A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture
Most materials for carbon dioxide (CO 2 ) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO 2 . Lin et al . show that a zinc-based metal organic framework material can physisorb CO...
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| Published in | Science (American Association for the Advancement of Science) Vol. 374; no. 6574; pp. 1464 - 1469 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
The American Association for the Advancement of Science
17.12.2021
AAAS |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0036-8075 1095-9203 1095-9203 |
| DOI | 10.1126/science.abi7281 |
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| Abstract | Most materials for carbon dioxide (CO
2
) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO
2
. Lin
et al
. show that a zinc-based metal organic framework material can physisorb CO
2
and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDS
A metal-organic framework captures CO
2
with high capacity and selectivity over steam with only a modest regeneration penalty.
Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO
2
) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO
2
with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO
2
physisorption below 40% relative humidity but also suppression of water sorption by CO
2
, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. |
|---|---|
| AbstractList | Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches.Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. A hydrophobic CO2 physisorbentMost materials for carbon dioxide (CO2) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO2. Lin et al. show that a zinc-based metal organic framework material can physisorb CO2 and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDSMetal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. Most materials for carbon dioxide (CO 2 ) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO 2 . Lin et al . show that a zinc-based metal organic framework material can physisorb CO 2 and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDS A metal-organic framework captures CO 2 with high capacity and selectivity over steam with only a modest regeneration penalty. Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO 2 ) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO 2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO 2 physisorption below 40% relative humidity but also suppression of water sorption by CO 2 , which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. A hydrophobic CO2physisorbent Most materials for carbon dioxide (CO2) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO2. Linet al. show that a zinc-based metal organic framework material can physisorb CO2and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDS Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO ) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO physisorption below 40% relative humidity but also suppression of water sorption by CO , which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches. |
| Author | Sarkar, Partha Taylor, Jared M. Fylstra, Nicholas Woo, Tom K. Dawson, Karl W. Ghaffari-Nik, Omid Burner, Jake Lin, Jian-Bin Akhtar, Farid Vaidhyanathan, Ramanathan Iremonger, Simon S. Hovington, Pierre Durekova, Hana Marx, Stefan Nguyen, Tai T. T. Rajendran, Arvind Shimizu, George K. H. Mah, Roger K. |
| Author_xml | – sequence: 1 givenname: Jian-Bin orcidid: 0000-0002-3117-1959 surname: Lin fullname: Lin, Jian-Bin organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada – sequence: 2 givenname: Tai T. T. orcidid: 0000-0001-5883-5105 surname: Nguyen fullname: Nguyen, Tai T. T. organization: Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada – sequence: 3 givenname: Ramanathan orcidid: 0000-0003-4490-4397 surname: Vaidhyanathan fullname: Vaidhyanathan, Ramanathan organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada., Indian Institute of Science Education and Research, Dr. Homi Bhabha Road, Pashan, Pune, Maharashtra, 411008, India – sequence: 4 givenname: Jake orcidid: 0000-0002-2834-5866 surname: Burner fullname: Burner, Jake organization: Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada – sequence: 5 givenname: Jared M. surname: Taylor fullname: Taylor, Jared M. organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada., ZoraMat Solutions Inc., Calgary, Alberta, Canada – sequence: 6 givenname: Hana surname: Durekova fullname: Durekova, Hana organization: Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada – sequence: 7 givenname: Farid orcidid: 0000-0003-4888-6237 surname: Akhtar fullname: Akhtar, Farid organization: Department of Materials Engineering, Luleå University of Technology, Luleå, Sweden – sequence: 8 givenname: Roger K. surname: Mah fullname: Mah, Roger K. organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada., ZoraMat Solutions Inc., Calgary, Alberta, Canada – sequence: 9 givenname: Omid orcidid: 0000-0003-3098-666X surname: Ghaffari-Nik fullname: Ghaffari-Nik, Omid organization: Svante Inc., Vancouver, British Columbia, Canada – sequence: 10 givenname: Stefan orcidid: 0000-0002-3282-9062 surname: Marx fullname: Marx, Stefan organization: BASF SE, Ludwigshafen am Rhein, Germany – sequence: 11 givenname: Nicholas orcidid: 0000-0001-5693-7204 surname: Fylstra fullname: Fylstra, Nicholas organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada – sequence: 12 givenname: Simon S. surname: Iremonger fullname: Iremonger, Simon S. organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada – sequence: 13 givenname: Karl W. surname: Dawson fullname: Dawson, Karl W. organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada – sequence: 14 givenname: Partha orcidid: 0000-0002-8733-3347 surname: Sarkar fullname: Sarkar, Partha organization: Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada – sequence: 15 givenname: Pierre orcidid: 0000-0002-0641-8614 surname: Hovington fullname: Hovington, Pierre organization: Svante Inc., Vancouver, British Columbia, Canada – sequence: 16 givenname: Arvind orcidid: 0000-0003-4367-4892 surname: Rajendran fullname: Rajendran, Arvind organization: Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada – sequence: 17 givenname: Tom K. orcidid: 0000-0003-0073-3901 surname: Woo fullname: Woo, Tom K. organization: Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada – sequence: 18 givenname: George K. H. orcidid: 0000-0003-3697-9890 surname: Shimizu fullname: Shimizu, George K. H. organization: Department of Chemistry, University of Calgary, Calgary, Alberta, Canada., ZoraMat Solutions Inc., Calgary, Alberta, Canada |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34914501$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1982953$$D View this record in Osti.gov https://urn.kb.se/resolve?urn=urn:nbn:se:ltu:diva-88558$$DView record from Swedish Publication Index |
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| Copyright | Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works |
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| DOI | 10.1126/science.abi7281 |
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| Snippet | Most materials for carbon dioxide (CO
2
) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly... Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO ) capture face the challenge of merging efficient capture with economical regeneration... A hydrophobic CO2 physisorbentMost materials for carbon dioxide (CO2) capture of fossil fuel combustion, such as amines, rely on strong chemisorption... Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration... A hydrophobic CO2physisorbent Most materials for carbon dioxide (CO2) capture of fossil fuel combustion, such as amines, rely on strong chemisorption... |
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| SubjectTerms | Amines Binding sites Carbon dioxide Carbon sequestration Chemisorption Composite materials Computer applications Durability Engineering Materials Flue gas Fossil fuels Fuel combustion Humidity Hydrogen bonding Hydrophobicity Materialteknik Metal-organic frameworks Regeneration Relative humidity Science & Technology - Other Topics Sorbents Water Water chemistry Zinc |
| Title | A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture |
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