Silica-based waste form for immobilization of iodine from reprocessing plant off-gas streams
A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO2-based waste form makes silver-functionalized silica aerogel (Ag0-aerogel) an attractive choice for the removal and sequestration of iodine compounds from the off-gas of a nuclear fuel reprocessing plan...
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| Published in | Journal of nuclear materials Vol. 476; pp. 255 - 261 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier B.V
01.08.2016
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO2-based waste form makes silver-functionalized silica aerogel (Ag0-aerogel) an attractive choice for the removal and sequestration of iodine compounds from the off-gas of a nuclear fuel reprocessing plant. Hot uniaxial pressing of iodine-loaded Ag0-aerogel (20.2 mass% iodine) at 1200 °C for 30 min under 29 MPa pressure provided a partially sintered product with residual open porosity of 16.9% that retained ∼93% of sorbed iodine. Highly iodine-loaded Ag0-aerogel was successfully consolidated by hot isostatic pressing at 1200 °C with a 30-min hold and under 207 MPa. The fully densified waste form had a bulk density of 3.3 × 103 kg/m3 and contained ∼39 mass% iodine. The iodine was retained in the form of nano- and micro-particles of AgI that were uniformly distributed inside and along boundaries of fused silica grains.
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•Silver-functionalized silica aerogel is an effective sorbent and a viable waste form for iodine.•Simultaneous application of fast heating rates and high pressures produced a fully dense product.•HIPing produced a fully consolidated waste form with a bulk density of 3.3 × 103 kg/m3 and containing ∼39 mass% of iodine. |
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| AbstractList | A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO sub(2)-based waste form makes silver-functionalized silica aerogel (Ag super(0)-aerogel) an attractive choice for the removal and sequestration of iodine compounds from the off-gas of a nuclear fuel reprocessing plant. Hot uniaxial pressing of iodine-loaded Ag super(0)-aerogel (20.2 mass% iodine) at 1200 degree C for 30 min under 29 MPa pressure provided a partially sintered product with residual open porosity of 16.9% that retained similar to 93% of sorbed iodine. Highly iodine-loaded Ag super(0)-aerogel was successfully consolidated by hot isostatic pressing at 1200 degree C with a 30-min hold and under 207 MPa. The fully densified waste form had a bulk density of 3.3 10 super(3) kg/m super(3) and contained similar to 39 mass% iodine. The iodine was retained in the form of nano- and micro-particles of AgI that were uniformly distributed inside and along boundaries of fused silica grains. A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO2-based waste form makes silver-functionalized silica aerogel (Ag0-aerogel) an attractive choice for the removal and sequestration of iodine compounds from the off-gas of a nuclear fuel reprocessing plant. Hot uniaxial pressing of iodine-loaded Ag0-aerogel (20.2 mass% iodine) at 1200°C for 30 min under 29 MPa pressure provided a partially sintered product with residual open porosity of 16.9% that retained ~93% of sorbed iodine. Highly iodine-loaded Ag0-aerogel was successfully consolidated by hot isostatic pressing at 1200°C with a 30-min hold and under 207 MPa. The fully densified waste form had a bulk density of 3.3 g/cm3 and contained ~39 mass% iodine. The iodine was retained in the form of nano- and micro-particles of AgI that were uniformly distributed inside and along boundaries of fused silica grains. A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO2-based waste form makes silver-functionalized silica aerogel (Ag0-aerogel) an attractive choice for the removal and sequestration of iodine compounds from the off-gas of a nuclear fuel reprocessing plant. Hot uniaxial pressing of iodine-loaded Ag0-aerogel (20.2 mass% iodine) at 1200 °C for 30 min under 29 MPa pressure provided a partially sintered product with residual open porosity of 16.9% that retained ∼93% of sorbed iodine. Highly iodine-loaded Ag0-aerogel was successfully consolidated by hot isostatic pressing at 1200 °C with a 30-min hold and under 207 MPa. The fully densified waste form had a bulk density of 3.3 × 103 kg/m3 and contained ∼39 mass% iodine. The iodine was retained in the form of nano- and micro-particles of AgI that were uniformly distributed inside and along boundaries of fused silica grains. [Display omitted] •Silver-functionalized silica aerogel is an effective sorbent and a viable waste form for iodine.•Simultaneous application of fast heating rates and high pressures produced a fully dense product.•HIPing produced a fully consolidated waste form with a bulk density of 3.3 × 103 kg/m3 and containing ∼39 mass% of iodine. |
| Author | Canfield, Nathan Matyáš, Josef Sulaiman, Sannoh Zumhoff, Mac |
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| Snippet | A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO2-based waste form makes silver-functionalized silica aerogel... A high selectivity and sorption capacity for iodine and a feasible consolidation to a durable SiO sub(2)-based waste form makes silver-functionalized silica... |
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| SubjectTerms | Consolidation Durability Hot isostatic pressing Hot uniaxial pressing Immobilization Iodine Nanostructure Reprocessing Silica-based waste form Silicon dioxide Silver-functionalized silica aerogel Sorption Wastes |
| Title | Silica-based waste form for immobilization of iodine from reprocessing plant off-gas streams |
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