Rediscovering black phosphorus as an anisotropic layered material for optoelectronics and electronics

Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable...

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Published in	Nature communications Vol. 5; no. 1; p. 4458
Main Authors	Xia, Fengnian, Wang, Han, Jia, Yichen
Format	Journal Article
Language	English
Published	London Nature Publishing Group UK 21.07.2014 Nature Publishing Group
Subjects	639/301/1005 639/624/1075/401 639/766/1130 Anisotropy Crystal structure Graphene Humanities and Social Sciences multidisciplinary Phosphorus Science Science (multidisciplinary) Thin films Transistors United States > US
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Abstract	Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm 2 V −1 s −1 for holes along the light ( x ) and heavy ( y ) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on–off current ratio exceeding 10 5 , a field-effect mobility of 205 cm 2 V −1 s −1 , and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable. The applications of graphene and transition metal dichalcogenides in electronics are limited by their zero-bandgap and low mobility, respectively. Here, the authors demonstrate the potential of an emerging layered material—black phosphorous—for thin film electronics and infrared optoelectronics.
AbstractList	Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm(2)V(-1)s(-1) for holes along the light (x) and heavy (y) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on-off current ratio exceeding 10(5), a field-effect mobility of 205 cm(2)V(-1)s(-1), and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable.Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm(2)V(-1)s(-1) for holes along the light (x) and heavy (y) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on-off current ratio exceeding 10(5), a field-effect mobility of 205 cm(2)V(-1)s(-1), and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable. Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm 2 V −1 s −1 for holes along the light ( x ) and heavy ( y ) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on–off current ratio exceeding 10 5 , a field-effect mobility of 205 cm 2 V −1 s −1 , and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable. The applications of graphene and transition metal dichalcogenides in electronics are limited by their zero-bandgap and low mobility, respectively. Here, the authors demonstrate the potential of an emerging layered material—black phosphorous—for thin film electronics and infrared optoelectronics. Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm(2)V(-1)s(-1) for holes along the light (x) and heavy (y) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on-off current ratio exceeding 10(5), a field-effect mobility of 205 cm(2)V(-1)s(-1), and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable. Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap nature of graphene and the relatively low mobility in TMDCs limit their applications. Here we reintroduce black phosphorus (BP), the most stable allotrope of phosphorus with strong intrinsic in-plane anisotropy, to the layered-material family. For 15-nm-thick BP, we measure a Hall mobility of 1,000 and 600 cm2 V-1 s-1 for holes along the light (x) and heavy (y) effective mass directions at 120 K. BP thin films also exhibit large and anisotropic in-plane optical conductivity from 2 to 5 μm. Field-effect transistors using 5 nm BP along x direction exhibit an on-off current ratio exceeding 105 , a field-effect mobility of 205 cm2 V-1 s-1 , and good current saturation characteristics all at room temperature. BP shows great potential for thin-film electronics, infrared optoelectronics and novel devices in which anisotropic properties are desirable.
ArticleNumber	4458
Author	Jia, Yichen Wang, Han Xia, Fengnian
Author_xml	– sequence: 1 givenname: Fengnian surname: Xia fullname: Xia, Fengnian email: fengnian.xia@yale.edu organization: Department of Electrical Engineering, Yale University – sequence: 2 givenname: Han surname: Wang fullname: Wang, Han email: wanghan@us.ibm.com organization: IBM Thomas J. Watson Research Center – sequence: 3 givenname: Yichen surname: Jia fullname: Jia, Yichen organization: Department of Electrical Engineering, Yale University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/25041752$$D View this record in MEDLINE/PubMed
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Snippet	Graphene and transition metal dichalcogenides (TMDCs) are the two major types of layered materials under intensive investigation. However, the zero-bandgap...
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SubjectTerms	639/301/1005 639/624/1075/401 639/766/1130 Anisotropy Crystal structure Graphene Humanities and Social Sciences multidisciplinary Phosphorus Science Science (multidisciplinary) Thin films Transistors
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Title	Rediscovering black phosphorus as an anisotropic layered material for optoelectronics and electronics
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