MOF Template-Derived Carbon Shell-Embedded CoP Hierarchical Nanosheet as Bifunctional Catalyst for Overall Water Splitting

The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for hydrogen production through overall water splitting. Herein, we report a novel nanostructure consisting of vertically oriented CoP hierarchic...

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Published inNanomaterials (Basel, Switzerland) Vol. 13; no. 17; p. 2421
Main Authors Liu, Mei-Jun, Yang, Fu-Hao, Mei, Ji-Cheng, Guo, Xu, Wang, Hua-Yang, He, Meng-Yao, Yao, Yu-Ang, Zhang, Hai-Feng, Liu, Cheng-Bin
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 25.08.2023
MDPI
Subjects
Carbon
Carbon compounds
Catalysts
Composite materials
Electric properties
Electrical conductivity
Electrical resistivity
Electrocatalysts
Electrodes
Ethanol
hierarchical nanosheet
Hybrids
Hydrogen evolution
Hydrogen production
Mechanical properties
Metal foils
Metal-organic frameworks
metal–organic framework
Morphology
Nanosheets
Nanostructure
Nitrates
Organometallic compounds
overall water splitting
Oxygen evolution reactions
Phosphorus compounds
Splitting
Titanium
transition metal phosphide
Water splitting
Zeolites
China
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Abstract The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for hydrogen production through overall water splitting. Herein, we report a novel nanostructure consisting of vertically oriented CoP hierarchical nanosheet arrays with in situ-assembled carbon skeletons on a Ti foil electrode. The novel Zeolitic Imidazolate Framework-67 (ZIF-67) template-derived hierarchical nanosheet architecture effectively improved electrical conductivity, facilitated electrolyte transport, and increased the exposure of the active sites. The obtained bifunctional hybrid exhibited a low overpotential of 72 mV at 10 mA cm−2 and a small Tafel slope of 65 mV dec−1 for HER, and an improved overpotential of 329 mV and a Tafel slope of 107 mV dec−1 for OER. Furthermore, the assembled C@CoP||C@CoP electrolyzer showed excellent overall water splitting performance (1.63 V) at a current density of 10 mA cm−2 and superior durability. This work provides a structure engineering strategy for metal–organic framework (MOF) template-derived hybrids with outstanding electrocatalytic performance.
AbstractList The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for hydrogen production through overall water splitting. Herein, we report a novel nanostructure consisting of vertically oriented CoP hierarchical nanosheet arrays with in situ-assembled carbon skeletons on a Ti foil electrode. The novel Zeolitic Imidazolate Framework-67 (ZIF-67) template-derived hierarchical nanosheet architecture effectively improved electrical conductivity, facilitated electrolyte transport, and increased the exposure of the active sites. The obtained bifunctional hybrid exhibited a low overpotential of 72 mV at 10 mA cm −2 and a small Tafel slope of 65 mV dec −1 for HER, and an improved overpotential of 329 mV and a Tafel slope of 107 mV dec −1 for OER. Furthermore, the assembled C@CoP||C@CoP electrolyzer showed excellent overall water splitting performance (1.63 V) at a current density of 10 mA cm −2 and superior durability. This work provides a structure engineering strategy for metal–organic framework (MOF) template-derived hybrids with outstanding electrocatalytic performance.
The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for hydrogen production through overall water splitting. Herein, we report a novel nanostructure consisting of vertically oriented CoP hierarchical nanosheet arrays with in situ-assembled carbon skeletons on a Ti foil electrode. The novel Zeolitic Imidazolate Framework-67 (ZIF-67) template-derived hierarchical nanosheet architecture effectively improved electrical conductivity, facilitated electrolyte transport, and increased the exposure of the active sites. The obtained bifunctional hybrid exhibited a low overpotential of 72 mV at 10 mA cm−2 and a small Tafel slope of 65 mV dec−1 for HER, and an improved overpotential of 329 mV and a Tafel slope of 107 mV dec−1 for OER. Furthermore, the assembled C@CoP||C@CoP electrolyzer showed excellent overall water splitting performance (1.63 V) at a current density of 10 mA cm−2 and superior durability. This work provides a structure engineering strategy for metal–organic framework (MOF) template-derived hybrids with outstanding electrocatalytic performance.
The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for hydrogen production through overall water splitting. Herein, we report a novel nanostructure consisting of vertically oriented CoP hierarchical nanosheet arrays with in situ-assembled carbon skeletons on a Ti foil electrode. The novel Zeolitic Imidazolate Framework-67 (ZIF-67) template-derived hierarchical nanosheet architecture effectively improved electrical conductivity, facilitated electrolyte transport, and increased the exposure of the active sites. The obtained bifunctional hybrid exhibited a low overpotential of 72 mV at 10 mA cm[sup.−2] and a small Tafel slope of 65 mV dec[sup.−1] for HER, and an improved overpotential of 329 mV and a Tafel slope of 107 mV dec[sup.−1] for OER. Furthermore, the assembled C@CoP||C@CoP electrolyzer showed excellent overall water splitting performance (1.63 V) at a current density of 10 mA cm[sup.−2] and superior durability. This work provides a structure engineering strategy for metal–organic framework (MOF) template-derived hybrids with outstanding electrocatalytic performance.
Audience Academic
Author Guo, Xu
Liu, Mei-Jun
Wang, Hua-Yang
Yao, Yu-Ang
Liu, Cheng-Bin
Zhang, Hai-Feng
He, Meng-Yao
Mei, Ji-Cheng
Yang, Fu-Hao
AuthorAffiliation 2 State Key Laboratory of Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, China
1 School of Chemical Engineering, Northeast Electric Power University, Jilin 132012, China; 20203003@neepu.edu.cn (M.-J.L.); 2202200810@neepu.edu.cn (F.-H.Y.); meijicheng@hnu.edu.cn (J.-C.M.); 2021304040115@neepu.edu.cn (X.G.); 2021304040226@neepu.edu.cn (H.-Y.W.); 2202100766@neepu.edu.cn (M.-Y.H.); 2202200809@neepu.edu.cn (Y.-A.Y.)
AuthorAffiliation_xml – name: 1 School of Chemical Engineering, Northeast Electric Power University, Jilin 132012, China; 20203003@neepu.edu.cn (M.-J.L.); 2202200810@neepu.edu.cn (F.-H.Y.); meijicheng@hnu.edu.cn (J.-C.M.); 2021304040115@neepu.edu.cn (X.G.); 2021304040226@neepu.edu.cn (H.-Y.W.); 2202100766@neepu.edu.cn (M.-Y.H.); 2202200809@neepu.edu.cn (Y.-A.Y.)
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Snippet The design of earth-abundant and highly efficient bifunctional electrocatalysts for hydrogen evolution and oxygen evolution reactions (HER/OER) is crucial for...
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SubjectTerms Carbon
Carbon compounds
Catalysts
Composite materials
Electric properties
Electrical conductivity
Electrical resistivity
Electrocatalysts
Electrodes
Ethanol
hierarchical nanosheet
Hybrids
Hydrogen evolution
Hydrogen production
Mechanical properties
Metal foils
Metal-organic frameworks
metal–organic framework
Morphology
Nanosheets
Nanostructure
Nitrates
Organometallic compounds
overall water splitting
Oxygen evolution reactions
Phosphorus compounds
Splitting
Titanium
transition metal phosphide
Water splitting
Zeolites
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Title MOF Template-Derived Carbon Shell-Embedded CoP Hierarchical Nanosheet as Bifunctional Catalyst for Overall Water Splitting
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https://search.proquest.com/docview/2863293793
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https://doaj.org/article/670388f426a4428cbc58e5ab82070f82
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