2D-2D growth of NiFe LDH nanoflakes on montmorillonite for cationic and anionic dye adsorption performance

[Display omitted] NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of m...

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Published in	Journal of colloid and interface science Vol. 540; pp. 398 - 409
Main Authors	Jiang, De Bin, Jing, Chuan, Yuan, Yunsong, Feng, Li, Liu, Xiaoying, Dong, Fan, Dong, Biqing, Zhang, Yu Xin
Format	Journal Article
Language	English
Published	United States Elsevier Inc 22.03.2019
Subjects	Adsorbent adsorbents adsorption differential thermal analysis Fourier transform infrared spectroscopy hot water treatment hydroxides Methyl orange Methylene blue Montmorillonite NiFe LDH scanning electron microscopy Sewage disposal surface area thermogravimetry wastewater X-ray diffraction X-ray photoelectron spectroscopy Sewage disposal Montmorillonite Adsorbent Methyl orange NiFe LDH Methylene blue
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Abstract	[Display omitted] NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni2+/Fe3+ could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g−1 and 99.18 mg g−1, respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification.
AbstractList	NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni /Fe could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g and 99.18 mg g , respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification. NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni2+/Fe3+ could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g−1 and 99.18 mg g−1, respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification. NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni2+/Fe3+ could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g-1 and 99.18 mg g-1, respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification.NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni2+/Fe3+ could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g-1 and 99.18 mg g-1, respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification. [Display omitted] NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth MMT@NiFe LDH was utilized as an effective adsorbent for removal of anionic dye of methyl orange (MO) and cationic dye of methylene blue (MB). The mole ratio of Ni2+/Fe3+ could quite influence the interlayer spacing, surface area per unit charge and the ultrathin hexagonal laminated morphology of NiFe LDH decorated on the surface of MMT. Various characterization techniques were conducted to identify it, such as XRD, FT-IR, TG-DTA, BET, XPS and SEM. Under the optimal conditions, the Langmuir-fitted maximum adsorption capacities for MO and MB are 108.80 mg g−1 and 99.18 mg g−1, respectively. Adsorption kinetics for MO and MB are both verified to be fit in with pseudo-second-order model. This work suggests a facile pathway to synthesize desirable bifunctional adsorbent for cationic and anionic dyes, which provides the potential application for the actual wastewater purification.
Author	Liu, Xiaoying Feng, Li Dong, Fan Jiang, De Bin Yuan, Yunsong Dong, Biqing Jing, Chuan Zhang, Yu Xin
Author_xml	– sequence: 1 givenname: De Bin surname: Jiang fullname: Jiang, De Bin organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 2 givenname: Chuan surname: Jing fullname: Jing, Chuan organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 3 givenname: Yunsong surname: Yuan fullname: Yuan, Yunsong email: yuan_ys@cqu.edu.cn organization: College of Urban Construction and Environmental Engineering, Chongqing University, Chongqing 400044, China – sequence: 4 givenname: Li surname: Feng fullname: Feng, Li organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China – sequence: 5 givenname: Xiaoying surname: Liu fullname: Liu, Xiaoying organization: Engineering Research Center for Waste Oil Recovery Technology and Equipment of Ministry of Education, College of Environment and Resources, Chongqing Technology and Business University, Chongqing 400067, China – sequence: 6 givenname: Fan surname: Dong fullname: Dong, Fan organization: Research Center for Environmental Science & Technology, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 611731, China – sequence: 7 givenname: Biqing surname: Dong fullname: Dong, Biqing organization: Guangdong Provincial Key Laboratory of Durability for Marine Civil Engineering, Shenzhen University, Shenzhen 518060, China – sequence: 8 givenname: Yu Xin orcidid: 0000-0003-4698-5645 surname: Zhang fullname: Zhang, Yu Xin email: zhangyuxin@cqu.edu.cn organization: State Key Laboratory of Mechanical Transmissions, College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China
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Keywords	Sewage disposal Montmorillonite Adsorbent Methyl orange NiFe LDH Methylene blue
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Snippet	[Display omitted] NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal... NiFe layered double hydroxides nanoflakes decorated montmorillonite (MMT@NiFe LDH) was successfully prepared by a one-pot hydrothermal method. The 2D-2D growth...
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SubjectTerms	Adsorbent adsorbents adsorption differential thermal analysis Fourier transform infrared spectroscopy hot water treatment hydroxides Methyl orange Methylene blue Montmorillonite NiFe LDH scanning electron microscopy Sewage disposal surface area thermogravimetry wastewater X-ray diffraction X-ray photoelectron spectroscopy
Title	2D-2D growth of NiFe LDH nanoflakes on montmorillonite for cationic and anionic dye adsorption performance
URI	https://dx.doi.org/10.1016/j.jcis.2019.01.022 https://www.ncbi.nlm.nih.gov/pubmed/30665166 https://www.proquest.com/docview/2179388923 https://www.proquest.com/docview/2220993860
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