Stability of molecular radicals in organic non-aqueous redox flow batteries: A mini review

The application of novel organic redox materials is a plausible pathway towards techno-economic energy storage targets due to their low cost and sustainable design. Their operation in non-aqueous redox flow batteries affords researchers the opportunity to innovate, design and optimise these new chem...

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Published inElectrochemistry communications Vol. 91; pp. 19 - 24
Main Authors Armstrong, Craig G., Toghill, Kathryn E.
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.06.2018
Subjects
Molecular radicals
Non-aqueous electrolyte
Redox active organics
Redox flow batteries
Redox flow batteries
Non-aqueous electrolyte
Redox active organics
Molecular radicals
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Abstract The application of novel organic redox materials is a plausible pathway towards techno-economic energy storage targets due to their low cost and sustainable design. Their operation in non-aqueous redox flow batteries affords researchers the opportunity to innovate, design and optimise these new chemistries towards practical energy densities. Despite this, the identification of high capacity organics which also display long-term stability is inherently challenging due to the high reactivity of molecular radicals. •Redox-active organic molecules are promising new energy storage materials.•The stability of molecular free radicals is concisely reviewed.•Decomposition of radical states results in irreversible battery capacity loss.•Radical half-life depends on chemical structure and electrolyte conditions.•Neutral, anionic and cationic radicals are distinct chemical species.
AbstractList The application of novel organic redox materials is a plausible pathway towards techno-economic energy storage targets due to their low cost and sustainable design. Their operation in non-aqueous redox flow batteries affords researchers the opportunity to innovate, design and optimise these new chemistries towards practical energy densities. Despite this, the identification of high capacity organics which also display long-term stability is inherently challenging due to the high reactivity of molecular radicals. •Redox-active organic molecules are promising new energy storage materials.•The stability of molecular free radicals is concisely reviewed.•Decomposition of radical states results in irreversible battery capacity loss.•Radical half-life depends on chemical structure and electrolyte conditions.•Neutral, anionic and cationic radicals are distinct chemical species.
Author Armstrong, Craig G.
Toghill, Kathryn E.
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Keywords Redox flow batteries
Non-aqueous electrolyte
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Snippet The application of novel organic redox materials is a plausible pathway towards techno-economic energy storage targets due to their low cost and sustainable...
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SubjectTerms Molecular radicals
Non-aqueous electrolyte
Redox active organics
Redox flow batteries
Title Stability of molecular radicals in organic non-aqueous redox flow batteries: A mini review
URI https://dx.doi.org/10.1016/j.elecom.2018.04.017
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