Durability of Sulfonated Aromatic Polymers for Proton-Exchange-Membrane Fuel Cells

As a key component of proton‐exchange‐membrane fuel cells (PEMFCs), proton‐exchange membranes (PEMs) must continuously withstand very harsh environments during long‐term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are...

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Published inChemSusChem Vol. 4; no. 11; pp. 1526 - 1536
Main Authors Hou, Hongying, Di Vona, Maria Luisa, Knauth, Philippe
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 18.11.2011
WILEY‐VCH Verlag
Subjects
aromatic substitution
degradation
Electric Power Supplies
Electrodes
fuel cells
materials science
Membranes, Artificial
polymers
Polymers - chemistry
Protons
Sulfonic Acids - chemistry
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Abstract As a key component of proton‐exchange‐membrane fuel cells (PEMFCs), proton‐exchange membranes (PEMs) must continuously withstand very harsh environments during long‐term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are becoming more and more urgent and interesting. Herein, various recent attempts and achievements to improve the durability of sulfonated aromatic polymers (SAPs) are reviewed and some further developments are predicted. Extensive investigations into inexpensive SAPs as alternative electrolyte membranes include modification of available polymer materials; design, synthesis, and optimization of new macromolecules; durability testing; and exploring the degradation mechanisms. Long‐lasting power: With the coming commercialization of proton‐exchange‐membrane fuel cells (PEMFCs), investigations into the durability and degradation of PEMs are more urgent (see picture; OCV=open‐circuit voltage). In recent years, increasing attention has been paid to sulfonated aromatic polymers, which are inexpensive, easily available, and promising for fuel cell applications, and the subject of this review.
AbstractList As a key component of proton-exchange-membrane fuel cells (PEMFCs), proton-exchange membranes (PEMs) must continuously withstand very harsh environments during long-term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are becoming more and more urgent and interesting. Herein, various recent attempts and achievements to improve the durability of sulfonated aromatic polymers (SAPs) are reviewed and some further developments are predicted. Extensive investigations into inexpensive SAPs as alternative electrolyte membranes include modification of available polymer materials; design, synthesis, and optimization of new macromolecules; durability testing; and exploring the degradation mechanisms.As a key component of proton-exchange-membrane fuel cells (PEMFCs), proton-exchange membranes (PEMs) must continuously withstand very harsh environments during long-term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are becoming more and more urgent and interesting. Herein, various recent attempts and achievements to improve the durability of sulfonated aromatic polymers (SAPs) are reviewed and some further developments are predicted. Extensive investigations into inexpensive SAPs as alternative electrolyte membranes include modification of available polymer materials; design, synthesis, and optimization of new macromolecules; durability testing; and exploring the degradation mechanisms.
As a key component of proton‐exchange‐membrane fuel cells (PEMFCs), proton‐exchange membranes (PEMs) must continuously withstand very harsh environments during long‐term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are becoming more and more urgent and interesting. Herein, various recent attempts and achievements to improve the durability of sulfonated aromatic polymers (SAPs) are reviewed and some further developments are predicted. Extensive investigations into inexpensive SAPs as alternative electrolyte membranes include modification of available polymer materials; design, synthesis, and optimization of new macromolecules; durability testing; and exploring the degradation mechanisms.
As a key component of proton‐exchange‐membrane fuel cells (PEMFCs), proton‐exchange membranes (PEMs) must continuously withstand very harsh environments during long‐term fuel cell operations. With the coming commercialization of PEMFCs, investigations into the durability and degradation of PEMs are becoming more and more urgent and interesting. Herein, various recent attempts and achievements to improve the durability of sulfonated aromatic polymers (SAPs) are reviewed and some further developments are predicted. Extensive investigations into inexpensive SAPs as alternative electrolyte membranes include modification of available polymer materials; design, synthesis, and optimization of new macromolecules; durability testing; and exploring the degradation mechanisms. Long‐lasting power: With the coming commercialization of proton‐exchange‐membrane fuel cells (PEMFCs), investigations into the durability and degradation of PEMs are more urgent (see picture; OCV=open‐circuit voltage). In recent years, increasing attention has been paid to sulfonated aromatic polymers, which are inexpensive, easily available, and promising for fuel cell applications, and the subject of this review.
Author Knauth, Philippe
Di Vona, Maria Luisa
Hou, Hongying
Author_xml – sequence: 1
  givenname: Hongying
  surname: Hou
  fullname: Hou, Hongying
  organization: Université de Provence-CNRS, UMR 6264: Laboratoire Chimie Provence, 13397 Marseille (France), Fax: (+33) 41355 1850
– sequence: 2
  givenname: Maria Luisa
  surname: Di Vona
  fullname: Di Vona, Maria Luisa
  email: divona@uniroma2.it
  organization: Dip. Scienze de Tecnologie Chimiche, Università di Roma Tor Vergata, Roma (Italy), Fax: (+39) 067259 4328
– sequence: 3
  givenname: Philippe
  surname: Knauth
  fullname: Knauth, Philippe
  email: philippe.knauth@univ-provence.fr
  organization: Université de Provence-CNRS, UMR 6264: Laboratoire Chimie Provence, 13397 Marseille (France), Fax: (+33) 41355 1850
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2004; 243
2009; 44
2004; 127
2007; 107
2009; 42
2001; 185
2007; 304
2006; 39
2005; 259
2010 2010; 122 49
2003; 15
2009; 113
2009; 194
2011; 192
1999; 125
2011; 56
2008; 182
2009; 50
2010; 354
2007; 296
2006; 163
2006; 285
2003; 5
2010; 195
2006; 161
2008; 20
2006; 281
2006; 128
2003; 41
2007; 17
2011; 379
2007; 167
2007; 129
2005; 152
2010; 35
2000; 25
2002; 75
2006; 55
2007; 165
2006; 17
2007; 164
2008; 209
2006; 8
2006; 18
2006; 110
2005; 43
2006; 153
2006; 6
2008; 325
2008; 11
2007; 52
2007; 53
2004; 229
2003; 33
2005; 46
2006; 279
2006; 157
2006; 89
2009; 192
2004; 16
2001; 4
2006; 44
2009; 193
2007; 111
2006; 47
2005; 5
1999; 154
2009; 189
2005; 7
2011; 44
2008; 46
2008; 41
2007; 40
2005; 50
2008; 178
2010; 51
2007; 48
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Snippet As a key component of proton‐exchange‐membrane fuel cells (PEMFCs), proton‐exchange membranes (PEMs) must continuously withstand very harsh environments during...
As a key component of proton-exchange-membrane fuel cells (PEMFCs), proton-exchange membranes (PEMs) must continuously withstand very harsh environments during...
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SubjectTerms aromatic substitution
degradation
Electric Power Supplies
Electrodes
fuel cells
materials science
Membranes, Artificial
polymers
Polymers - chemistry
Protons
Sulfonic Acids - chemistry
Title Durability of Sulfonated Aromatic Polymers for Proton-Exchange-Membrane Fuel Cells
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