In situ investigation of particle clustering dynamics in colloidal assemblies using fluorescence microscopy
Herein, particle clustering dynamics and thermofluidic transprot in colloidal assemblies are experimentally examined using a novel fluorescence technique with the aim to investigate colloidal physics that decide cracking mechanics during self-assembly. The results show that grain boundaries are dete...
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| Published in | Journal of colloid and interface science Vol. 576; pp. 195 - 202 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
15.09.2020
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0021-9797 1095-7103 1095-7103 |
| DOI | 10.1016/j.jcis.2020.04.054 |
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| Abstract | Herein, particle clustering dynamics and thermofluidic transprot in colloidal assemblies are experimentally examined using a novel fluorescence technique with the aim to investigate colloidal physics that decide cracking mechanics during self-assembly. The results show that grain boundaries are determined by dynamic structuring regimes governed by the film’s saturation level.
[Display omitted]
Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly, packed particles are subject to solvent-evaporation induced dynamic structuring phases, which leads to microscale defects called the grain boundaries. While it is imperative to precisely control detailed grain boundaries to fabricate well-defined self-assembled crystals, the understanding of the colloidal physics that govern grain boundaries remains a challenge due to limited resolutions of current visualization approaches. In this work, we experimentally report in situ particle clustering dynamics during evaporative colloidal assembly by studying a novel microscale laser induced fluorescence technique. The fluorescence microscopy measures the saturation levels with high fidelity to identify distinct colloidal structuring regimes during self-assembly as well as cracking mechanics. The techniques discussed in this work not only enables unprecedented levels of colloidal self-assembly analysis but also have potential to be used for various sensing applications with microscopic resolutions. |
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| AbstractList | Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly, packed particles are subject to solvent-evaporation induced dynamic structuring phases, which leads to microscale defects called the grain boundaries. While it is imperative to precisely control detailed grain boundaries to fabricate well-defined self-assembled crystals, the understanding of the colloidal physics that govern grain boundaries remains a challenge due to limited resolutions of current visualization approaches. In this work, we experimentally report in situ particle clustering dynamics during evaporative colloidal assembly by studying a novel microscale laser induced fluorescence technique. The fluorescence microscopy measures the saturation levels with high fidelity to identify distinct colloidal structuring regimes during self-assembly as well as cracking mechanics. The techniques discussed in this work not only enables unprecedented levels of colloidal self-assembly analysis but also have potential to be used for various sensing applications with microscopic resolutions.Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly, packed particles are subject to solvent-evaporation induced dynamic structuring phases, which leads to microscale defects called the grain boundaries. While it is imperative to precisely control detailed grain boundaries to fabricate well-defined self-assembled crystals, the understanding of the colloidal physics that govern grain boundaries remains a challenge due to limited resolutions of current visualization approaches. In this work, we experimentally report in situ particle clustering dynamics during evaporative colloidal assembly by studying a novel microscale laser induced fluorescence technique. The fluorescence microscopy measures the saturation levels with high fidelity to identify distinct colloidal structuring regimes during self-assembly as well as cracking mechanics. The techniques discussed in this work not only enables unprecedented levels of colloidal self-assembly analysis but also have potential to be used for various sensing applications with microscopic resolutions. Herein, particle clustering dynamics and thermofluidic transprot in colloidal assemblies are experimentally examined using a novel fluorescence technique with the aim to investigate colloidal physics that decide cracking mechanics during self-assembly. The results show that grain boundaries are determined by dynamic structuring regimes governed by the film’s saturation level. [Display omitted] Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly, packed particles are subject to solvent-evaporation induced dynamic structuring phases, which leads to microscale defects called the grain boundaries. While it is imperative to precisely control detailed grain boundaries to fabricate well-defined self-assembled crystals, the understanding of the colloidal physics that govern grain boundaries remains a challenge due to limited resolutions of current visualization approaches. In this work, we experimentally report in situ particle clustering dynamics during evaporative colloidal assembly by studying a novel microscale laser induced fluorescence technique. The fluorescence microscopy measures the saturation levels with high fidelity to identify distinct colloidal structuring regimes during self-assembly as well as cracking mechanics. The techniques discussed in this work not only enables unprecedented levels of colloidal self-assembly analysis but also have potential to be used for various sensing applications with microscopic resolutions. Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly, packed particles are subject to solvent-evaporation induced dynamic structuring phases, which leads to microscale defects called the grain boundaries. While it is imperative to precisely control detailed grain boundaries to fabricate well-defined self-assembled crystals, the understanding of the colloidal physics that govern grain boundaries remains a challenge due to limited resolutions of current visualization approaches. In this work, we experimentally report in situ particle clustering dynamics during evaporative colloidal assembly by studying a novel microscale laser induced fluorescence technique. The fluorescence microscopy measures the saturation levels with high fidelity to identify distinct colloidal structuring regimes during self-assembly as well as cracking mechanics. The techniques discussed in this work not only enables unprecedented levels of colloidal self-assembly analysis but also have potential to be used for various sensing applications with microscopic resolutions. |
| Author | Won, Yoonjin Suh, Youngjoon Gowda, Hamsa |
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| Keywords | In situ measurements Self-assembly Saturation level Laser induced fluorescence Grain boundary |
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| Snippet | Herein, particle clustering dynamics and thermofluidic transprot in colloidal assemblies are experimentally examined using a novel fluorescence technique with... Colloidal self-assembly is a process in which dispersed matter spontaneously form higher-order structures without external intervention. During self-assembly,... |
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| SubjectTerms | cracking crystals fluorescence fluorescence microscopy Grain boundary In situ measurements Laser induced fluorescence mechanics Saturation level Self-assembly |
| Title | In situ investigation of particle clustering dynamics in colloidal assemblies using fluorescence microscopy |
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