Harmonic spin–orbit angular momentum cascade in nonlinear optical crystals
Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical processes in spatially engineered optical materials 1 . Re-examining the basics of nonlinear optics of homogeneous crystals under circularly polar...
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| Published in | Nature photonics Vol. 14; no. 11; pp. 658 - 662 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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London
Nature Publishing Group UK
01.11.2020
Nature Publishing Group |
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| Online Access | Get full text |
| ISSN | 1749-4885 1749-4893 |
| DOI | 10.1038/s41566-020-0691-0 |
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| Abstract | Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical processes in spatially engineered optical materials
1
. Re-examining the basics of nonlinear optics of homogeneous crystals under circularly polarized light
2
,
3
, we report experiments on the enrichment of the spin–orbit angular momentum spectrum of paraxial light. The demonstration is made within the framework of second-harmonic generation using a crystal with three-fold rotational symmetry. Four spin–orbit optical states for the second harmonic field are predicted from a single fundamental state owing to the interplay between linear spin–orbit coupling and nonlinear wave mixing; three of these states are experimentally verified. Besides representing a spin-controlled nonlinear route to orbital angular multiplexing
4
, modal vortex light sources
5
,
6
, high-dimensional parametric processes
7
and multi-state optical magnetization
8
, our findings suggest that the fundamentals of nonlinear optics are worth revisiting through the prism of the spin–orbit interaction of light.
An experimental study of the second-harmonic-generation process in a beta barium borate crystal shows that homogeneous optical crystals can exhibit the rich physics of the spin–orbit angular momentum cascade in the nonlinear optical regime. |
|---|---|
| AbstractList | Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical processes in spatially engineered optical materials1. Re-examining the basics of nonlinear optics of homogeneous crystals under circularly polarized light2,3, we report experiments on the enrichment of the spin–orbit angular momentum spectrum of paraxial light. The demonstration is made within the framework of second-harmonic generation using a crystal with three-fold rotational symmetry. Four spin–orbit optical states for the second harmonic field are predicted from a single fundamental state owing to the interplay between linear spin–orbit coupling and nonlinear wave mixing; three of these states are experimentally verified. Besides representing a spin-controlled nonlinear route to orbital angular multiplexing4, modal vortex light sources5,6, high-dimensional parametric processes7 and multi-state optical magnetization8, our findings suggest that the fundamentals of nonlinear optics are worth revisiting through the prism of the spin–orbit interaction of light.An experimental study of the second-harmonic-generation process in a beta barium borate crystal shows that homogeneous optical crystals can exhibit the rich physics of the spin–orbit angular momentum cascade in the nonlinear optical regime. Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical processes in spatially engineered optical materials 1 . Re-examining the basics of nonlinear optics of homogeneous crystals under circularly polarized light 2 , 3 , we report experiments on the enrichment of the spin–orbit angular momentum spectrum of paraxial light. The demonstration is made within the framework of second-harmonic generation using a crystal with three-fold rotational symmetry. Four spin–orbit optical states for the second harmonic field are predicted from a single fundamental state owing to the interplay between linear spin–orbit coupling and nonlinear wave mixing; three of these states are experimentally verified. Besides representing a spin-controlled nonlinear route to orbital angular multiplexing 4 , modal vortex light sources 5 , 6 , high-dimensional parametric processes 7 and multi-state optical magnetization 8 , our findings suggest that the fundamentals of nonlinear optics are worth revisiting through the prism of the spin–orbit interaction of light. An experimental study of the second-harmonic-generation process in a beta barium borate crystal shows that homogeneous optical crystals can exhibit the rich physics of the spin–orbit angular momentum cascade in the nonlinear optical regime. Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical processes in spatially engineered optical materials1. Re-examining the basics of nonlinear optics of homogeneous crystals under circularly polarized light2,3, we report experiments on the enrichment of the spin–orbit angular momentum spectrum of paraxial light. The demonstration is made within the framework of second-harmonic generation using a crystal with three-fold rotational symmetry. Four spin–orbit optical states for the second harmonic field are predicted from a single fundamental state owing to the interplay between linear spin–orbit coupling and nonlinear wave mixing; three of these states are experimentally verified. Besides representing a spin-controlled nonlinear route to orbital angular multiplexing4, modal vortex light sources5,6, high-dimensional parametric processes7 and multi-state optical magnetization8, our findings suggest that the fundamentals of nonlinear optics are worth revisiting through the prism of the spin–orbit interaction of light |
| Author | Brasselet, Etienne Zhang, Xuecai Deng, Junhong Tang, Yutao Li, Kingfai Li, Guixin |
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| Snippet | Optical angular momentum-based photonic technologies demonstrate the key role of the optical spin–orbit interaction that usually refers to linear optical... |
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| SubjectTerms | 639/624/400/385 639/766/400/385 Angular momentum Applied and Technical Physics Barium BBO crystals Circular polarization Crystals Letter Nonlinear control Nonlinear optics Optics Photonic crystals Physics Physics and Astronomy Quantum Physics Second harmonic generation Spin-orbit interactions |
| Title | Harmonic spin–orbit angular momentum cascade in nonlinear optical crystals |
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