Efficient removal of methylene blue from aqueous solutions using magnetic graphene oxide modified zeolite
[Display omitted] In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized b...
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| Published in | Journal of colloid and interface science Vol. 543; pp. 43 - 51 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
01.05.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized by SEM, XRD, FTIR, XPS, and magnetization curves. In order to understand the pollutant removal performance of the as-prepared composites, methylene blue (MB) was used as the target pollutant in adsorption experiments. The removal efficiency of MB onto Cu-Z-GO-M composite was enhanced obviously with pH > 9. The adsorption capacities of MB onto Cu-Z-GO-M 1:1 were 82.147, 89.315, 97.346 mg/g at 298, 308, and 318 K, respectively. The removal ability of MB increased with the increase of GO content in modified composites. The adsorption behavior can be well described using a pseudo-second-order kinetic and Freundlich isotherm model. The thermodynamic analysis indicated the MB adsorption by Cu-Z-GO-M was a spontaneous and endothermic reaction. The results showed that the prepared Cu-Z-GO-M composite could be a promising adsorbent with good adsorption capacity and reusability for MB removal from wastewater. |
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| AbstractList | In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized by SEM, XRD, FTIR, XPS, and magnetization curves. In order to understand the pollutant removal performance of the as-prepared composites, methylene blue (MB) was used as the target pollutant in adsorption experiments. The removal efficiency of MB onto Cu-Z-GO-M composite was enhanced obviously with pH > 9. The adsorption capacities of MB onto Cu-Z-GO-M 1:1 were 82.147, 89.315, 97.346 mg/g at 298, 308, and 318 K, respectively. The removal ability of MB increased with the increase of GO content in modified composites. The adsorption behavior can be well described using a pseudo-second-order kinetic and Freundlich isotherm model. The thermodynamic analysis indicated the MB adsorption by Cu-Z-GO-M was a spontaneous and endothermic reaction. The results showed that the prepared Cu-Z-GO-M composite could be a promising adsorbent with good adsorption capacity and reusability for MB removal from wastewater.In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized by SEM, XRD, FTIR, XPS, and magnetization curves. In order to understand the pollutant removal performance of the as-prepared composites, methylene blue (MB) was used as the target pollutant in adsorption experiments. The removal efficiency of MB onto Cu-Z-GO-M composite was enhanced obviously with pH > 9. The adsorption capacities of MB onto Cu-Z-GO-M 1:1 were 82.147, 89.315, 97.346 mg/g at 298, 308, and 318 K, respectively. The removal ability of MB increased with the increase of GO content in modified composites. The adsorption behavior can be well described using a pseudo-second-order kinetic and Freundlich isotherm model. The thermodynamic analysis indicated the MB adsorption by Cu-Z-GO-M was a spontaneous and endothermic reaction. The results showed that the prepared Cu-Z-GO-M composite could be a promising adsorbent with good adsorption capacity and reusability for MB removal from wastewater. In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized by SEM, XRD, FTIR, XPS, and magnetization curves. In order to understand the pollutant removal performance of the as-prepared composites, methylene blue (MB) was used as the target pollutant in adsorption experiments. The removal efficiency of MB onto Cu-Z-GO-M composite was enhanced obviously with pH > 9. The adsorption capacities of MB onto Cu-Z-GO-M 1:1 were 82.147, 89.315, 97.346 mg/g at 298, 308, and 318 K, respectively. The removal ability of MB increased with the increase of GO content in modified composites. The adsorption behavior can be well described using a pseudo-second-order kinetic and Freundlich isotherm model. The thermodynamic analysis indicated the MB adsorption by Cu-Z-GO-M was a spontaneous and endothermic reaction. The results showed that the prepared Cu-Z-GO-M composite could be a promising adsorbent with good adsorption capacity and reusability for MB removal from wastewater. [Display omitted] In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M 1:1) were synthesized by solid-state dispersion (SSD) method. The properties of zeolite-based composites were characterized by SEM, XRD, FTIR, XPS, and magnetization curves. In order to understand the pollutant removal performance of the as-prepared composites, methylene blue (MB) was used as the target pollutant in adsorption experiments. The removal efficiency of MB onto Cu-Z-GO-M composite was enhanced obviously with pH > 9. The adsorption capacities of MB onto Cu-Z-GO-M 1:1 were 82.147, 89.315, 97.346 mg/g at 298, 308, and 318 K, respectively. The removal ability of MB increased with the increase of GO content in modified composites. The adsorption behavior can be well described using a pseudo-second-order kinetic and Freundlich isotherm model. The thermodynamic analysis indicated the MB adsorption by Cu-Z-GO-M was a spontaneous and endothermic reaction. The results showed that the prepared Cu-Z-GO-M composite could be a promising adsorbent with good adsorption capacity and reusability for MB removal from wastewater. |
| Author | Zeng, Guangming Yuan, Lei Peng, Min He, Kai Yan, Ming Li, Hui Chen, Guiqiu Chen, Anwei Huang, Zhenzhen Huang, Tiantian |
| Author_xml | – sequence: 1 givenname: Tiantian surname: Huang fullname: Huang, Tiantian organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 2 givenname: Ming surname: Yan fullname: Yan, Ming organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 3 givenname: Kai surname: He fullname: He, Kai organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 4 givenname: Zhenzhen surname: Huang fullname: Huang, Zhenzhen organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 5 givenname: Guangming orcidid: 0000-0002-4230-7647 surname: Zeng fullname: Zeng, Guangming email: zgming@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 6 givenname: Anwei surname: Chen fullname: Chen, Anwei email: A.Chen@hunau.edu.cn organization: College of Resources and Environment, Hunan Agricultural University, Changsha 410128, PR China – sequence: 7 givenname: Min surname: Peng fullname: Peng, Min organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 8 givenname: Hui surname: Li fullname: Li, Hui organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 9 givenname: Lei surname: Yuan fullname: Yuan, Lei organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 10 givenname: Guiqiu surname: Chen fullname: Chen, Guiqiu organization: College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30776669$$D View this record in MEDLINE/PubMed |
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In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M... In this study, magnetic graphene oxide modified zeolite (Cu-Z-GO-M) composites with two different ratios of GO to zeolite (named Cu-Z-GO-M 1:2 and Cu-Z-GO-M... |
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| SubjectTerms | adsorbents Adsorption aqueous solutions endothermy Fourier transform infrared spectroscopy Graphene oxide magnetism Methylene blue MnFe2O4 pollutants pollution control scanning electron microscopy sorption isotherms thermodynamics wastewater X-ray diffraction X-ray photoelectron spectroscopy Zeolite zeolites |
| Title | Efficient removal of methylene blue from aqueous solutions using magnetic graphene oxide modified zeolite |
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