Ferroelectricity in a one-dimensional organic quantum magnet
In magnetically controllable ferroelectrics, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy associated with both the magnetic order and interaction of spins with an applied magnetic field. Conventional approaches to designing materi...
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| Published in | Nature physics Vol. 6; no. 3; pp. 169 - 172 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.03.2010
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | In magnetically controllable ferroelectrics, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy associated with both the magnetic order and interaction of spins with an applied magnetic field. Conventional approaches to designing materials that exploit such spin-mediated behaviour have focused mainly on developing the cycloidal spin order, and thereby producing ferroelectric behaviour through the so-called antisymmetric Dzyaloshinskii-Moriya interaction. However, engineering such spin structures is challenging. Here we suggest a different approach. Direct measurements of magnetic-field-dependent variations in the polarization of the one-dimensional organic quantum magnet, tetrathiafulvalene-p-bromanil, suggest a spin-Peierls instability has an important role in its response. Our results imply that one-dimensional quantum magnets, such as organic charge-transfer complexes, could be promising candidates in the development of magnetically controllable ferroelectric materials. |
|---|---|
| AbstractList | Measurements of the magnetic-field-dependent polarization of a one-dimensional organic quantum magnet suggest its ferroelectric behaviour is mediated by a spin–Peierls instability. Such behaviour could provide a promising new approach to the design of spin-driven ferroelectrics.
In magnetically controllable ferroelectrics
1
,
2
,
3
, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy associated with both the magnetic order and interaction of spins with an applied magnetic field. Conventional approaches to designing materials that exploit such spin-mediated behaviour have focused mainly on developing the cycloidal spin order
4
,
5
, and thereby producing ferroelectric behaviour through the so-called antisymmetric Dzyaloshinskii–Moriya interaction
6
,
7
,
8
. However, engineering such spin structures is challenging. Here we suggest a different approach. Direct measurements of magnetic-field-dependent variations in the polarization of the one-dimensional organic quantum magnet, tetrathiafulvalene-
p
-bromanil, suggest a spin–Peierls instability has an important role in its response. Our results imply that one-dimensional quantum magnets, such as organic charge-transfer complexes, could be promising candidates in the development of magnetically controllable ferroelectric materials. In magnetically controllable ferroelectrics, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy associated with both the magnetic order and interaction of spins with an applied magnetic field. Conventional approaches to designing materials that exploit such spin-mediated behaviour have focused mainly on developing the cycloidal spin order, and thereby producing ferroelectric behaviour through the so-called antisymmetric Dzyaloshinskii-Moriya interaction. However, engineering such spin structures is challenging. Here we suggest a different approach. Direct measurements of magnetic-field-dependent variations in the polarization of the one-dimensional organic quantum magnet, tetrathiafulvalene-p-bromanil, suggest a spin-Peierls instability has an important role in its response. Our results imply that one-dimensional quantum magnets, such as organic charge-transfer complexes, could be promising candidates in the development of magnetically controllable ferroelectric materials. In magnetically controllable ferroelectrics1-3, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy associated with both the magnetic order and interaction of spins with an applied magnetic field. Conventional approaches to designing materials that exploit such spin-mediated behaviour have focused mainly on developing the cycloidal spin order4,5, and thereby producing ferroelectric behaviour through the so-called antisymmetric Dzyaloshinskii-Moriya interaction6-8. However, engineering such spin structures is challenging. Here we suggest a different approach. Direct measurements of magnetic-field-dependent variations in the polarization of the one-dimensional organic quantum magnet, tetrathiafulvalene-p-bromanil, suggest a spin-Peierls instability has an important role in its response. Our results imply that one-dimensional quantum magnets, such as organic charge-transfer complexes, could be promising candidates in the development of magnetically controllable ferroelectric materials. [PUBLICATION ABSTRACT] |
| Author | Fujioka, Jun Horiuchi, Sachio Kagawa, Fumitaka Tokunaga, Masashi Tokura, Yoshinori |
| Author_xml | – sequence: 1 givenname: Fumitaka surname: Kagawa fullname: Kagawa, Fumitaka organization: Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics, University of Tokyo – sequence: 2 givenname: Sachio surname: Horiuchi fullname: Horiuchi, Sachio organization: National Institute of Advanced Industrial Science and Technology (AIST) – sequence: 3 givenname: Masashi surname: Tokunaga fullname: Tokunaga, Masashi organization: Institute for Solid State Physics, University of Tokyo – sequence: 4 givenname: Jun surname: Fujioka fullname: Fujioka, Jun organization: Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics, University of Tokyo – sequence: 5 givenname: Yoshinori surname: Tokura fullname: Tokura, Yoshinori organization: Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics, University of Tokyo National Institute of Advanced Industrial Science and Technology (AIST) Department of Applied Physics, University of Tokyo Cross-Correlated Materials Research Group (CMRG), RIKEN, Advanced Science Institute |
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| Copyright | Springer Nature Limited 2010 Copyright Nature Publishing Group Mar 2010 |
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| DOI | 10.1038/nphys1503 |
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| Snippet | In magnetically controllable ferroelectrics, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the energy... Measurements of the magnetic-field-dependent polarization of a one-dimensional organic quantum magnet suggest its ferroelectric behaviour is mediated by a... In magnetically controllable ferroelectrics1-3, electric polarization is induced by charge redistribution or lattice distortions that occur to minimize the... |
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| SubjectTerms | Atomic Classical and Continuum Physics Complex Systems Condensed Matter Physics Ferroelectrics letter Magnetic fields Mathematical and Computational Physics Molecular Optical and Plasma Physics Physics Physics and Astronomy Polarization Quantum physics Theoretical |
| Title | Ferroelectricity in a one-dimensional organic quantum magnet |
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