An inward and outward natural gas hydrates growth shell model considering intrinsic kinetics, mass and heat transfer

► The natural gas hydrates formation and growth were studied in the flow loop at three water cuts. ► The gas consumption value increased with increment of water cut. ► The total water conversion rates depended on water cut, amount of dissolved gas and surface/volume ratio of particles. ► An inward a...

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Published in	Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 171; no. 3; pp. 1308 - 1316
Main Authors	Shi, Bo-Hui, Gong, Jing, Sun, Chang-Yu, Zhao, Jian-Kui, Ding, Yao, Chen, Guang-Jin
Format	Journal Article
Language	English
Published	Oxford Elsevier B.V 15.07.2011 Elsevier
Subjects	Applied sciences Chemical engineering Conversion Diffusion emulsions Exact sciences and technology Fluid flows Heat and mass transfer. Packings, plates Heat transfer Hydrates Kinetics Mass transfer Natural gas Natural gas hydrates oils Shells Water consumption Natural gas hydrates Kinetics Diffusion Mass transfer Heat transfer Fluid flows Conversion rate Modeling Emulsion Dissolved gas Water consumption Gas hydrates Natural gas
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Abstract	► The natural gas hydrates formation and growth were studied in the flow loop at three water cuts. ► The gas consumption value increased with increment of water cut. ► The total water conversion rates depended on water cut, amount of dissolved gas and surface/volume ratio of particles. ► An inward and outward natural gas hydrates growth shell model was proposed, considered intrinsic kinetics, mass and heat transfer. ► The simulated results fitted the experimental data well. The natural gas hydrates formation and growth at 2 MPa and 277.15 K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop unit. The variations of gas consumption with time at different water cuts were obtained. The experimental results showed that the gas consumption value increased with the rise of water cut. The total water conversion rates not only depended on the water cuts, but also related to several other factors, two of which were the amount of the dissolved gas and the surface/volume ratio of the particles. No more natural gas transformed into hydrates after 3 h, which was likely caused by intrinsic kinetics, mass transfer and heat transfer limitations. An inward and outward natural gas hydrates growth shell model was proposed considering all the three limitations to simulate the gas and water consumptions to form natural gas hydrates.
AbstractList	► The natural gas hydrates formation and growth were studied in the flow loop at three water cuts. ► The gas consumption value increased with increment of water cut. ► The total water conversion rates depended on water cut, amount of dissolved gas and surface/volume ratio of particles. ► An inward and outward natural gas hydrates growth shell model was proposed, considered intrinsic kinetics, mass and heat transfer. ► The simulated results fitted the experimental data well. The natural gas hydrates formation and growth at 2 MPa and 277.15 K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop unit. The variations of gas consumption with time at different water cuts were obtained. The experimental results showed that the gas consumption value increased with the rise of water cut. The total water conversion rates not only depended on the water cuts, but also related to several other factors, two of which were the amount of the dissolved gas and the surface/volume ratio of the particles. No more natural gas transformed into hydrates after 3 h, which was likely caused by intrinsic kinetics, mass transfer and heat transfer limitations. An inward and outward natural gas hydrates growth shell model was proposed considering all the three limitations to simulate the gas and water consumptions to form natural gas hydrates. The natural gas hydrates formation and growth at 2 MPa and 277.15 K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop unit. The variations of gas consumption with time at different water cuts were obtained. The experimental results showed that the gas consumption value increased with the rise of water cut. The total water conversion rates not only depended on the water cuts, but also related to several other factors, two of which were the amount of the dissolved gas and the surface/volume ratio of the particles. No more natural gas transformed into hydrates after 3 h, which was likely caused by intrinsic kinetics, mass transfer and heat transfer limitations. An inward and outward natural gas hydrates growth shell model was proposed considering all the three limitations to simulate the gas and water consumptions to form natural gas hydrates. The natural gas hydrates formation and growth at 2MPa and 277.15K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop unit. The variations of gas consumption with time at different water cuts were obtained. The experimental results showed that the gas consumption value increased with the rise of water cut. The total water conversion rates not only depended on the water cuts, but also related to several other factors, two of which were the amount of the dissolved gas and the surface/volume ratio of the particles. No more natural gas transformed into hydrates after 3h, which was likely caused by intrinsic kinetics, mass transfer and heat transfer limitations. An inward and outward natural gas hydrates growth shell model was proposed considering all the three limitations to simulate the gas and water consumptions to form natural gas hydrates.
Author	Ding, Yao Gong, Jing Sun, Chang-Yu Chen, Guang-Jin Shi, Bo-Hui Zhao, Jian-Kui
Author_xml	– sequence: 1 givenname: Bo-Hui surname: Shi fullname: Shi, Bo-Hui organization: Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, Department of Oil & Gas Storage and Transportation Engineering, China University of Petroleum, Beijing 102249, China – sequence: 2 givenname: Jing surname: Gong fullname: Gong, Jing email: ydgj@cup.edu.cn organization: Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, Department of Oil & Gas Storage and Transportation Engineering, China University of Petroleum, Beijing 102249, China – sequence: 3 givenname: Chang-Yu surname: Sun fullname: Sun, Chang-Yu email: cysun@cup.edu.cn organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China – sequence: 4 givenname: Jian-Kui surname: Zhao fullname: Zhao, Jian-Kui organization: Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, Department of Oil & Gas Storage and Transportation Engineering, China University of Petroleum, Beijing 102249, China – sequence: 5 givenname: Yao surname: Ding fullname: Ding, Yao organization: Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, Department of Oil & Gas Storage and Transportation Engineering, China University of Petroleum, Beijing 102249, China – sequence: 6 givenname: Guang-Jin surname: Chen fullname: Chen, Guang-Jin organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China
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Snippet	► The natural gas hydrates formation and growth were studied in the flow loop at three water cuts. ► The gas consumption value increased with increment of... The natural gas hydrates formation and growth at 2MPa and 277.15K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop... The natural gas hydrates formation and growth at 2 MPa and 277.15 K were studied at different water cuts for water-in-condensate oil emulsions in the flow loop...
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SubjectTerms	Applied sciences Chemical engineering Conversion Diffusion emulsions Exact sciences and technology Fluid flows Heat and mass transfer. Packings, plates Heat transfer Hydrates Kinetics Mass transfer Natural gas Natural gas hydrates oils Shells Water consumption
Title	An inward and outward natural gas hydrates growth shell model considering intrinsic kinetics, mass and heat transfer
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