Thermal conductivity determination of suspended mono- and bilayer WS2 by Raman spectroscopy
We report the thermal conductivities of monolayer （1L） and bilayer （2L） WS2 grown by chemical vapor deposition （CVD）, which are determined by use of temperature and excitation dependences of E2g^1 and A1g Raman modes. The first-order temperature coefficients of E2g^1 and Alg modes in both supported...
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| Published in | Nano research Vol. 8; no. 4; pp. 1210 - 1221 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Tsinghua University Press
01.04.2015
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | We report the thermal conductivities of monolayer （1L） and bilayer （2L） WS2 grown by chemical vapor deposition （CVD）, which are determined by use of temperature and excitation dependences of E2g^1 and A1g Raman modes. The first-order temperature coefficients of E2g^1 and Alg modes in both supported and suspended WS2 layers were extracted. The frequency shift of the A3g mode with temperature is larger than that of the E1 mode for 1L-WS2, which is 2g attributed to stronger electron-phonon coupling for the A1g mode than that for the E12g mode. Moreover, by use of the shift of the phonon mode induced by laser heating, the thermal conductivities at room temperature were estimated to be 32 and 53 W/（m.K） for 1L- and 2L-WS2, respectively. Our results provide fundamental information about the thermal properties of WS2 layers, which is crucial for developing applications of atomically-thin WS2 devices. |
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| AbstractList | We report the thermal conductivities of monolayer (1L) and bilayer (2L) WS
2
grown by chemical vapor deposition (CVD), which are determined by use of temperature and excitation dependences of E
2g
1
and A
1g
Raman modes. The first-order temperature coefficients of E
2g
1
and A
1g
modes in both supported and suspended WS
2
layers were extracted. The frequency shift of the A
1g
mode with temperature is larger than that of the E
2g
1
mode for 1L-WS
2
, which is attributed to stronger electron-phonon coupling for the A
1g
mode than that for the E
2g
1
mode. Moreover, by use of the shift of the phonon mode induced by laser heating, the thermal conductivities at room temperature were estimated to be 32 and 53 W/(m·K) for 1L- and 2L-WS
2
, respectively. Our results provide fundamental information about the thermal properties of WS
2
layers, which is crucial for developing applications of atomically-thin WS
2
devices. We report the thermal conductivities of monolayer （1L） and bilayer （2L） WS2 grown by chemical vapor deposition （CVD）, which are determined by use of temperature and excitation dependences of E2g^1 and A1g Raman modes. The first-order temperature coefficients of E2g^1 and Alg modes in both supported and suspended WS2 layers were extracted. The frequency shift of the A3g mode with temperature is larger than that of the E1 mode for 1L-WS2, which is 2g attributed to stronger electron-phonon coupling for the A1g mode than that for the E12g mode. Moreover, by use of the shift of the phonon mode induced by laser heating, the thermal conductivities at room temperature were estimated to be 32 and 53 W/（m.K） for 1L- and 2L-WS2, respectively. Our results provide fundamental information about the thermal properties of WS2 layers, which is crucial for developing applications of atomically-thin WS2 devices. |
| Author | Namphung Peimyoo Jingzhi Shang Weihuang Yang Yanlong wang Chunxiao Cong Ting Yu |
| AuthorAffiliation | Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, 637371 Singapore, Singapore Department of Physics, Faculty of Science, National University of Singapore, 117542 Singapore, Singapore Graphene Research Center, Faculty of Science, National University of Singapore, 117546 Singapore, Singapore |
| Author_xml | – sequence: 1 givenname: Namphung surname: Peimyoo fullname: Peimyoo, Namphung organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 2 givenname: Jingzhi surname: Shang fullname: Shang, Jingzhi organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 3 givenname: Weihuang surname: Yang fullname: Yang, Weihuang organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 4 givenname: Yanlong surname: Wang fullname: Wang, Yanlong organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 5 givenname: Chunxiao surname: Cong fullname: Cong, Chunxiao organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 6 givenname: Ting surname: Yu fullname: Yu, Ting email: yuting@ntu.edu.sg organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Department of Physics, Faculty of Science, National University of Singapore, Graphene Research Center, Faculty of Science, National University of Singapore |
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| ContentType | Journal Article |
| Copyright | Tsinghua University Press and Springer-Verlag Berlin Heidelberg 2014 |
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| DocumentTitleAlternate | Thermal conductivity determination of suspended mono- and bilayer WS2 by Raman spectroscopy |
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| Issue | 4 |
| Keywords | temperature dependence tungsten disulfide Raman thermal conductivity excitation power |
| Language | English |
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| Notes | 11-5974/O4 We report the thermal conductivities of monolayer （1L） and bilayer （2L） WS2 grown by chemical vapor deposition （CVD）, which are determined by use of temperature and excitation dependences of E2g^1 and A1g Raman modes. The first-order temperature coefficients of E2g^1 and Alg modes in both supported and suspended WS2 layers were extracted. The frequency shift of the A3g mode with temperature is larger than that of the E1 mode for 1L-WS2, which is 2g attributed to stronger electron-phonon coupling for the A1g mode than that for the E12g mode. Moreover, by use of the shift of the phonon mode induced by laser heating, the thermal conductivities at room temperature were estimated to be 32 and 53 W/（m.K） for 1L- and 2L-WS2, respectively. Our results provide fundamental information about the thermal properties of WS2 layers, which is crucial for developing applications of atomically-thin WS2 devices. thermal conductivity,tungsten disulfide,Raman,temperature dependence,excitation power |
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| PublicationCentury | 2000 |
| PublicationDate | 2015-04-01 |
| PublicationDateYYYYMMDD | 2015-04-01 |
| PublicationDate_xml | – month: 04 year: 2015 text: 2015-04-01 day: 01 |
| PublicationDecade | 2010 |
| PublicationPlace | Beijing |
| PublicationPlace_xml | – name: Beijing |
| PublicationTitle | Nano research |
| PublicationTitleAbbrev | Nano Res |
| PublicationTitleAlternate | Nano Research |
| PublicationYear | 2015 |
| Publisher | Tsinghua University Press |
| Publisher_xml | – name: Tsinghua University Press |
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| Snippet | We report the thermal conductivities of monolayer （1L） and bilayer （2L） WS2 grown by chemical vapor deposition （CVD）, which are determined by use of... We report the thermal conductivities of monolayer (1L) and bilayer (2L) WS 2 grown by chemical vapor deposition (CVD), which are determined by use of... |
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| SubjectTerms | Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Chemistry and Materials Science Condensed Matter Physics Materials Science Nanotechnology Research Article WS2 化学气相沉积 发展中国家 声子耦合 拉曼光谱 海藻酸钠 激光诱导加热 热导率 |
| Title | Thermal conductivity determination of suspended mono- and bilayer WS2 by Raman spectroscopy |
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