Carbon Structures with Three-Dimensional Periodicity at Optical Wavelengths
Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltrat...
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| Published in | Science (American Association for the Advancement of Science) Vol. 282; no. 5390; pp. 897 - 901 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Society for the Advancement of Science
30.10.1998
American Association for the Advancement of Science The American Association for the Advancement of Science |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltration with carbon or a carbon precursor. The resulting porous carbons had different structures depending on synthesis conditions. Both diamond and glassy carbon inverse opals resulted from volume filling. Graphite inverse opals, comprising 40-angstrom-thick layers of graphite sheets tiled on spherical surfaces, were produced by surface templating. The carbon inverse opals provide examples of both dielectric and metallic optical photonic crystals. They strongly diffract light and may provide a route toward photonic band-gap materials. |
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| AbstractList | Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltration with carbon or a carbon precursor. The resulting porous carbons had different structures depending on synthesis conditions. Both diamond and glassy carbon inverse opals resulted from volume filling. Graphite inverse opals, comprising 40-angstrom-thick layers of graphite sheets tiled on spherical surfaces, were produced by surface templating. The carbon inverse opals provide examples of both dielectric and metallic optical photonic crystals. They strongly diffract light and may provide a route toward photonic band-gap materials. Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltration with carbon or a carbon precursor. Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltration with carbon or a carbon precursor. The resulting porous carbons had different structures depending on synthesis conditions. Both diamond and glassy carbon inverse opals resulted from volume fitting. Graphite inverse opals, comprising 40-angstrom-thick layers of graphite sheets tiled on spherical surfaces, were produced by surface templating. The carbon inverse opals provide examples of both dielectric and metallic optical photonic crystals. They strongly diffract light and may provide a route toward photonic band-gap materials. |
| Audience | Academic |
| Author | Dantas, Socrates O. Ralchenko, Victor G. Khayrullin, Ilyas Baughman, Ray H. Iqbal, Zafar Marti, Jordi Zakhidov, Anvar A. Cui, Changxing |
| Author_xml | – sequence: 1 givenname: Anvar A. surname: Zakhidov fullname: Zakhidov, Anvar A. – sequence: 2 givenname: Ray H. surname: Baughman fullname: Baughman, Ray H. – sequence: 3 givenname: Zafar surname: Iqbal fullname: Iqbal, Zafar – sequence: 4 givenname: Changxing surname: Cui fullname: Cui, Changxing – sequence: 5 givenname: Ilyas surname: Khayrullin fullname: Khayrullin, Ilyas – sequence: 6 givenname: Socrates O. surname: Dantas fullname: Dantas, Socrates O. – sequence: 7 givenname: Jordi surname: Marti fullname: Marti, Jordi – sequence: 8 givenname: Victor G. surname: Ralchenko fullname: Ralchenko, Victor G. |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/9794752$$D View this record in MEDLINE/PubMed |
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| References_xml | – volume: 208 start-page: 371 year: 1993 ident: e_1_3_1_7_2 publication-title: Physica C doi: 10.1016/0921-4534(93)90211-8 contributor: fullname: Bogomolov V. N. – ident: e_1_3_1_8_3 – volume: 391 start-page: 667 year: 1998 ident: e_1_3_1_3_3 publication-title: Nature doi: 10.1038/35570 contributor: fullname: Yablonovitch E. – volume: 385 start-page: 321 year: 1997 ident: e_1_3_1_5_3 publication-title: ibid. contributor: fullname: van Blaaderen A. – volume: 68 start-page: 511 year: 1992 ident: e_1_3_1_17_4 publication-title: Phys. Rev Lett. doi: 10.1103/PhysRevLett.68.511 contributor: fullname: Vanderbilt D. – ident: e_1_3_1_8_5 – ident: e_1_3_1_12_2 – ident: e_1_3_1_13_2 doi: 10.1016/S0925-9635(96)00743-1 – ident: e_1_3_1_2_2 doi: 10.1103/PhysRevLett.58.2486 – ident: #cr-split#-e_1_3_1_9_2.1 doi: 10.1038/scientificamerican0476-84 – volume: 355 start-page: 333 year: 1992 ident: e_1_3_1_17_3 publication-title: ibid. contributor: fullname: Lenosky T. – volume: 58 start-page: 3896 year: 1998 ident: e_1_3_1_2_4 publication-title: Phys. Rev. E. doi: 10.1103/PhysRevE.58.3896 contributor: fullname: Busch K. – ident: e_1_3_1_7_4 – volume: 389 start-page: 829 year: 1997 ident: e_1_3_1_5_2 publication-title: Nature doi: 10.1038/39834 contributor: fullname: Holtz J. H. – ident: e_1_3_1_18_2 – ident: e_1_3_1_3_2 doi: 10.1103/PhysRevLett.58.2059 – ident: e_1_3_1_11_2 – volume: 76 start-page: 2480 year: 1996 ident: e_1_3_1_4_2 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.76.2480 contributor: fullname: Sievenpiper D. F. – volume: 281 start-page: 538 year: 1998 ident: e_1_3_1_8_4 publication-title: Science doi: 10.1126/science.281.5376.538 contributor: fullname: Blanford C. F. – volume: 8 start-page: 1371 year: 1987 ident: e_1_3_1_6_2 publication-title: J. Mater. Sci. Lett. doi: 10.1007/BF00720190 contributor: fullname: Philipse A. P. – ident: e_1_3_1_14_2 – ident: e_1_3_1_2_3 doi: 10.1063/1.881300 – ident: #cr-split#-e_1_3_1_9_2.2 – ident: e_1_3_1_4_3 – ident: e_1_3_1_6_3 doi: 10.1006/spmi.1996.0313 – ident: e_1_3_1_8_2 doi: 10.1038/40105 – volume: 6 start-page: 1783 year: 1988 ident: e_1_3_1_15_2 publication-title: J. Vac. Sci. Technol. A doi: 10.1116/1.575297 contributor: fullname: Nemanich R. J. – volume: 352 start-page: 762 year: 1991 ident: e_1_3_1_17_2 publication-title: Nature doi: 10.1038/352762a0 contributor: fullname: Mackay A. L. – ident: e_1_3_1_10_2 – ident: e_1_3_1_16_2 doi: 10.1016/S0008-6223(98)00014-1 – volume: 36 start-page: L714 year: 1997 ident: e_1_3_1_7_3 publication-title: Jpn. J. Appl. Phys. doi: 10.1143/JJAP.36.6699 contributor: fullname: Yoshino K. |
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