films have been deposited using reactive high power impulse magnetron sputtering (HiPIMS) and reactive direct current (DC)... |
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SubjectTerms | AZO Electronic properties HiPIMS Thin films Transparent conducting oxide |
Title | Room temperature deposition of homogeneous, highly transparent and conductive Al-doped ZnO films by reactive high power impulse magnetron sputtering |
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