Iodine(III)‐Based Halogen Bond Donors: Properties and Applications
Halogen bonding, the non‐covalent interaction of Lewis bases with an electron‐deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen‐containing species as halogen bond donors have been subject to intense research....
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| Published in | Chemical record Vol. 21; no. 8; pp. 1912 - 1927 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken
Wiley Subscription Services, Inc
01.08.2021
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| Online Access | Get full text |
| ISSN | 1527-8999 1528-0691 1528-0691 |
| DOI | 10.1002/tcr.202100119 |
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| Abstract | Halogen bonding, the non‐covalent interaction of Lewis bases with an electron‐deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen‐containing species as halogen bond donors have been subject to intense research. More recently, organoiodine compounds at the iodine(III) state have been receiving growing attention in the field. Due to their electronic and structural properties, they provide access to unique binding modes. For this reason, our groups have been involved in the development of such compounds, in the quantification of their halogen bonding strength (through the evaluation of their Lewis acidities), as well as in the evaluation of their activities as catalysts in several model reactions. This account will describe these contributions.
Iodine(III)‐based halogen bond donors (halogen‐based Lewis acids) have received increasing attention lately. This account provides an overview of the topic and summarizes our studies on Lewis acidity measurements and applications in catalysis. |
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| AbstractList | Halogen bonding, the non‐covalent interaction of Lewis bases with an electron‐deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen‐containing species as halogen bond donors have been subject to intense research. More recently, organoiodine compounds at the iodine(III) state have been receiving growing attention in the field. Due to their electronic and structural properties, they provide access to unique binding modes. For this reason, our groups have been involved in the development of such compounds, in the quantification of their halogen bonding strength (through the evaluation of their Lewis acidities), as well as in the evaluation of their activities as catalysts in several model reactions. This account will describe these contributions. Halogen bonding, the non‐covalent interaction of Lewis bases with an electron‐deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen‐containing species as halogen bond donors have been subject to intense research. More recently, organoiodine compounds at the iodine(III) state have been receiving growing attention in the field. Due to their electronic and structural properties, they provide access to unique binding modes. For this reason, our groups have been involved in the development of such compounds, in the quantification of their halogen bonding strength (through the evaluation of their Lewis acidities), as well as in the evaluation of their activities as catalysts in several model reactions. This account will describe these contributions. Iodine(III)‐based halogen bond donors (halogen‐based Lewis acids) have received increasing attention lately. This account provides an overview of the topic and summarizes our studies on Lewis acidity measurements and applications in catalysis. Halogen bonding, the non-covalent interaction of Lewis bases with an electron-deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen-containing species as halogen bond donors have been subject to intense research. More recently, organoiodine compounds at the iodine(III) state have been receiving growing attention in the field. Due to their electronic and structural properties, they provide access to unique binding modes. For this reason, our groups have been involved in the development of such compounds, in the quantification of their halogen bonding strength (through the evaluation of their Lewis acidities), as well as in the evaluation of their activities as catalysts in several model reactions. This account will describe these contributions.Halogen bonding, the non-covalent interaction of Lewis bases with an electron-deficient region of halogen substituents, received increased attention recently. Consequently, the design and evaluation of numerous halogen-containing species as halogen bond donors have been subject to intense research. More recently, organoiodine compounds at the iodine(III) state have been receiving growing attention in the field. Due to their electronic and structural properties, they provide access to unique binding modes. For this reason, our groups have been involved in the development of such compounds, in the quantification of their halogen bonding strength (through the evaluation of their Lewis acidities), as well as in the evaluation of their activities as catalysts in several model reactions. This account will describe these contributions. |
| Author | Legault, Claude Y. Huber, Stefan M. Reinhard, Dominik L. Robidas, Raphaël |
| Author_xml | – sequence: 1 givenname: Raphaël surname: Robidas fullname: Robidas, Raphaël organization: Université de Sherbrooke – sequence: 2 givenname: Dominik L. surname: Reinhard fullname: Reinhard, Dominik L. organization: Ruhr-Universität Bochum – sequence: 3 givenname: Claude Y. surname: Legault fullname: Legault, Claude Y. email: claude.legault@usherbrooke.ca organization: Université de Sherbrooke – sequence: 4 givenname: Stefan M. orcidid: 0000-0002-4125-159X surname: Huber fullname: Huber, Stefan M. email: stefan.m.huber@rub.de organization: Ruhr-Universität Bochum |
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| ContentType | Journal Article |
| Copyright | 2021 The Authors. Published by The Chemical Society of Japan & Wiley-VCH GmbH 2021. This article is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. 2021 The Authors. Published by The Chemical Society of Japan & Wiley-VCH GmbH. |
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| Snippet | Halogen bonding, the non‐covalent interaction of Lewis bases with an electron‐deficient region of halogen substituents, received increased attention recently.... Halogen bonding, the non-covalent interaction of Lewis bases with an electron-deficient region of halogen substituents, received increased attention recently.... |
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| StartPage | 1912 |
| SubjectTerms | Bonding strength Catalysts Diaryliodonium Donors (electronic) Halogen bonding Hypervalent iodine Iodine Iodolium Lewis acidity |
| Title | Iodine(III)‐Based Halogen Bond Donors: Properties and Applications |
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