Evaluation through column leaching tests of metal release from contaminated estuarine sediment subject to CO2 leakages from Carbon Capture and Storage sites

The pH change and the release of organic matter and metals from sediment, due to the potential CO2 acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent...

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Published inEnvironmental pollution (1987) Vol. 171; pp. 174 - 184
Main Authors Payán, M. Cruz, Galan, Berta, Coz, Alberto, Vandecasteele, Carlo, Viguri, Javier R.
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier Ltd 01.12.2012
Elsevier
Subjects
acidification
analysis
Applied sciences
arsenic
Biological and physicochemical properties of pollutants. Interaction in the soil
cadmium
carbon
carbon dioxide
Carbon Dioxide - analysis
Carbon Dioxide - chemistry
Carbon Sequestration
chemistry
chromium
climate change
Climatology. Bioclimatology. Climate change
CO2 leakage
CO2-acidified seawater
Column leaching tests
copper
dissolved organic carbon
Earth sciences
Earth, ocean, space
Engineering and environment geology. Geothermics
Environmental Monitoring
Estuaries
Exact sciences and technology
External geophysics
Geologic Sediments
Geologic Sediments - chemistry
Hydrogen-Ion Concentration
leaching
lead
Metal release
Metals
Metals - analysis
Metals - chemistry
Meteorology
Models, Chemical
neutralization
nickel
Pollution
Pollution, environment geology
Risk Assessment
seawater
Seawater - chemistry
Sediment
sediments
Soil and sediments pollution
Spain
Water Pollutants, Chemical
Water Pollutants, Chemical - analysis
Water Pollutants, Chemical - chemistry
zinc
Spain
CO2 leakage
Sediment
CO2-acidified seawater
Column leaching tests
Metal release
heavy metals
Carbon dioxide
acidification
greenhouse gas
environment impact
trace elements
lixiviation
estuaries
acidified seawater
climate change
sea water
Sediment water interaction
Pollutant behavior
CO2 sequestration
Geological formation
arsenic
CO
Carbon sequestration
sustainable development
Mitigation
Carcinogen
Geoengineering
Poison
leakage
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Abstract The pH change and the release of organic matter and metals from sediment, due to the potential CO2 acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied. ► Tier structured approach for assessment of the release of metals from sediment. ► Standard column leaching test to simulate CO2 acidified seawater CCS leakages. ► Metal and DOC release from marine sediment in contact to CO2 acidified seawater. ► From empirical to geochemical modeling approaches of DOC and metals release in column tests. ► Contamination line of evidence input of CCS risk assessment. Column metal release from CO2 acidified seawater leakages in contact with estuarine contaminated sediment in CCS sites
AbstractList The pH change and the release of organic matter and metals from sediment, due to the potential CO(2) acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied.
The pH change and the release of organic matter and metals from sediment, due to the potential CO₂ acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied.
The pH change and the release of organic matter and metals from sediment, due to the potential CO2 acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied. ► Tier structured approach for assessment of the release of metals from sediment. ► Standard column leaching test to simulate CO2 acidified seawater CCS leakages. ► Metal and DOC release from marine sediment in contact to CO2 acidified seawater. ► From empirical to geochemical modeling approaches of DOC and metals release in column tests. ► Contamination line of evidence input of CCS risk assessment. Column metal release from CO2 acidified seawater leakages in contact with estuarine contaminated sediment in CCS sites
The pH change and the release of organic matter and metals from sediment, due to the potential CO(2) acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied.The pH change and the release of organic matter and metals from sediment, due to the potential CO(2) acidified seawater leakages from a CCS (Carbon Capture and Storage) site are presented. Column leaching test is used to simulate a scenario where a flow of acidified seawater is in contact with recent contaminated sediment. The behavior of pH, dissolved organic carbon (DOC) and metals As, Cd, Cr, Cu, Ni, Pb, Zn, with liquid to solid (L/S) ratio and pH is analyzed. A stepwise strategy using empirical expressions and a geochemical model was conducted to fit experimental release concentrations. Despite the neutralization capacity of the seawater-carbonate rich sediment system, important acidification and releases are expected at local scale at lower pH. The obtained results would be relevant as a line of evidence input of CCS risk assessment, in an International context where strategies to mitigate the climate change would be applied.
Author Coz, Alberto
Vandecasteele, Carlo
Viguri, Javier R.
Payán, M. Cruz
Galan, Berta
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  surname: Payán
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  email: vigurij@unican.es
  organization: Department of Chemical Engineering and Inorganic Chemistry, ETSIIT, University of Cantabria, Avda. de los Castros s/n, 39005 Santander, Spain
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Keywords CO2 leakage
Sediment
CO2-acidified seawater
Column leaching tests
Metal release
heavy metals
Carbon dioxide
acidification
greenhouse gas
environment impact
trace elements
lixiviation
estuaries
acidified seawater
climate change
sea water
Sediment water interaction
Pollutant behavior
CO2 sequestration
Geological formation
arsenic
CO
Carbon sequestration
sustainable development
Mitigation
Carcinogen
Geoengineering
Poison
leakage
Language English
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Snippet The pH change and the release of organic matter and metals from sediment, due to the potential CO2 acidified seawater leakages from a CCS (Carbon Capture and...
The pH change and the release of organic matter and metals from sediment, due to the potential CO₂ acidified seawater leakages from a CCS (Carbon Capture and...
The pH change and the release of organic matter and metals from sediment, due to the potential CO(2) acidified seawater leakages from a CCS (Carbon Capture and...
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StartPage 174
SubjectTerms acidification
analysis
Applied sciences
arsenic
Biological and physicochemical properties of pollutants. Interaction in the soil
cadmium
carbon
carbon dioxide
Carbon Dioxide - analysis
Carbon Dioxide - chemistry
Carbon Sequestration
chemistry
chromium
climate change
Climatology. Bioclimatology. Climate change
CO2 leakage
CO2-acidified seawater
Column leaching tests
copper
dissolved organic carbon
Earth sciences
Earth, ocean, space
Engineering and environment geology. Geothermics
Environmental Monitoring
Estuaries
Exact sciences and technology
External geophysics
Geologic Sediments
Geologic Sediments - chemistry
Hydrogen-Ion Concentration
leaching
lead
Metal release
Metals
Metals - analysis
Metals - chemistry
Meteorology
Models, Chemical
neutralization
nickel
Pollution
Pollution, environment geology
Risk Assessment
seawater
Seawater - chemistry
Sediment
sediments
Soil and sediments pollution
Spain
Water Pollutants, Chemical
Water Pollutants, Chemical - analysis
Water Pollutants, Chemical - chemistry
zinc
Title Evaluation through column leaching tests of metal release from contaminated estuarine sediment subject to CO2 leakages from Carbon Capture and Storage sites
URI https://dx.doi.org/10.1016/j.envpol.2012.07.029
https://www.ncbi.nlm.nih.gov/pubmed/22926654
https://www.proquest.com/docview/1074764869
https://www.proquest.com/docview/1663592202
Volume 171
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