Anion Exchange of Ni–Co Layered Double Hydroxide (LDH) Nanoarrays for a High‐Capacitance Supercapacitor Electrode: A Comparison of Alkali Anion Exchange and Sulfuration
A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO32− and OH− results in the construction of a reservoir for OH− anions, and the decoration of thin nano...
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| Published in | Chemistry : a European journal Vol. 24; no. 72; pp. 19309 - 19316 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Germany
20.12.2018
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| Subjects | |
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| Abstract | A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO32− and OH− results in the construction of a reservoir for OH− anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as‐soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm−2 (684 F g−1) to 6.22 F cm−2 (2391 F g−1) at 2 mA cm−2 after soaking for 12 h. Moreover, the soaked NiCo‐OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni–Co‐S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as‐assembled all‐solid‐state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg−1 at a power density of 1066 W kg−1.
Supercapacitor electrodes: Anion exchange is used to enhance the diffusion of OH− of layered double hydroxide (LDH) nanoarrays to achieve promising capacitive performance for supercapacitors (see figure). |
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| AbstractList | A facile and new anion exchange process is presented, which involves the conversion of NiCo-CO
layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO
and OH
results in the construction of a reservoir for OH
anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as-soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm
(684 F g
) to 6.22 F cm
(2391 F g
) at 2 mA cm
after soaking for 12 h. Moreover, the soaked NiCo-OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni-Co-S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as-assembled all-solid-state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg
at a power density of 1066 W kg
. A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO 3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO 3 2− and OH − results in the construction of a reservoir for OH − anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as‐soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm −2 (684 F g −1 ) to 6.22 F cm −2 (2391 F g −1 ) at 2 mA cm −2 after soaking for 12 h. Moreover, the soaked NiCo‐OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni–Co‐S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as‐assembled all‐solid‐state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg −1 at a power density of 1066 W kg −1 . A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO32− and OH− results in the construction of a reservoir for OH− anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as‐soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm−2 (684 F g−1) to 6.22 F cm−2 (2391 F g−1) at 2 mA cm−2 after soaking for 12 h. Moreover, the soaked NiCo‐OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni–Co‐S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as‐assembled all‐solid‐state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg−1 at a power density of 1066 W kg−1. Supercapacitor electrodes: Anion exchange is used to enhance the diffusion of OH− of layered double hydroxide (LDH) nanoarrays to achieve promising capacitive performance for supercapacitors (see figure). A facile and new anion exchange process is presented, which involves the conversion of NiCo-CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO3 2- and OH- results in the construction of a reservoir for OH- anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as-soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm-2 (684 F g-1 ) to 6.22 F cm-2 (2391 F g-1 ) at 2 mA cm-2 after soaking for 12 h. Moreover, the soaked NiCo-OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni-Co-S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as-assembled all-solid-state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg-1 at a power density of 1066 W kg-1 .A facile and new anion exchange process is presented, which involves the conversion of NiCo-CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline solution. The anion exchange between CO3 2- and OH- results in the construction of a reservoir for OH- anions, and the decoration of thin nanoflakes on the surface of nanosheets effectively enlarges the surface area of NiCo LDH nanoarrays. The capacitance of the as-soaked NiCo LDH nanoarrays electrode increases from 1.78 F cm-2 (684 F g-1 ) to 6.22 F cm-2 (2391 F g-1 ) at 2 mA cm-2 after soaking for 12 h. Moreover, the soaked NiCo-OH LDH electrode exhibits an enhanced rate capacity, high coulombic efficiency, and good cycling stability compared with the Ni-Co-S nanosheet electrode synthesized through a hydrothermal sulfuration process. The as-assembled all-solid-state NiCo LDH//active carbon asymmetric supercapacitor shows a maximum energy density of 83.4 W h kg-1 at a power density of 1066 W kg-1 . |
| Author | Ye, Qinglan Zou, Wenru Luo, Yunli Xu, Xuetang Guo, Wenxin Wang, Fan Liu, Xinyi |
| Author_xml | – sequence: 1 givenname: Wenru surname: Zou fullname: Zou, Wenru organization: Guangxi University – sequence: 2 givenname: Wenxin surname: Guo fullname: Guo, Wenxin organization: Guangxi University – sequence: 3 givenname: Xinyi surname: Liu fullname: Liu, Xinyi organization: Guangxi University – sequence: 4 givenname: Yunli surname: Luo fullname: Luo, Yunli organization: Guangxi University – sequence: 5 givenname: Qinglan surname: Ye fullname: Ye, Qinglan organization: Guangxi University – sequence: 6 givenname: Xuetang surname: Xu fullname: Xu, Xuetang email: xxtang@gxu.edu.cn organization: Guangxi University – sequence: 7 givenname: Fan orcidid: 0000-0002-6106-4724 surname: Wang fullname: Wang, Fan email: fanwang@gxu.edu.cn organization: Guangxi University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30326158$$D View this record in MEDLINE/PubMed |
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| Copyright | 2018 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Keywords | electrochemistry anions supercapacitors coulombic efficiency sulfuration ion exchange |
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| Snippet | A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline... A facile and new anion exchange process is presented, which involves the conversion of NiCo‐CO 3 layered double hydroxide (LDH) nanosheet arrays in an alkaline... A facile and new anion exchange process is presented, which involves the conversion of NiCo-CO layered double hydroxide (LDH) nanosheet arrays in an alkaline... A facile and new anion exchange process is presented, which involves the conversion of NiCo-CO3 layered double hydroxide (LDH) nanosheet arrays in an alkaline... |
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| SubjectTerms | anions coulombic efficiency electrochemistry ion exchange sulfuration supercapacitors |
| Title | Anion Exchange of Ni–Co Layered Double Hydroxide (LDH) Nanoarrays for a High‐Capacitance Supercapacitor Electrode: A Comparison of Alkali Anion Exchange and Sulfuration |
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