De Novo Design of Covalent Organic Framework Membranes toward Ultrafast Anion Transport
The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frame...
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| Published in | Advanced materials (Weinheim) Vol. 32; no. 36; pp. e2001284 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
01.09.2020
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| Online Access | Get full text |
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| Abstract | The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase‐transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium‐functionalized side chains along the channels within the frameworks. The resultant self‐standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm−1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all‐organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes.
The de novo design of covalent organic frameworks (COFs) affords a dense and ordered alignment of quaternary ammonium‐functionalized side chains along the intrinsic channels within the frameworks, rendering one of the highest hydroxide conductivities among the reported anion‐exchange membranes (AEMs), and demonstrating the feasibility of COFs as the building blocks for high‐performance AEMs. |
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| AbstractList | The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase‐transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium‐functionalized side chains along the channels within the frameworks. The resultant self‐standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm−1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all‐organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes. The emergence of all-organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase-transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium-functionalized side chains along the channels within the frameworks. The resultant self-standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm-1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all-organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes.The emergence of all-organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase-transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium-functionalized side chains along the channels within the frameworks. The resultant self-standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm-1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all-organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes. The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase‐transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium‐functionalized side chains along the channels within the frameworks. The resultant self‐standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm−1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all‐organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes. The de novo design of covalent organic frameworks (COFs) affords a dense and ordered alignment of quaternary ammonium‐functionalized side chains along the intrinsic channels within the frameworks, rendering one of the highest hydroxide conductivities among the reported anion‐exchange membranes (AEMs), and demonstrating the feasibility of COFs as the building blocks for high‐performance AEMs. The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy conversion and storage applications. Herein, inspired by the efficient anion transport within organisms, a de novo design of covalent organic frameworks (COFs) toward ultrafast anion transport is demonstrated. A phase‐transfer polymerization process is developed to acquire dense and ordered alignment of quaternary ammonium‐functionalized side chains along the channels within the frameworks. The resultant self‐standing COFs membranes exhibit one of the highest hydroxide conductivities (212 mS cm −1 at 80 °C) among the reported anion exchange membranes. Meanwhile, it is found that shorter, more hydrophilic side chains are favorable for anion conduction. The present work highlights the prospects of all‐organic framework materials as the platform building blocks in designing ion exchange membranes and ion sieving membranes. |
| Author | Zhang, Zhenjie Jiang, Zhongyi Wu, Hong Tongsh, Chasen Kong, Yan He, Guangwei Zhu, Kongying He, Xueyi Shi, Benbing Cao, Li Jiao, Kui Xu, Zhongxing Yang, Yi |
| Author_xml | – sequence: 1 givenname: Xueyi surname: He fullname: He, Xueyi organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 2 givenname: Yi surname: Yang fullname: Yang, Yi organization: Nankai University – sequence: 3 givenname: Hong surname: Wu fullname: Wu, Hong organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 4 givenname: Guangwei surname: He fullname: He, Guangwei organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 5 givenname: Zhongxing surname: Xu fullname: Xu, Zhongxing organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 6 givenname: Yan surname: Kong fullname: Kong, Yan organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 7 givenname: Li surname: Cao fullname: Cao, Li organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 8 givenname: Benbing surname: Shi fullname: Shi, Benbing organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 9 givenname: Zhenjie surname: Zhang fullname: Zhang, Zhenjie organization: Nankai University – sequence: 10 givenname: Chasen surname: Tongsh fullname: Tongsh, Chasen organization: Tianjin University – sequence: 11 givenname: Kui surname: Jiao fullname: Jiao, Kui organization: Tianjin University – sequence: 12 givenname: Kongying surname: Zhu fullname: Zhu, Kongying organization: Tianjin University – sequence: 13 givenname: Zhongyi orcidid: 0000-0002-0048-8849 surname: Jiang fullname: Jiang, Zhongyi email: zhyjiang@tju.edu.cn organization: International Campus of Tianjin University |
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| Snippet | The emergence of all‐organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy... The emergence of all-organic frameworks is of fundamental significance, and designing such structures for anion conduction holds great promise in energy... |
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| SubjectTerms | Anion exchanging anion transport covalent organic framework membranes de novo design Energy conversion Energy storage Ion exchange Membranes phase‐transfer polymerization side‐chain engineering |
| Title | De Novo Design of Covalent Organic Framework Membranes toward Ultrafast Anion Transport |
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