Managing grains and interfaces via ligand anchoring enables 22.3%-efficiency inverted perovskite solar cells
Inverted perovskite solar cells have attracted increasing attention because they have achieved long operating lifetimes. However, they have exhibited significantly inferior power conversion efficiencies compared to regular perovskite solar cells. Here we reduce this efficiency gap using a trace amou...
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| Published in | Nature energy Vol. 5; no. 2; pp. 131 - 140 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.02.2020
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2058-7546 2058-7546 |
| DOI | 10.1038/s41560-019-0538-4 |
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| Abstract | Inverted perovskite solar cells have attracted increasing attention because they have achieved long operating lifetimes. However, they have exhibited significantly inferior power conversion efficiencies compared to regular perovskite solar cells. Here we reduce this efficiency gap using a trace amount of surface-anchoring alkylamine ligands (AALs) with different chain lengths as grain and interface modifiers. We show that long-chain AALs added to the precursor solution suppress nonradiative carrier recombination and improve the optoelectronic properties of mixed-cation mixed-halide perovskite films. The resulting AAL surface-modified films exhibit a prominent (100) orientation and lower trap-state density as well as enhanced carrier mobilities and diffusion lengths. These translate into a certified stabilized power conversion efficiency of 22.3% (23.0% power conversion efficiency for lab-measured champion devices). The devices operate for over 1,000 h at the maximum power point under simulated AM1.5 illumination, without loss of efficiency.
While perovskite solar cells with an inverted architecture hold great promise for operation stability, their power conversion efficiency lags behind that of conventional cells. Here, Zheng et al. achieve a certified 22.34% efficiency, exploiting alkylamine ligands as grain and interface modifiers. |
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| AbstractList | Inverted perovskite solar cells have attracted increasing attention because they have achieved long operating lifetimes. However, they have exhibited significantly inferior power conversion efficiencies compared to regular perovskite solar cells. Here we reduce this efficiency gap using a trace amount of surface-anchoring alkylamine ligands (AALs) with different chain lengths as grain and interface modifiers. We show that long-chain AALs added to the precursor solution suppress nonradiative carrier recombination and improve the optoelectronic properties of mixed-cation mixed-halide perovskite films. The resulting AAL surface-modified films exhibit a prominent (100) orientation and lower trap-state density as well as enhanced carrier mobilities and diffusion lengths. These translate into a certified stabilized power conversion efficiency of 22.3% (23.0% power conversion efficiency for lab-measured champion devices). The devices operate for over 1,000 h at the maximum power point under simulated AM1.5 illumination, without loss of efficiency. While perovskite solar cells with an inverted architecture hold great promise for operation stability, their power conversion efficiency lags behind that of conventional cells. Here, Zheng et al. achieve a certified 22.34% efficiency, exploiting alkylamine ligands as grain and interface modifiers. Inverted perovskite solar cells have attracted increasing attention because they have achieved long operating lifetimes. However, they have exhibited significantly inferior power conversion efficiencies compared to regular perovskite solar cells. Here we reduce this efficiency gap using a trace amount of surface-anchoring alkylamine ligands (AALs) with different chain lengths as grain and interface modifiers. We show that long-chain AALs added to the precursor solution suppress nonradiative carrier recombination and improve the optoelectronic properties of mixed-cation mixed-halide perovskite films. The resulting AAL surface-modified films exhibit a prominent (100) orientation and lower trap-state density as well as enhanced carrier mobilities and diffusion lengths. These translate into a certified stabilized power conversion efficiency of 22.3% (23.0% power conversion efficiency for lab-measured champion devices). The devices operate for over 1,000 h at the maximum power point under simulated AM1.5 illumination, without loss of efficiency. While perovskite solar cells with an inverted architecture hold great promise for operation stability, their power conversion efficiency lags behind that of conventional cells. Here, Zheng et al. achieve a certified 22.34% efficiency, exploiting alkylamine ligands as grain and interface modifiers. |
| Author | Lu, Zheng-Hong Song, Kepeng Wei, Nini Maity, Partha Han, Yu Yuan, Fanglong Bakr, Osman M. Zheng, Xiaopeng Mohammed, Omar F. Yang, Chen Alsalloum, Abdullah Y. Yin, Jun Xue, Ding-Jiang Baran, Derya Sargent, Edward H. Gao, Feng Liu, Jiakai Bao, Chunxiong Troughton, Joel Huang, Ziru Anthopoulos, Thomas D. Chen, Bin Turedi, Bekir Zhou, Chun Johnston, Andrew K. Hedhili, Mohamed Nejib Gasparini, Nicola Wei, Mingyang Hou, Yi Lin, Yuanbao |
| Author_xml | – sequence: 1 givenname: Xiaopeng orcidid: 0000-0001-5061-3655 surname: Zheng fullname: Zheng, Xiaopeng organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 2 givenname: Yi orcidid: 0000-0002-1532-816X surname: Hou fullname: Hou, Yi organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 3 givenname: Chunxiong orcidid: 0000-0001-7076-7635 surname: Bao fullname: Bao, Chunxiong organization: Department of Physics, Chemistry and Biology (IFM), Linköping University – sequence: 4 givenname: Jun orcidid: 0000-0002-1749-1120 surname: Yin fullname: Yin, Jun organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 5 givenname: Fanglong surname: Yuan fullname: Yuan, Fanglong organization: Department of Electrical and Computer Engineering, University of Toronto, Department of Materials Science and Engineering, University of Toronto – sequence: 6 givenname: Ziru orcidid: 0000-0001-7983-913X surname: Huang fullname: Huang, Ziru organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 7 givenname: Kepeng surname: Song fullname: Song, Kepeng organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 8 givenname: Jiakai surname: Liu fullname: Liu, Jiakai organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 9 givenname: Joel surname: Troughton fullname: Troughton, Joel organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 10 givenname: Nicola orcidid: 0000-0002-3226-8234 surname: Gasparini fullname: Gasparini, Nicola organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 11 givenname: Chun surname: Zhou fullname: Zhou, Chun organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 12 givenname: Yuanbao surname: Lin fullname: Lin, Yuanbao organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 13 givenname: Ding-Jiang surname: Xue fullname: Xue, Ding-Jiang organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 14 givenname: Bin surname: Chen fullname: Chen, Bin organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 15 givenname: Andrew K. orcidid: 0000-0002-4545-532X surname: Johnston fullname: Johnston, Andrew K. organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 16 givenname: Nini surname: Wei fullname: Wei, Nini organization: Imaging and Characterization Core Lab, King Abdullah University of Science and Technology (KAUST) – sequence: 17 givenname: Mohamed Nejib surname: Hedhili fullname: Hedhili, Mohamed Nejib organization: Imaging and Characterization Core Lab, King Abdullah University of Science and Technology (KAUST) – sequence: 18 givenname: Mingyang orcidid: 0000-0003-4820-2210 surname: Wei fullname: Wei, Mingyang organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 19 givenname: Abdullah Y. orcidid: 0000-0001-8988-1307 surname: Alsalloum fullname: Alsalloum, Abdullah Y. organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 20 givenname: Partha orcidid: 0000-0002-0293-7118 surname: Maity fullname: Maity, Partha organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 21 givenname: Bekir orcidid: 0000-0003-2208-0737 surname: Turedi fullname: Turedi, Bekir organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 22 givenname: Chen surname: Yang fullname: Yang, Chen organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 23 givenname: Derya orcidid: 0000-0003-2196-8187 surname: Baran fullname: Baran, Derya organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 24 givenname: Thomas D. orcidid: 0000-0002-0978-8813 surname: Anthopoulos fullname: Anthopoulos, Thomas D. organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 25 givenname: Yu orcidid: 0000-0003-1462-1118 surname: Han fullname: Han, Yu organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 26 givenname: Zheng-Hong surname: Lu fullname: Lu, Zheng-Hong organization: Department of Materials Science and Engineering, University of Toronto – sequence: 27 givenname: Omar F. surname: Mohammed fullname: Mohammed, Omar F. organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) – sequence: 28 givenname: Feng orcidid: 0000-0002-2582-1740 surname: Gao fullname: Gao, Feng organization: Department of Physics, Chemistry and Biology (IFM), Linköping University – sequence: 29 givenname: Edward H. orcidid: 0000-0003-0396-6495 surname: Sargent fullname: Sargent, Edward H. email: ted.sargent@utoronto.ca organization: Department of Electrical and Computer Engineering, University of Toronto – sequence: 30 givenname: Osman M. orcidid: 0000-0002-3428-1002 surname: Bakr fullname: Bakr, Osman M. email: osman.bakr@kaust.edu.sa organization: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST) |
| BackLink | https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-163633$$DView record from Swedish Publication Index |
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| Copyright | The Author(s), under exclusive licence to Springer Nature Limited 2020 2020© The Author(s), under exclusive licence to Springer Nature Limited 2020 The Author(s), under exclusive licence to Springer Nature Limited 2020. |
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| Snippet | Inverted perovskite solar cells have attracted increasing attention because they have achieved long operating lifetimes. However, they have exhibited... |
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| SubjectTerms | 639/301/299/946 639/4077/909/4101/4096 639/638/675 Alkylamines Carrier recombination Economics and Management Efficiency Energy Energy conversion efficiency Energy Policy Energy Storage Energy Systems Ligands Maximum power Optoelectronics Perovskites Photovoltaic cells Renewable and Green Energy Solar cells |
| Title | Managing grains and interfaces via ligand anchoring enables 22.3%-efficiency inverted perovskite solar cells |
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