Lithiophilic-lithiophobic gradient interfacial layer for a highly stable lithium metal anode
The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic–lithiophobic gradient interfacial layer strategy in which the bott...
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| Published in | Nature communications Vol. 9; no. 1; pp. 3729 - 11 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
13.09.2018
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic–lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm
2
pouch cell and lithium–sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic–lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries.
Lithium metal batteries suffer from the dendrite growth upon electrochemical cycling. Here the authors introduce a lithiophilic-lithiophobic gradient interfacial ZnO/CNT layer, which facilitates the formation of a stable solid electrolyte interphase, and suppresses the growth of lithium dendrite. |
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| AbstractList | The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic–lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm
2
pouch cell and lithium–sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic–lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries. The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic–lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm 2 pouch cell and lithium–sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic–lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries. Lithium metal batteries suffer from the dendrite growth upon electrochemical cycling. Here the authors introduce a lithiophilic-lithiophobic gradient interfacial ZnO/CNT layer, which facilitates the formation of a stable solid electrolyte interphase, and suppresses the growth of lithium dendrite. Lithium metal batteries suffer from the dendrite growth upon electrochemical cycling. Here the authors introduce a lithiophilic-lithiophobic gradient interfacial ZnO/CNT layer, which facilitates the formation of a stable solid electrolyte interphase, and suppresses the growth of lithium dendrite. The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic-lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm pouch cell and lithium-sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic-lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries. The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic–lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm2 pouch cell and lithium–sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic–lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries. The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic-lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm2 pouch cell and lithium-sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic-lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries.The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for high-energy density batteries. Here, we demonstrate a promising lithiophilic-lithiophobic gradient interfacial layer strategy in which the bottom lithiophilic zinc oxide/carbon nanotube sublayer tightly anchors the whole layer onto the lithium foil, facilitating the formation of a stable solid electrolyte interphase, and prevents the formation of an intermediate mossy lithium corrosion layer. Together with the top lithiophobic carbon nanotube sublayer, this gradient interfacial layer can effectively suppress dendrite growth and ensure ultralong-term stable lithium stripping/plating. This strategy is further demonstrated to provide substantially improved cycle performance in copper current collector, 10 cm2 pouch cell and lithium-sulfur batteries, which, coupled with a simple fabrication process and wide applicability in various materials for lithium-metal protection, makes the lithiophilic-lithiophobic gradient interfacial layer a favored strategy for next-generation lithium-metal batteries. |
| ArticleNumber | 3729 |
| Author | Zhang, Huimin Li, Meng Qiu, Jingyi Lu, Lin Xiang, Yu Zhang, Wenfeng Zhang, Hao Liao, Xiaobin Zhu, Xiayu Mai, Liqiang Guan, Yuepeng Cao, Gaoping Yang, Yusheng Ming, Hai Zhao, Yan Huang, Yaqin |
| Author_xml | – sequence: 1 givenname: Huimin surname: Zhang fullname: Zhang, Huimin organization: Research Institute of Chemical Defense, Beijing Institute of Technology – sequence: 2 givenname: Xiaobin surname: Liao fullname: Liao, Xiaobin organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 3 givenname: Yuepeng surname: Guan fullname: Guan, Yuepeng organization: State Key Laboratory of Chemical Resource Engineering, The Key Laboratory of Beijing City on Preparation and Processing of Novel Polymer Materials, Beijing University of Chemical Technology – sequence: 4 givenname: Yu surname: Xiang fullname: Xiang, Yu organization: Research Institute of Chemical Defense – sequence: 5 givenname: Meng surname: Li fullname: Li, Meng organization: Research Institute of Chemical Defense – sequence: 6 givenname: Wenfeng surname: Zhang fullname: Zhang, Wenfeng organization: Research Institute of Chemical Defense – sequence: 7 givenname: Xiayu surname: Zhu fullname: Zhu, Xiayu organization: Research Institute of Chemical Defense – sequence: 8 givenname: Hai surname: Ming fullname: Ming, Hai organization: Research Institute of Chemical Defense – sequence: 9 givenname: Lin surname: Lu fullname: Lu, Lin organization: Research Institute of Chemical Defense – sequence: 10 givenname: Jingyi surname: Qiu fullname: Qiu, Jingyi organization: Research Institute of Chemical Defense – sequence: 11 givenname: Yaqin surname: Huang fullname: Huang, Yaqin organization: State Key Laboratory of Chemical Resource Engineering, The Key Laboratory of Beijing City on Preparation and Processing of Novel Polymer Materials, Beijing University of Chemical Technology – sequence: 12 givenname: Gaoping surname: Cao fullname: Cao, Gaoping organization: Research Institute of Chemical Defense – sequence: 13 givenname: Yusheng surname: Yang fullname: Yang, Yusheng organization: Research Institute of Chemical Defense – sequence: 14 givenname: Liqiang orcidid: 0000-0003-4259-7725 surname: Mai fullname: Mai, Liqiang email: mlq518@whut.edu.cn organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology – sequence: 15 givenname: Yan orcidid: 0000-0002-1234-4455 surname: Zhao fullname: Zhao, Yan email: yan2000@whut.edu.cn organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 16 givenname: Hao surname: Zhang fullname: Zhang, Hao email: dr.h.zhang@hotmail.com organization: Research Institute of Chemical Defense |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30213936$$D View this record in MEDLINE/PubMed |
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| Snippet | The long-standing issue of lithium dendrite growth during repeated deposition or dissolution processes hinders the practical use of lithium-metal anodes for... Lithium metal batteries suffer from the dendrite growth upon electrochemical cycling. Here the authors introduce a lithiophilic-lithiophobic gradient... |
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| SubjectTerms | 147/135 639/4077 639/925 Anodes Anodic dissolution Carbon nanotubes Corrosion prevention Dendrites Dendritic structure Dissolution Fabrication Flux density Foils Humanities and Social Sciences Lithium Lithium batteries Metals multidisciplinary Nanotubes Science Science (multidisciplinary) Solid electrolytes Strategy Sulfur Zinc oxide |
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| Title | Lithiophilic-lithiophobic gradient interfacial layer for a highly stable lithium metal anode |
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