Large-area high-quality 2D ultrathin Mo2C superconducting crystals
Transition metal carbides (TMCs) are a large family of materials with many intriguing properties and applications, and high-quality 2D TMCs are essential for investigating new physics and properties in the 2D limit. However, the 2D TMCs obtained so far are chemically functionalized, defective nanosh...
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| Published in | Nature materials Vol. 14; no. 11; pp. 1135 - 1141 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.11.2015
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Transition metal carbides (TMCs) are a large family of materials with many intriguing properties and applications, and high-quality 2D TMCs are essential for investigating new physics and properties in the 2D limit. However, the 2D TMCs obtained so far are chemically functionalized, defective nanosheets having maximum lateral dimensions of ∼10 μm. Here we report the fabrication of large-area high-quality 2D ultrathin α-Mo
2
C crystals by chemical vapour deposition (CVD). The crystals are a few nanometres thick, over 100 μm in size, and very stable under ambient conditions. They show 2D characteristics of superconducting transitions that are consistent with Berezinskii–Kosterlitz–Thouless behaviour and show strong anisotropy with magnetic field orientation; moreover, the superconductivity is also strongly dependent on the crystal thickness. Our versatile CVD process allows the fabrication of other high-quality 2D TMC crystals, such as ultrathin WC and TaC crystals, which further expand the large family of 2D materials.
Chemical vapour deposition is used to grow stable, ultrathin crystals of α-Mo
2
C and other transition metal carbides with lateral size up to 100 μm. α-Mo
2
C shows a superconducting behaviour with 2D character, strongly dependent on the crystal thickness. |
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| AbstractList | Transition metal carbides (TMCs) are a large family of materials with many intriguing properties and applications, and high-quality 2D TMCs are essential for investigating new physics and properties in the 2D limit. However, the 2D TMCs obtained so far are chemically functionalized, defective nanosheets having maximum lateral dimensions of ∼10 μm. Here we report the fabrication of large-area high-quality 2D ultrathin α-Mo2C crystals by chemical vapour deposition (CVD). The crystals are a few nanometres thick, over 100 μm in size, and very stable under ambient conditions. They show 2D characteristics of superconducting transitions that are consistent with Berezinskii-Kosterlitz-Thouless behaviour and show strong anisotropy with magnetic field orientation; moreover, the superconductivity is also strongly dependent on the crystal thickness. Our versatile CVD process allows the fabrication of other high-quality 2D TMC crystals, such as ultrathin WC and TaC crystals, which further expand the large family of 2D materials. Transition metal carbides (TMCs) are a large family of materials with many intriguing properties and applications, and high-quality 2D TMCs are essential for investigating new physics and properties in the 2D limit. However, the 2D TMCs obtained so far are chemically functionalized, defective nanosheets having maximum lateral dimensions of 10 m. Here we report the fabrication of large-area high-quality 2D ultrathin -Mo2C crystals by chemical vapour deposition (CVD). The crystals are a few nanometres thick, over 100 m in size, and very stable under ambient conditions. They show 2D characteristics of superconducting transitions that are consistent with BerezinskiiKosterlitzThouless behaviour and show strong anisotropy with magnetic eld orientation; moreover, the superconductivity is also strongly dependent on the crystal thickness. Our versatile CVD process allows the fabrication of other high-quality 2D TMC crystals, such as ultrathin WC and TaC crystals, which further expand the large family of 2D materials. Transition metal carbides (TMCs) are a large family of materials with many intriguing properties and applications, and high-quality 2D TMCs are essential for investigating new physics and properties in the 2D limit. However, the 2D TMCs obtained so far are chemically functionalized, defective nanosheets having maximum lateral dimensions of ∼10 μm. Here we report the fabrication of large-area high-quality 2D ultrathin α-Mo 2 C crystals by chemical vapour deposition (CVD). The crystals are a few nanometres thick, over 100 μm in size, and very stable under ambient conditions. They show 2D characteristics of superconducting transitions that are consistent with Berezinskii–Kosterlitz–Thouless behaviour and show strong anisotropy with magnetic field orientation; moreover, the superconductivity is also strongly dependent on the crystal thickness. Our versatile CVD process allows the fabrication of other high-quality 2D TMC crystals, such as ultrathin WC and TaC crystals, which further expand the large family of 2D materials. Chemical vapour deposition is used to grow stable, ultrathin crystals of α-Mo 2 C and other transition metal carbides with lateral size up to 100 μm. α-Mo 2 C shows a superconducting behaviour with 2D character, strongly dependent on the crystal thickness. |
| Author | Xu, Chuan Guo, Jingkun Cheng, Hui-Ming Kang, Ning Ma, Xiu-Liang Liu, Zhibo Chen, Long Wang, Libin Ren, Wencai |
| Author_xml | – sequence: 1 givenname: Chuan surname: Xu fullname: Xu, Chuan organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences – sequence: 2 givenname: Libin surname: Wang fullname: Wang, Libin organization: Key Laboratory for the Physics and Chemistry of Nanodevices and Department of Electronics, Peking University – sequence: 3 givenname: Zhibo surname: Liu fullname: Liu, Zhibo organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences – sequence: 4 givenname: Long surname: Chen fullname: Chen, Long organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences – sequence: 5 givenname: Jingkun surname: Guo fullname: Guo, Jingkun organization: Key Laboratory for the Physics and Chemistry of Nanodevices and Department of Electronics, Peking University – sequence: 6 givenname: Ning surname: Kang fullname: Kang, Ning email: nkang@pku.edu.cn organization: Key Laboratory for the Physics and Chemistry of Nanodevices and Department of Electronics, Peking University – sequence: 7 givenname: Xiu-Liang surname: Ma fullname: Ma, Xiu-Liang organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences – sequence: 8 givenname: Hui-Ming surname: Cheng fullname: Cheng, Hui-Ming organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences – sequence: 9 givenname: Wencai surname: Ren fullname: Ren, Wencai email: wcren@imr.ac.cn organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26280223$$D View this record in MEDLINE/PubMed |
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| Title | Large-area high-quality 2D ultrathin Mo2C superconducting crystals |
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