Modeling and simulation of catalytic partial oxidation of methane to synthesis gas by using a plasma-assisted gliding arc reactor

In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc) reactor is presented. A 2D heterogeneous plug-flow model with radial dispersion and no gradients inside the catalyst pellet are used, including...

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Published inFuel processing technology Vol. 101; pp. 44 - 57
Main Authors Rafiq, M.H., Jakobsen, H.A., Hustad, J.E.
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 01.09.2012
Elsevier
Subjects
Applied sciences
catalysts
Catalytic partial oxidation
Energy
energy density
Energy. Thermal use of fuels
equations
Exact sciences and technology
Fuels
GlidArc reactor
hydrogen
Methane
oxidation
oxygen
Reactor modeling
simulation models
Synthesis gas
temperature
yields
Methane
GlidArc reactor
Reactor modeling
Synthesis gas
Catalytic partial oxidation
Transport equation
Plasma arc
Differential equation
Gas solid reaction
Density
Modeling
Partial oxidation
Non linear equation
Numerical analysis
Simulation
Catalyst
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Abstract In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc) reactor is presented. A 2D heterogeneous plug-flow model with radial dispersion and no gradients inside the catalyst pellet are used, including the transport equations for the gas and solid phase and reaction rate equations. The governing equations of this model formed a set of stationary differential algebraic equations coupled with the non-linear algebraic equations, and were solved numerically using in-house MATLAB® code. Model results of CPO of methane were compared to previous experimental data with the GlidArc reactor found in the literature. A close match between the calculated and experimental results for temperature, reactant (CH4 and O2) conversion, H2 and CO yields and species mole-fraction was obtained. The developed model was extended to predict and quantify the influence of the gas hour space velocity (GHSV) as well as determine the influence of the reactor energy density (RED), the O2/CH4 molar ratio and the O2/N2 molar ratio. The predicted behaviors for the species mole-fraction, reactants conversion, H2 and CO yields and temperature along the length of the reactor have been analyzed. ► A 2D heterogeneous model for plasma-assisted CPO of methane to syngas is developed. ► The reactor model includes transport equations and main global surface reactions. ► A close match between the calculated and experimental results is obtained. ► Parametric sensitivity analysis with detailed numerical simulations is also provided.
AbstractList In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc) reactor is presented. A 2D heterogeneous plug-flow model with radial dispersion and no gradients inside the catalyst pellet are used, including the transport equations for the gas and solid phase and reaction rate equations. The governing equations of this model formed a set of stationary differential algebraic equations coupled with the non-linear algebraic equations, and were solved numerically using in-house MATLAB® code. Model results of CPO of methane were compared to previous experimental data with the GlidArc reactor found in the literature. A close match between the calculated and experimental results for temperature, reactant (CH4 and O2) conversion, H2 and CO yields and species mole-fraction was obtained. The developed model was extended to predict and quantify the influence of the gas hour space velocity (GHSV) as well as determine the influence of the reactor energy density (RED), the O2/CH4 molar ratio and the O2/N2 molar ratio. The predicted behaviors for the species mole-fraction, reactants conversion, H2 and CO yields and temperature along the length of the reactor have been analyzed. ► A 2D heterogeneous model for plasma-assisted CPO of methane to syngas is developed. ► The reactor model includes transport equations and main global surface reactions. ► A close match between the calculated and experimental results is obtained. ► Parametric sensitivity analysis with detailed numerical simulations is also provided.
In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc) reactor is presented. A 2D heterogeneous plug-flow model with radial dispersion and no gradients inside the catalyst pellet are used, including the transport equations for the gas and solid phase and reaction rate equations. The governing equations of this model formed a set of stationary differential algebraic equations coupled with the non-linear algebraic equations, and were solved numerically using in-house MATLABARG code. Model results of CPO of methane were compared to previous experimental data with the GlidArc reactor found in the literature. A close match between the calculated and experimental results for temperature, reactant (CH4 and O2) conversion, H2 and CO yields and species mole-fraction was obtained. The developed model was extended to predict and quantify the influence of the gas hour space velocity (GHSV) as well as determine the influence of the reactor energy density (RED), the O2/CH4 molar ratio and the O2/N2 molar ratio. The predicted behaviors for the species mole-fraction, reactants conversion, H2 and CO yields and temperature along the length of the reactor have been analyzed.
In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc) reactor is presented. A 2D heterogeneous plug-flow model with radial dispersion and no gradients inside the catalyst pellet are used, including the transport equations for the gas and solid phase and reaction rate equations. The governing equations of this model formed a set of stationary differential algebraic equations coupled with the non-linear algebraic equations, and were solved numerically using in-house MATLAB® code. Model results of CPO of methane were compared to previous experimental data with the GlidArc reactor found in the literature. A close match between the calculated and experimental results for temperature, reactant (CH₄ and O₂) conversion, H₂ and CO yields and species mole-fraction was obtained. The developed model was extended to predict and quantify the influence of the gas hour space velocity (GHSV) as well as determine the influence of the reactor energy density (RED), the O₂/CH₄ molar ratio and the O₂/N₂ molar ratio. The predicted behaviors for the species mole-fraction, reactants conversion, H₂ and CO yields and temperature along the length of the reactor have been analyzed.
Author Jakobsen, H.A.
Hustad, J.E.
Rafiq, M.H.
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Keywords Methane
GlidArc reactor
Reactor modeling
Synthesis gas
Catalytic partial oxidation
Transport equation
Plasma arc
Differential equation
Gas solid reaction
Density
Modeling
Partial oxidation
Non linear equation
Numerical analysis
Simulation
Catalyst
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Snippet In the present study, a numerical investigation of the catalytic partial oxidation (CPO) of methane to synthesis gas (syngas) using a gliding arc (GlidArc)...
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SubjectTerms Applied sciences
catalysts
Catalytic partial oxidation
Energy
energy density
Energy. Thermal use of fuels
equations
Exact sciences and technology
Fuels
GlidArc reactor
hydrogen
Methane
oxidation
oxygen
Reactor modeling
simulation models
Synthesis gas
temperature
yields
Title Modeling and simulation of catalytic partial oxidation of methane to synthesis gas by using a plasma-assisted gliding arc reactor
URI https://dx.doi.org/10.1016/j.fuproc.2011.12.044
https://search.proquest.com/docview/1034820149
Volume 101
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