Wide frequency range diagnostic impedance behavior of the multiple interfaces charge transport and transfer processes in dye-sensitized solar cells

► Model the interaction among multiple interface processes of charge transport and transfer in DSC with wide frequency range. ► Diagnostic changes of impedance behavior over a wide range of changing conditions in DSC. ► The TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance can al...

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Published in	Electrochimica acta Vol. 88; pp. 395 - 403
Main Authors	LIU, Wei-Qing, LIANG, Zhong-Guan, KOU, Dong-Xing, HU, Lin-Hua, DAI, Song-Yuan
Format	Journal Article
Language	English
Published	Kidlington Elsevier Ltd 15.01.2013 Elsevier
Subjects	Applied sciences Channels Charge transfer Charge transport Chemistry Differential scanning calorimetry Dye-sensitized Electrochemistry Electrolytic cells Energy Exact sciences and technology General and physical chemistry Impedance Multiple interfaces Natural energy Photovoltaic conversion Solar cells Solar cells. Photoelectrochemical cells Solar energy Titanium dioxide Solar cells Dye-sensitized Multiple interfaces Impedance Dye-sensitized solar cell Frequency range Dyes Solar cell Transport process Diagnosis Charge transfer Interface Electrical impedance
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Abstract	► Model the interaction among multiple interface processes of charge transport and transfer in DSC with wide frequency range. ► Diagnostic changes of impedance behavior over a wide range of changing conditions in DSC. ► The TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance can also influence the overall impedance characteristics of DSC under certain circumstances. The special “sandwich” structure of dye-sensitized solar cells (DSC) provides multiple electron transfer interfaces and two charge transport channels inside the cell. Some processes that take place on such interfaces have generally been left unnoticed when electrochemical impedance spectroscopy was used to study charge transfer process on these interfaces and charge transport process in these channels. In this paper, by dramatically varying the values of parameters of the impedance components of a DSC full-interface equivalent circuit containing 4 interfaces and 2 layers, we have studied the interaction between the charge interface transfer impedance and transport impedance and its effect on the overall impedance of the cell. We have also conducted a detailed study of the impedance characteristics of the internal charge transport, transfer, and collection processes of DSC. The results show that some previously ignored interfaces, such as the TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance in the electrolyte solution, can also influence the overall impedance characteristics of DSC under certain circumstances.
AbstractList	The special asandwicha structure of dye-sensitized solar cells (DSC) provides multiple electron transfer interfaces and two charge transport channels inside the cell. Some processes that take place on such interfaces have generally been left unnoticed when electrochemical impedance spectroscopy was used to study charge transfer process on these interfaces and charge transport process in these channels. In this paper, by dramatically varying the values of parameters of the impedance components of a DSC full-interface equivalent circuit containing 4 interfaces and 2 layers, we have studied the interaction between the charge interface transfer impedance and transport impedance and its effect on the overall impedance of the cell. We have also conducted a detailed study of the impedance characteristics of the internal charge transport, transfer, and collection processes of DSC. The results show that some previously ignored interfaces, such as the TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance in the electrolyte solution, can also influence the overall impedance characteristics of DSC under certain circumstances. ► Model the interaction among multiple interface processes of charge transport and transfer in DSC with wide frequency range. ► Diagnostic changes of impedance behavior over a wide range of changing conditions in DSC. ► The TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance can also influence the overall impedance characteristics of DSC under certain circumstances. The special “sandwich” structure of dye-sensitized solar cells (DSC) provides multiple electron transfer interfaces and two charge transport channels inside the cell. Some processes that take place on such interfaces have generally been left unnoticed when electrochemical impedance spectroscopy was used to study charge transfer process on these interfaces and charge transport process in these channels. In this paper, by dramatically varying the values of parameters of the impedance components of a DSC full-interface equivalent circuit containing 4 interfaces and 2 layers, we have studied the interaction between the charge interface transfer impedance and transport impedance and its effect on the overall impedance of the cell. We have also conducted a detailed study of the impedance characteristics of the internal charge transport, transfer, and collection processes of DSC. The results show that some previously ignored interfaces, such as the TCO/TiO2 and TCO/EL interfaces, as well as Nernst diffusion impedance in the electrolyte solution, can also influence the overall impedance characteristics of DSC under certain circumstances.
Author	Wei-Qing, Liu Dong-Xing, Kou Song-Yuan, Dai Zhong-Guan, Liang Lin-Hua, Hu
Author_xml	– sequence: 1 givenname: Wei-Qing surname: LIU fullname: LIU, Wei-Qing organization: Key Laboratory of Novel Thin Film Solar cells, Institute of Plasma Physics, Chinese Academy of science, Hefei 230031, China – sequence: 2 givenname: Zhong-Guan surname: LIANG fullname: LIANG, Zhong-Guan organization: Key Laboratory of Nondestructive Testing of Ministry of Education and School of the Testing and Photoeletric Enginering, Nanchang Hangkong University, Nanchang 330063, China – sequence: 3 givenname: Dong-Xing surname: KOU fullname: KOU, Dong-Xing organization: Key Laboratory of Novel Thin Film Solar cells, Institute of Plasma Physics, Chinese Academy of science, Hefei 230031, China – sequence: 4 givenname: Lin-Hua surname: HU fullname: HU, Lin-Hua organization: Key Laboratory of Novel Thin Film Solar cells, Institute of Plasma Physics, Chinese Academy of science, Hefei 230031, China – sequence: 5 givenname: Song-Yuan surname: DAI fullname: DAI, Song-Yuan organization: Key Laboratory of Novel Thin Film Solar cells, Institute of Plasma Physics, Chinese Academy of science, Hefei 230031, China
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Keywords	Solar cells Dye-sensitized Multiple interfaces Impedance Dye-sensitized solar cell Frequency range Dyes Solar cell Transport process Diagnosis Charge transfer Interface Electrical impedance
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Snippet	► Model the interaction among multiple interface processes of charge transport and transfer in DSC with wide frequency range. ► Diagnostic changes of impedance... The special asandwicha structure of dye-sensitized solar cells (DSC) provides multiple electron transfer interfaces and two charge transport channels inside...
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SubjectTerms	Applied sciences Channels Charge transfer Charge transport Chemistry Differential scanning calorimetry Dye-sensitized Electrochemistry Electrolytic cells Energy Exact sciences and technology General and physical chemistry Impedance Multiple interfaces Natural energy Photovoltaic conversion Solar cells Solar cells. Photoelectrochemical cells Solar energy Titanium dioxide
Title	Wide frequency range diagnostic impedance behavior of the multiple interfaces charge transport and transfer processes in dye-sensitized solar cells
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