Progress in the synthesis and applications of hexaaluminate-based catalysts
The development of materials that can exhibit thermal resistance at very high temperatures, thus allowing them to be applied as catalysts and thermal insulators, amongst other possible uses, is a research subject of great interest. This is the case for hexaaluminates, a class of hexagonal aluminate...
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| Published in | Catalysis reviews. Science and engineering Vol. 64; no. 3; pp. 592 - 630 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Taylor & Francis
03.07.2022
Taylor & Francis Ltd |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0161-4940 1520-5703 |
| DOI | 10.1080/01614940.2020.1831756 |
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| Abstract | The development of materials that can exhibit thermal resistance at very high temperatures, thus allowing them to be applied as catalysts and thermal insulators, amongst other possible uses, is a research subject of great interest. This is the case for hexaaluminates, a class of hexagonal aluminate compounds with a unique structure that are stable at very high temperatures up to 1600°C and exhibit exceptional resistance to sintering and thermal shock, thus making them attractive catalysts for high-temperature applications. In this review, the structure of hexaaluminates is presented first. The most recent advances in synthetic methods (sol-gel, reverse microemulsion, hydrothermal synthesis, carbon-templating, solution combustion synthesis, and freeze-drying methods) are discussed subsequently, with the aim of maximizing textural properties and including in their structure metals known to be active in catalytic applications, such as combustion of CH
4
, partial oxidation, and dry reforming of CH
4
to produce synthetic gas, and the decomposition of N
2
O. Finally, other applications, such as their function as a thermal barrier, are also addressed. |
|---|---|
| AbstractList | The development of materials that can exhibit thermal resistance at very high temperatures, thus allowing them to be applied as catalysts and thermal insulators, amongst other possible uses, is a research subject of great interest. This is the case for hexaaluminates, a class of hexagonal aluminate compounds with a unique structure that are stable at very high temperatures up to 1600°C and exhibit exceptional resistance to sintering and thermal shock, thus making them attractive catalysts for high-temperature applications. In this review, the structure of hexaaluminates is presented first. The most recent advances in synthetic methods (sol-gel, reverse microemulsion, hydrothermal synthesis, carbon-templating, solution combustion synthesis, and freeze-drying methods) are discussed subsequently, with the aim of maximizing textural properties and including in their structure metals known to be active in catalytic applications, such as combustion of CH
4
, partial oxidation, and dry reforming of CH
4
to produce synthetic gas, and the decomposition of N
2
O. Finally, other applications, such as their function as a thermal barrier, are also addressed. The development of materials that can exhibit thermal resistance at very high temperatures, thus allowing them to be applied as catalysts and thermal insulators, amongst other possible uses, is a research subject of great interest. This is the case for hexaaluminates, a class of hexagonal aluminate compounds with a unique structure that are stable at very high temperatures up to 1600°C and exhibit exceptional resistance to sintering and thermal shock, thus making them attractive catalysts for high-temperature applications. In this review, the structure of hexaaluminates is presented first. The most recent advances in synthetic methods (sol-gel, reverse microemulsion, hydrothermal synthesis, carbon-templating, solution combustion synthesis, and freeze-drying methods) are discussed subsequently, with the aim of maximizing textural properties and including in their structure metals known to be active in catalytic applications, such as combustion of CH4, partial oxidation, and dry reforming of CH4 to produce synthetic gas, and the decomposition of N2O. Finally, other applications, such as their function as a thermal barrier, are also addressed. |
| Author | Korili, S.A. Gil, A. Torrez-Herrera, J.J. |
| Author_xml | – sequence: 1 givenname: J.J. surname: Torrez-Herrera fullname: Torrez-Herrera, J.J. organization: Edificio de los Acebos, Universidad Pública de Navarra – sequence: 2 givenname: S.A. surname: Korili fullname: Korili, S.A. organization: Edificio de los Acebos, Universidad Pública de Navarra – sequence: 3 givenname: A. orcidid: 0000-0001-9323-5981 surname: Gil fullname: Gil, A. email: andoni@unavarra.es organization: Edificio de los Acebos, Universidad Pública de Navarra |
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| Snippet | The development of materials that can exhibit thermal resistance at very high temperatures, thus allowing them to be applied as catalysts and thermal... |
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| SubjectTerms | Catalysts catalytic high-temperature applications Combustion synthesis Drying hexaaluminate hibonite High temperature Insulators magnetoplumbite Methane Oxidation Reforming Sol-gel processes synthesis methods Thermal resistance Thermal shock |
| Title | Progress in the synthesis and applications of hexaaluminate-based catalysts |
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