Review-Localized High-Concentration Electrolytes for Lithium Batteries
The conventional LiPF6/carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years because a stable solid electrolyte interphase (SEI) layer forms on the graphite surface and enables its long-term cycling stability. However, few...
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| Published in | Journal of the Electrochemical Society Vol. 168; no. 1; pp. 10522 - 10534 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
IOP Publishing
01.01.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The conventional LiPF6/carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years because a stable solid electrolyte interphase (SEI) layer forms on the graphite surface and enables its long-term cycling stability. However, few of these electrolytes are stable under the more stringent conditions needed with a Li metal anode (LMA) and other anodes, such as silicon (Si), which exhibit large volume changes during charge/discharge processes. Many different approaches have been developed lately to stabilize Li metal batteries (LMBs) and Si-based LIBs. From this aspect, localized high-concentration electrolytes (LHCEs) have unique advantages: not only are they stable in a wide electrochemical window, they can also form stable SEI layers on LMA and Si anode surfaces to enable their long-term cycling stability. The ultrathin SEI layer formed on a Gr anode can also improve the safety and high-rate operation of conventional LIBs. In this paper, we give a brief summary of our recent work on LHCEs, including their design principle and applications in both LMBs and LIBs. A perspective on the future development of LHCEs is also discussed. |
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| AbstractList | The conventional LiPF6/carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years because a stable solid electrolyte interphase (SEI) layer forms on the graphite surface and enables its long-term cycling stability. However, few of these electrolytes are stable under the more stringent conditions needed with a Li metal anode (LMA) and other anodes, such as silicon (Si), which exhibit large volume changes during charge/discharge processes. Many different approaches have been developed lately to stabilize Li metal batteries (LMBs) and Si-based LIBs. From this aspect, localized high-concentration electrolytes (LHCEs) have unique advantages: not only are they stable in a wide electrochemical window, they can also form stable SEI layers on LMA and Si anode surfaces to enable their long-term cycling stability. The ultrathin SEI layer formed on a Gr anode can also improve the safety and high-rate operation of conventional LIBs. In this paper, we give a brief summary of our recent work on LHCEs, including their design principle and applications in both LMBs and LIBs. A perspective on the future development of LHCEs is also discussed. The conventional LiPF 6 /carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years because a stable solid electrolyte interphase (SEI) layer forms on the graphite surface and enables its long-term cycling stability. However, few of these electrolytes are stable under the more stringent conditions needed with a Li metal anode (LMA) and other anodes, such as silicon (Si), which exhibit large volume changes during charge/discharge processes. Many different approaches have been developed lately to stabilize Li metal batteries (LMBs) and Si-based LIBs. From this aspect, localized high-concentration electrolytes (LHCEs) have unique advantages: not only are they stable in a wide electrochemical window, they can also form stable SEI layers on LMA and Si anode surfaces to enable their long-term cycling stability. The ultrathin SEI layer formed on a Gr anode can also improve the safety and high-rate operation of conventional LIBs. In this paper, we give a brief summary of our recent work on LHCEs, including their design principle and applications in both LMBs and LIBs. A perspective on the future development of LHCEs is also discussed. |
| Author | Xu, Wu Zhang, Ji-Guang Cao, Xia Jia, Hao |
| Author_xml | – sequence: 1 givenname: Xia orcidid: 0000-0003-1610-4341 surname: Cao fullname: Cao, Xia organization: Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, United States of America – sequence: 2 givenname: Hao orcidid: 0000-0003-2814-5589 surname: Jia fullname: Jia, Hao organization: Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, United States of America – sequence: 3 givenname: Wu orcidid: 0000-0002-2685-8684 surname: Xu fullname: Xu, Wu organization: Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, United States of America – sequence: 4 givenname: Ji-Guang orcidid: 0000-0001-7343-4609 surname: Zhang fullname: Zhang, Ji-Guang email: jiguang.zhang@pnnl.gov organization: Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, United States of America |
| BackLink | https://www.osti.gov/biblio/1760040$$D View this record in Osti.gov |
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| CODEN | JESOAN |
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| Snippet | The conventional LiPF6/carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years... The conventional LiPF 6 /carbonate-based electrolytes have been widely used in graphite (Gr)-based lithium (Li) ion batteries (LIBs) for more than 30 years... |
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| SubjectTerms | ENERGY STORAGE graphite lithium metal localized high-concentration electrolytes Silicon solid electrolyte interphase |
| Title | Review-Localized High-Concentration Electrolytes for Lithium Batteries |
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