A multifaceted approach to hydrogen storage

The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be overcome. Not the least of these is the problem of storage, particularly when aimed at use onboard light-vehicles. The aim of this overview is to l...

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Published inPhysical chemistry chemical physics : PCCP Vol. 13; no. 38; pp. 16955 - 16972
Main Authors Churchard, Andrew J., Banach, Ewa, Borgschulte, Andreas, Caputo, Riccarda, Chen, Jian-Cheng, Clary, David, Fijalkowski, Karol J., Geerlings, Hans, Genova, Radostina V., Grochala, Wojciech, Jaroń, Tomasz, Juanes-Marcos, Juan Carlos, Kasemo, Bengt, Kroes, Geert-Jan, Ljubić, Ivan, Naujoks, Nicola, Nørskov, Jens K., Olsen, Roar A., Pendolino, Flavio, Remhof, Arndt, Románszki, Loránd, Tekin, Adem, Vegge, Tejs, Zäch, Michael, Züttel, Andreas
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 01.01.2011
Subjects
Borohydrides
Catalysis
Chemistry
clathrate hydrate
cox-free hydrogen
crystal microbalance
density-functional theory
Exact sciences and technology
General and physical chemistry
generalized gradient approximation
Hydrogen storage
imidazolate frameworks
metal borohydrides
Nanostructure
Networks
Onboard
quartz
Readers
reorientational motion
sodium aluminum-hydride
Stores
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
thermal-decomposition
Confinement
Catalytic reaction
Hydrogen
Selection
Hydrides
Transition metal
Review
Complexes
Mechanism
Solid
Storage
Energy
Catalysis
Kinetics
Catalyst
Online AccessGet full text
ISSN1463-9076
1463-9084
1463-9084
DOI10.1039/c1cp22312g

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Abstract The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be overcome. Not the least of these is the problem of storage, particularly when aimed at use onboard light-vehicles. The aim of this overview is to look in depth at a number of areas linked by the recently concluded HYDROGEN research network, representing an intentionally multi-faceted selection with the goal of advancing the field on a number of fronts simultaneously. For the general reader we provide a concise outline of the main approaches to storing hydrogen before moving on to detailed reviews of recent research in the solid chemical storage of hydrogen, and so provide an entry point for the interested reader on these diverse topics. The subjects covered include: the mechanisms of Ti catalysis in alanates; the kinetics of the borohydrides and the resulting limitations; novel transition metal catalysts for use with complex hydrides; less common borohydrides; protic-hydridic stores; metal ammines and novel approaches to nano-confined metal hydrides.
AbstractList The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be overcome. Not the least of these is the problem of storage, particularly when aimed at use onboard light-vehicles. The aim of this overview is to look in depth at a number of areas linked by the recently concluded HYDROGEN research network, representing an intentionally multi-faceted selection with the goal of advancing the field on a number of fronts simultaneously. For the general reader we provide a concise outline of the main approaches to storing hydrogen before moving on to detailed reviews of recent research in the solid chemical storage of hydrogen, and so provide an entry point for the interested reader on these diverse topics. The subjects covered include: the mechanisms of Ti catalysis in alanates; the kinetics of the borohydrides and the resulting limitations; novel transition metal catalysts for use with complex hydrides; less common borohydrides; protic-hydridic stores; metal ammines and novel approaches to nano-confined metal hydrides.The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be overcome. Not the least of these is the problem of storage, particularly when aimed at use onboard light-vehicles. The aim of this overview is to look in depth at a number of areas linked by the recently concluded HYDROGEN research network, representing an intentionally multi-faceted selection with the goal of advancing the field on a number of fronts simultaneously. For the general reader we provide a concise outline of the main approaches to storing hydrogen before moving on to detailed reviews of recent research in the solid chemical storage of hydrogen, and so provide an entry point for the interested reader on these diverse topics. The subjects covered include: the mechanisms of Ti catalysis in alanates; the kinetics of the borohydrides and the resulting limitations; novel transition metal catalysts for use with complex hydrides; less common borohydrides; protic-hydridic stores; metal ammines and novel approaches to nano-confined metal hydrides.
The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be overcome. Not the least of these is the problem of storage, particularly when aimed at use onboard light-vehicles. The aim of this overview is to look in depth at a number of areas linked by the recently concluded HYDROGEN research network, representing an intentionally multi-faceted selection with the goal of advancing the field on a number of fronts simultaneously. For the general reader we provide a concise outline of the main approaches to storing hydrogen before moving on to detailed reviews of recent research in the solid chemical storage of hydrogen, and so provide an entry point for the interested reader on these diverse topics. The subjects covered include: the mechanisms of Ti catalysis in alanates; the kinetics of the borohydrides and the resulting limitations; novel transition metal catalysts for use with complex hydrides; less common borohydrides; protic-hydridic stores; metal ammines and novel approaches to nano-confined metal hydrides.
Author Románszki, Loránd
Zäch, Michael
Banach, Ewa
Juanes-Marcos, Juan Carlos
Clary, David
Pendolino, Flavio
Kroes, Geert-Jan
Kasemo, Bengt
Ljubić, Ivan
Nørskov, Jens K.
Tekin, Adem
Vegge, Tejs
Churchard, Andrew J.
Naujoks, Nicola
Jaroń, Tomasz
Olsen, Roar A.
Genova, Radostina V.
Chen, Jian-Cheng
Grochala, Wojciech
Fijalkowski, Karol J.
Remhof, Arndt
Züttel, Andreas
Geerlings, Hans
Borgschulte, Andreas
Caputo, Riccarda
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Issue 38
Keywords Confinement
Catalytic reaction
Hydrogen
Selection
Hydrides
Transition metal
Review
Complexes
Mechanism
Solid
Storage
Energy
Catalysis
Kinetics
Catalyst
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Snippet The widespread adoption of hydrogen as an energy carrier could bring significant benefits, but only if a number of currently intractable problems can be...
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StartPage 16955
SubjectTerms Borohydrides
Catalysis
Chemistry
clathrate hydrate
cox-free hydrogen
crystal microbalance
density-functional theory
Exact sciences and technology
General and physical chemistry
generalized gradient approximation
Hydrogen storage
imidazolate frameworks
metal borohydrides
Nanostructure
Networks
Onboard
quartz
Readers
reorientational motion
sodium aluminum-hydride
Stores
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
thermal-decomposition
Title A multifaceted approach to hydrogen storage
URI https://www.ncbi.nlm.nih.gov/pubmed/21887432
https://www.proquest.com/docview/893978922
https://www.proquest.com/docview/963869948
https://www.osti.gov/biblio/1255915
https://research.chalmers.se/publication/147427
Volume 13
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