Complexation and coacervation of polyelectrolytes with oppositely charged colloids
Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of the colloid, and (2) reducing the heterogeneity and configurational complexity of polyelectrolyte–polyelectrolyte (PE–PE) systems. Interest i...
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| Published in | Advances in colloid and interface science Vol. 167; no. 1; pp. 24 - 37 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
14.09.2011
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of the colloid, and (2) reducing the heterogeneity and configurational complexity of polyelectrolyte–polyelectrolyte (PE–PE) systems. Interest in protein-polyelectrolyte coacervates arises from preservation of biofunctionality; in addition, the geometric and charge isotropy of micelles allows for better comparison with theory, taking into account the central role of colloid charge density. In the context of these two systems, we describe critical conditions for complex formation and for coacervation with regard to colloid and polyelectrolyte charge densities, ionic strength, PE molecular weight (MW), and stoichiometry; and effects of temperature and shear, which are unique to the PE-micelle systems. The coacervation process is discussed in terms of theoretical treatments and models, as supported by experimental findings. We point out how soluble aggregates, subject to various equilibria and disproportionation effects, can self-assemble leading to heterogeneity in macroscopically homogeneous coacervates, on multiple length scales. |
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| AbstractList | Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of the colloid, and (2) reducing the heterogeneity and configurational complexity of polyelectrolyte–polyelectrolyte (PE–PE) systems. Interest in protein-polyelectrolyte coacervates arises from preservation of biofunctionality; in addition, the geometric and charge isotropy of micelles allows for better comparison with theory, taking into account the central role of colloid charge density. In the context of these two systems, we describe critical conditions for complex formation and for coacervation with regard to colloid and polyelectrolyte charge densities, ionic strength, PE molecular weight (MW), and stoichiometry; and effects of temperature and shear, which are unique to the PE-micelle systems. The coacervation process is discussed in terms of theoretical treatments and models, as supported by experimental findings. We point out how soluble aggregates, subject to various equilibria and disproportionation effects, can self-assemble leading to heterogeneity in macroscopically homogeneous coacervates, on multiple length scales. Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of the colloid, and (2) reducing the heterogeneity and configurational complexity of polyelectrolyte-polyelectrolyte (PE-PE) systems. Interest in protein-polyelectrolyte coacervates arises from preservation of biofunctionality; in addition, the geometric and charge isotropy of micelles allows for better comparison with theory, taking into account the central role of colloid charge density. In the context of these two systems, we describe critical conditions for complex formation and for coacervation with regard to colloid and polyelectrolyte charge densities, ionic strength, PE molecular weight (MW), and stoichiometry; and effects of temperature and shear, which are unique to the PE-micelle systems. The coacervation process is discussed in terms of theoretical treatments and models, as supported by experimental findings. We point out how soluble aggregates, subject to various equilibria and disproportionation effects, can self-assemble leading to heterogeneity in macroscopically homogeneous coacervates, on multiple length scales.Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of the colloid, and (2) reducing the heterogeneity and configurational complexity of polyelectrolyte-polyelectrolyte (PE-PE) systems. Interest in protein-polyelectrolyte coacervates arises from preservation of biofunctionality; in addition, the geometric and charge isotropy of micelles allows for better comparison with theory, taking into account the central role of colloid charge density. In the context of these two systems, we describe critical conditions for complex formation and for coacervation with regard to colloid and polyelectrolyte charge densities, ionic strength, PE molecular weight (MW), and stoichiometry; and effects of temperature and shear, which are unique to the PE-micelle systems. The coacervation process is discussed in terms of theoretical treatments and models, as supported by experimental findings. We point out how soluble aggregates, subject to various equilibria and disproportionation effects, can self-assemble leading to heterogeneity in macroscopically homogeneous coacervates, on multiple length scales. |
| Author | Dubin, Paul L. Kayitmazer, A. Basak Kizilay, Ebru |
| Author_xml | – sequence: 1 givenname: Ebru surname: Kizilay fullname: Kizilay, Ebru email: ekizilay@chem.umass.edu organization: Department of Chemistry, University of Massachusetts Amherst, MA 01003, United States – sequence: 2 givenname: A. Basak surname: Kayitmazer fullname: Kayitmazer, A. Basak email: basak.kayitmazer@boun.edu.tr organization: Department of Chemistry, Bogazici University, Bebek, 34342 Istanbul, Turkey – sequence: 3 givenname: Paul L. surname: Dubin fullname: Dubin, Paul L. organization: Department of Chemistry, University of Massachusetts Amherst, MA 01003, United States |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/21803318$$D View this record in MEDLINE/PubMed |
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| Snippet | Polyelectrolyte-colloid coacervation could be viewed as a sub-category of complex coacervation, but is unique in (1) retaining the structure and properties of... |
| SourceID | proquest pubmed crossref elsevier |
| SourceType | Aggregation Database Index Database Enrichment Source Publisher |
| StartPage | 24 |
| SubjectTerms | Charge Charge density Coacervate Colloids Complex coacervation electrolytes Heterogeneity ionic strength Isotropy micelles molecular weight Polyelectrolyte-colloid interactions Polyelectrolytes Polyethylenes Shear stoichiometry Structure temperature |
| Title | Complexation and coacervation of polyelectrolytes with oppositely charged colloids |
| URI | https://dx.doi.org/10.1016/j.cis.2011.06.006 https://www.ncbi.nlm.nih.gov/pubmed/21803318 https://www.proquest.com/docview/1746464212 https://www.proquest.com/docview/888092094 https://www.proquest.com/docview/926318560 |
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