MOF-derived carbon coating on self-supported ZnCo2O4–ZnO nanorod arrays as high-performance anode for lithium-ion batteries
The C–ZnCo 2 O 4 –ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo 2 O 4 –ZnO NRAs, are rational designed and synthesized via a facile template-based solution route on Ti foil and used as high-performance anode for lithium-ion batteries (LIBs). The uniform coated MOF-de...
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| Published in | Journal of materials science Vol. 52; no. 13; pp. 7768 - 7780 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.07.2017
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The C–ZnCo
2
O
4
–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo
2
O
4
–ZnO NRAs, are rational designed and synthesized via a facile template-based solution route on Ti foil and used as high-performance anode for lithium-ion batteries (LIBs). The uniform coated MOF-derived carbon layers on the ZnCo
2
O
4
–ZnO nanorods surface can serve as a conductive substrate as well as buffer layer to restrain volume expansion during charge–discharge process. When tested as anodes for LIBs, the C–ZnCo
2
O
4
–ZnO NRAs show high reversible capacity of 1318 mA h g
−1
at 0.2 A g
−1
after 150 charge–discharge cycles. Furthermore, C–ZnCo
2
O
4
–ZnO NRAs also exhibit brilliant rate performance of 886.2, 812.8, 732.2 and 580.6 mA h g
−1
at 0.5, 1, 2 and 5 A g
−1
, respectively. The outstanding lithium storage performance of C–ZnCo
2
O
4
–ZnO NRAs could be ascribed to the stimulated kinetics of ion diffusion and electron transport originated from the shortened lithium-ion diffusion pathway and improved electronic conductivity benefit from uniformly coating MOF-derived carbon. |
|---|---|
| AbstractList | The C–ZnCo₂O₄–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo₂O₄–ZnO NRAs, are rational designed and synthesized via a facile template-based solution route on Ti foil and used as high-performance anode for lithium-ion batteries (LIBs). The uniform coated MOF-derived carbon layers on the ZnCo₂O₄–ZnO nanorods surface can serve as a conductive substrate as well as buffer layer to restrain volume expansion during charge–discharge process. When tested as anodes for LIBs, the C–ZnCo₂O₄–ZnO NRAs show high reversible capacity of 1318 mA h g⁻¹ at 0.2 A g⁻¹ after 150 charge–discharge cycles. Furthermore, C–ZnCo₂O₄–ZnO NRAs also exhibit brilliant rate performance of 886.2, 812.8, 732.2 and 580.6 mA h g⁻¹ at 0.5, 1, 2 and 5 A g⁻¹, respectively. The outstanding lithium storage performance of C–ZnCo₂O₄–ZnO NRAs could be ascribed to the stimulated kinetics of ion diffusion and electron transport originated from the shortened lithium-ion diffusion pathway and improved electronic conductivity benefit from uniformly coating MOF-derived carbon. The C–ZnCo 2 O 4 –ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo 2 O 4 –ZnO NRAs, are rational designed and synthesized via a facile template-based solution route on Ti foil and used as high-performance anode for lithium-ion batteries (LIBs). The uniform coated MOF-derived carbon layers on the ZnCo 2 O 4 –ZnO nanorods surface can serve as a conductive substrate as well as buffer layer to restrain volume expansion during charge–discharge process. When tested as anodes for LIBs, the C–ZnCo 2 O 4 –ZnO NRAs show high reversible capacity of 1318 mA h g −1 at 0.2 A g −1 after 150 charge–discharge cycles. Furthermore, C–ZnCo 2 O 4 –ZnO NRAs also exhibit brilliant rate performance of 886.2, 812.8, 732.2 and 580.6 mA h g −1 at 0.5, 1, 2 and 5 A g −1 , respectively. The outstanding lithium storage performance of C–ZnCo 2 O 4 –ZnO NRAs could be ascribed to the stimulated kinetics of ion diffusion and electron transport originated from the shortened lithium-ion diffusion pathway and improved electronic conductivity benefit from uniformly coating MOF-derived carbon. The C–ZnCo2O4–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo2O4–ZnO NRAs, are rational designed and synthesized via a facile template-based solution route on Ti foil and used as high-performance anode for lithium-ion batteries (LIBs). The uniform coated MOF-derived carbon layers on the ZnCo2O4–ZnO nanorods surface can serve as a conductive substrate as well as buffer layer to restrain volume expansion during charge–discharge process. When tested as anodes for LIBs, the C–ZnCo2O4–ZnO NRAs show high reversible capacity of 1318 mA h g−1 at 0.2 A g−1 after 150 charge–discharge cycles. Furthermore, C–ZnCo2O4–ZnO NRAs also exhibit brilliant rate performance of 886.2, 812.8, 732.2 and 580.6 mA h g−1 at 0.5, 1, 2 and 5 A g−1, respectively. The outstanding lithium storage performance of C–ZnCo2O4–ZnO NRAs could be ascribed to the stimulated kinetics of ion diffusion and electron transport originated from the shortened lithium-ion diffusion pathway and improved electronic conductivity benefit from uniformly coating MOF-derived carbon. |
| Author | Gan, Qingmeng He, Zhen Zhao, Kuangmin Liu, Suqin |
| Author_xml | – sequence: 1 givenname: Qingmeng surname: Gan fullname: Gan, Qingmeng organization: College of Chemistry and Chemical Engineering, Central South University – sequence: 2 givenname: Kuangmin surname: Zhao fullname: Zhao, Kuangmin organization: College of Chemistry and Chemical Engineering, Central South University – sequence: 3 givenname: Suqin surname: Liu fullname: Liu, Suqin email: sqliu2003@126.com organization: College of Chemistry and Chemical Engineering, Central South University – sequence: 4 givenname: Zhen surname: He fullname: He, Zhen email: zhenhe@csu.edu.cn organization: College of Chemistry and Chemical Engineering, Central South University |
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| Snippet | The C–ZnCo
2
O
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–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo
2
O
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–ZnO NRAs, are rational designed and synthesized via a... The C–ZnCo2O4–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo2O4–ZnO NRAs, are rational designed and synthesized via a facile... The C–ZnCo₂O₄–ZnO nanorod arrays (NRAs), which consist of MOF-derived carbon coating on ZnCo₂O₄–ZnO NRAs, are rational designed and synthesized via a facile... |
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| SubjectTerms | Anodes Arrays Buffer layers Carbon Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics coatings Crystallography and Scattering Methods Diffusion coating Discharge electron transfer Electron transport Energy Materials foil Foils Ion diffusion Lithium lithium batteries Lithium-ion batteries Materials Science Nanorods Polymer Sciences Rechargeable batteries Solid Mechanics Substrates Zinc oxide |
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