Powering up the Future: Radical Polymers for Battery Applications

Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals...

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Published in	Advanced materials (Weinheim) Vol. 24; no. 48; pp. 6397 - 6409
Main Authors	Janoschka, Tobias, Hager, Martin D., Schubert, Ulrich S.
Format	Journal Article
Language	English
Published	Weinheim WILEY-VCH Verlag 18.12.2012 WILEY‐VCH Verlag
Subjects	Electric Power Supplies Electrochemical Techniques Electrodes Free Radicals - chemical synthesis Free Radicals - chemistry green batteries Li-ion battery Nitrogen Oxides - chemical synthesis Nitrogen Oxides - chemistry organic radical battery polymer battery Polymers - chemical synthesis Polymers - chemistry rechargeable batteries
Online Access	Get full text
ISSN	0935-9648 1521-4095 1521-4095
DOI	10.1002/adma.201203119

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Abstract	Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance. For over a hundred years, rechargeable batteries have facilitated the evolution from a mains‐operated to a mobile society. During this process, our society's dependency on limited resources such as lithium, cobalt, and rare earth metals grew steadily. With the recent development of electroactive nitroxide‐radical‐bearing polymers, a new and seminal class of electrode material is evolving quickly.
AbstractList	Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance. For over a hundred years, rechargeable batteries have facilitated the evolution from a mains‐operated to a mobile society. During this process, our society's dependency on limited resources such as lithium, cobalt, and rare earth metals grew steadily. With the recent development of electroactive nitroxide‐radical‐bearing polymers, a new and seminal class of electrode material is evolving quickly. Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance. Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance. Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance.Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will eventually culminate in resource wars on limited commodities like lithium, cobalt, and rare earth metals. The substitution of conventional metals as means of electric charge storage by organic and polymeric materials, which may ultimately be derived from renewable resources, appears to be the only feasible way out. In this context, the novel class of organic radical batteries (ORBs) excelling in rate capability (i.e., charging speed) and cycling stability (>1000 cycles) sets new standards in battery research. This review examines stable nitroxide radical bearing polymers, their processing to battery systems, and their promising performance.
Author	Schubert, Ulrich S. Hager, Martin D. Janoschka, Tobias
Author_xml	– sequence: 1 givenname: Tobias surname: Janoschka fullname: Janoschka, Tobias organization: Laboratory of Organic and Macromolecular Chemistry (IOMC), Friedrich-Schiller-University Jena, Humboldtstr. 10, D-07743 Jena, Germany – sequence: 2 givenname: Martin D. surname: Hager fullname: Hager, Martin D. organization: Laboratory of Organic and Macromolecular Chemistry (IOMC), Friedrich-Schiller-University Jena, Humboldtstr. 10, D-07743 Jena, Germany – sequence: 3 givenname: Ulrich S. surname: Schubert fullname: Schubert, Ulrich S. email: ulrich.schubert@uni-jena.de organization: Laboratory of Organic and Macromolecular Chemistry (IOMC), Friedrich-Schiller-University Jena, Humboldtstr. 10, D-07743 Jena, Germany
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/23238940$$D View this record in MEDLINE/PubMed
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Snippet	Our society's dependency on portable electric energy, i.e., rechargeable batteries, which permit power consumption at any place and in any time, will...
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SubjectTerms	Electric Power Supplies Electrochemical Techniques Electrodes Free Radicals - chemical synthesis Free Radicals - chemistry green batteries Li-ion battery Nitrogen Oxides - chemical synthesis Nitrogen Oxides - chemistry organic radical battery polymer battery Polymers - chemical synthesis Polymers - chemistry rechargeable batteries
Title	Powering up the Future: Radical Polymers for Battery Applications
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